Arrays of neutral atoms excited to Rydberg levels have emerged as one of the most promising platforms for quantum computation and simulation. With the hope to outperform classical devices, the number of atoms has been increased by orders of magnitude. However, the interaction time, i.e., the maximum accumulated time during which an atom interacts with its neighbours, has been limited to a few microseconds only. This restrains the number of gates per atom or prevents the simulation of long-time dynamics of quantum many-body systems. Here, we observe the spin-exchange interaction between two spin 1/2s encoded in laser-trapped circular Rydberg atoms over more than $60μs$ and 40 spin-oscillation periods, improving the state of the art by an order of magnitude. These unprecedented timescales allow us to record for weak atomic trapping a collapse and revival of the spin-exchange oscillation contrast induced by spin-motion coupling. Our results constitute the first observation of this coupling with laser-trapped Rydberg atoms. To counteract its detrimental effect for quantum simulation, we demonstrate a novel dynamical decoupling method that prevents the collapse of the spin oscillations. This method exploits the advantages of our recently developed hybrid platform that enables the measurement and the optical manipulation of long-lived circular Rydberg atoms with auxiliary Rydberg atoms. This work opens a direct route to long-duration quantum simulation of strongly-interacting many-body systems.
Arrays of neutral atoms excited to Rydberg levels have emerged as one of the most promising platforms for quantum computation and simulation. With the hope to outperform classical devices, the number of atoms has been increased by orders of magnitude. However, the interaction time, i.e., the maximum accumulated time during which an atom interacts with its neighbours, has been limited to a few microseconds only. This restrains the number of gates per atom or prevents the simulation of long-time dynamics of quantum many-body systems. Here, we observe the spin-exchange interaction between two spin 1/2s encoded in laser-trapped circular Rydberg atoms over more than 60μs and 40 spin-oscillation periods, improving the state of the art by an order of magnitude. These unprecedented timescales allow us to record for weak atomic trapping a collapse and revival of the spin-exchange oscillation contrast induced by spin-motion coupling. Our results constitute the first observation of this coupling with laser-trapped Rydberg atoms. To counteract its detrimental effect for quantum simulation, we demonstrate a novel dynamical decoupling method that prevents the collapse of the spin oscillations. This method exploits the advantages of our recently developed hybrid platform that enables the measurement and the optical manipulation of long-lived circular Rydberg atoms with auxiliary Rydberg atoms. This work opens a direct route to long-duration quantum simulation of strongly-interacting many-body systems.
Rydberg atoms are remarkable tools for quantum simulation and computation. They are the focus of an intense experimental activity, mainly based on low-angular-momentum Rydberg states. Unfortunately, atomic motion and levels lifetime limit the experimental timescale to about 100 μs. Here, we demonstrate two-dimensional laser trapping of long-lived circular Rydberg states for up to 10 ms. Our method is very general and opens many opportunities for quantum technologies with Rydberg atoms. The 10 ms trapping time corresponds to thousands of interaction cycles in a circular-state-based quantum simulator. It is also promising for quantum metrology and quantum information with Rydberg atoms, by bringing atom-field interaction times into unprecedented regimes.
Ultracold molecular systems have recently emerged as a versatile platform for quantum computation and simulation. Spin-exchange interactions arising from direct molecular dipolar interactions constitute the key mechanism for generating quantum entanglement and simulating quantum spin models. However, the relatively small electric dipole moments result in weak spin-exchange couplings, fundamentally limiting the speed of quantum information processing and interaction cycle of many-body dynamics. Here, we introduce a framework that employs Rydberg atoms with large electric dipole moments to mediate strong interactions between molecules in optical tweezer arrays that enables individually laser addressing both the Rydberg atom and molecules. Our result reveals that the mediated coupling can realize an effective molecular spin-exchange interaction with an intrinsic Dzyaloshinskii-Moriya character, with the Rydberg atoms dynamically decoupled from the molecular degrees of freedom, and the effective interaction strength enhanced by up to three orders of magnitude. We further demonstrate its versatility through rapid entanglement generation, high-fidelity two-qubit gate operations, and the realization of non-equilibrium symmetry-protected topological phase with long-lived edge coherence. Our work establishes a route toward strong molecular spin interactions and opens opportunities for fast, scalable quantum information processing and quantum simulation of long-time non-equilibrium quantum many-body physics in optical tweezer arrays of ultracold molecules.
Summary form only given. Quantum simulation offers a highly promising way to understand large correlated quantum systems, and many experimental platforms are now being developed. Rydberg atoms are specially appealing thanks to their strong and short-range dipole-dipole interaction and to their long lifetime. Low-angular momentum Rydberg atoms have been successfully used recently to realize early quantum simulators. These experiments suffer, however, from the limited (despite long) lifetime of these levels and the fact that they cannot be efficiently trapped [1, 2].Here, we propose to use circular Rydberg atoms, i.e., Rydberg atoms with maximum angular momentum, to realize a quantum simulator: A chain of circular atoms is laser trapped inside a spontaneous emission inhibiting structure. A defect-free chain of 40 atoms could be prepared. It is expected to live several seconds inside the inhibition structure. Given the strong interaction frequencies between nearby Rydberg atoms, such a system would, thus, allow us to observe the dynamics of the spin chain over several 10 4 interaction cycles. In addition, the solid state Hamiltonian that would be simulated is fully tuneable experimentally. The proposed circular atoms quantum simulator should therefore open the way towards the simulations of systems and of their dynamics beyond the grasp of classical computation.
This thesis develops and exploits a room-temperature platform for quantum simulation with optically trapped circular Rydberg states of rubidium. The core of the work is a single-element hybrid architecture in which circular states encode the data degree of freedom, while optically accessible low-l Rydberg ancillae enable local addressing, conditional operations, and readout. These capabilities rely on operation near a Förster resonance. A first part of the thesis addresses a major scalability bottleneck of wide-field tweezer arrays: optical aberrations that degrade trap quality away from the optical axis. We present an atom-based method to calibrate a field-dependent wavefront-distortion model. This model is a central component of an array-generation algorithm developed previously within the team, enabling site-wise aberration correction at the programmed tweezer positions. Using the commercial aspheric lens integrated in our experimental setup, we obtain homogeneous, near-diffraction-limited traps over a 150 × 342 µm² field of view, ultimately limited by optical clipping. Building on these tools, we realize hybrid arrays combining bottle-beam traps for circular atoms and Gaussian tweezers for ancilla atoms. We then observe coherent resonant dipole-dipole spin-exchange (flip-flop) dynamics between two circular atoms prepared in |53C;54C⟩. The ancilla layer intervenes at three stages: it enables conditional preparation of the circular-atom pair state, contributes to a post-selection signal that identifies successful runs, and enables readout of the circular data-atom state. Because the ancilla is optically accessible, it provides local control and measurement of otherwise optically dark circular states. These results constitute a proof-of-principle for ancilla-enabled quantum simulation with circular Rydberg atoms in a hybrid platform. They motivate near-term upgrades that directly target the identified limitations, in particular cryogenic operation to access the long intrinsic lifetime of circular states, and efficient motional cooling to prepare atoms close to the motional ground state. By extending coherence times and reducing motion-induced damping, these upgrades would expand the accessible parameter regime and could enable the observation of hundreds of exchange oscillations with near-unit contrast. Combined with the site-resolved local control and non-destructive readout enabled by the ancilla layer, these upgrades would enable larger programmable arrays to probe slow many-body dynamics. With further improvements, for instance in fast and high-fidelity imaging, they would also pave the way for ancilla-assisted mid-circuit measurements.
Among the thriving quantum computation and quantum simulation platforms based on arrays of Rydberg atoms, those using circular Rydberg atoms are particularly promising. These atoms uniquely combine the strong dipole-dipole interactions typical of Rydberg states with long lifetimes. However, low-angular-momentum ( ℓ ) laser-accessible Rydberg levels have been so far mostly used, because circular Rydberg atoms have no optical transitions, hindering their individual detection and manipulation. We remove this limitation with a hybrid platform, combining an array of data laser-trapped circular Rydberg atoms of rubidium with an auxiliary array of Rb ancilla atoms transiently excited to a low- ℓ Rydberg level. We perform a quantum nondemolition detection of the data qubit with the ancilla, through the blockade of the ancilla optical excitation induced by a Förster resonance. Conversely, we locally manipulate the data qubit through the excitation of the ancilla. This dual-Rydberg platform is highly promising for quantum computation and simulation. It adds to the circular-atom toolbox the midcircuit measurements, essential for error correction. More strikingly, it gives access to time correlations in long-term quantum simulations, uniquely accessible to circular Rydberg atoms.
We propose a new paradigm for quantum simulation of spin-1/2 arrays, providing unprecedented flexibility and allowing one to explore domains that remain unexplored, based on laser-trapped circular Rydberg atoms. The long intrinsic atomic lifetimes, combined with the inhibition of their microwave spontaneous emission and their negligible photoionisation, make operation in the minute range realistic. The proposed simulator realizes an XXZ spin-1/2 Hamiltonian, with nearest-neighbour couplings ranging from a few to tens of kilohertz. All the model parameters can be dynamically tuned at will, making a large range of simulations accessible. Thus, the system evolution can be followed long enough to be relevant for ground-state adiabatic preparation and for the study of thermalization and disorder. In this thesis, as a first step towards the implementation of this quantum simulation scheme, we (i) demonstrate the preparation of cold circular Rydberg states in a 4,2 K cryogenic environment with optical access out of a cold atom cloud. Their lifetime reveals an effective microwave black-body temperature of 11±2 K. We (ii) assess the single qubit coherence time (268±5 μs) and lifetime (3,7±0,1 ms), and, finally, we (iii) demonstrate the laser trapping of circular Rydberg atoms to prove their negligible photoionisation at the timescale of 10 ms.