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arXiv:2509.24691 · Physical Review X

Nondestructive Optical Readout and Manipulation of Circular Rydberg Atoms

Yohann Machu, Andrés Durán Hernández, Gautier Creutzer, A. A. Young, J. M. Raimond, M. Brune, C. Sayrin

Published Apr 3, 2026• 1 citation
arXivHTMLPDF

Abstract

Among the thriving quantum computation and quantum simulation platforms based on arrays of Rydberg atoms, those using circular Rydberg atoms are particularly promising. These atoms uniquely combine the strong dipole-dipole interactions typical of Rydberg states with long lifetimes. However, low-angular-momentum ( ℓ ) laser-accessible Rydberg levels have been so far mostly used, because circular Rydberg atoms have no optical transitions, hindering their individual detection and manipulation. We remove this limitation with a hybrid platform, combining an array of data laser-trapped circular Rydberg atoms of rubidium with an auxiliary array of Rb ancilla atoms transiently excited to a low- ℓ Rydberg level. We perform a quantum nondemolition detection of the data qubit with the ancilla, through the blockade of the ancilla optical excitation induced by a Förster resonance. Conversely, we locally manipulate the data qubit through the excitation of the ancilla. This dual-Rydberg platform is highly promising for quantum computation and simulation. It adds to the circular-atom toolbox the midcircuit measurements, essential for error correction. More strikingly, it gives access to time correlations in long-term quantum simulations, uniquely accessible to circular Rydberg atoms.

DOI
10.1103/st3l-14d7

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Among the thriving quantum computation and quantum simulation platforms based on arrays of Rydberg atoms, those using circular Rydberg atoms are particularly promising. These atoms uniquely combine the strong dipole-dipole interactions typical of Rydberg states with long lifetimes. However, low-angular-momentum ( ℓ ) laser-accessible Rydberg levels have been so far mostly used, because circular Rydberg atoms have no optical transitions, hindering their individual detection and manipulation. We remove this limitation with a hybrid platform, combining an array of data laser-trapped circular Rydberg atoms of rubidium with an auxiliary array of Rb ancilla atoms transiently excited to a low- ℓ Rydberg level. We perform a quantum nondemolition detection of the data qubit with the ancilla, through the blockade of the ancilla optical excitation induced by a Förster resonance. Conversely, we locally manipulate the data qubit through the excitation of the ancilla. This dual-Rydberg platform is highly promising for quantum computation and simulation. It adds to the circular-atom toolbox the midcircuit measurements, essential for error correction. More strikingly, it gives access to time correlations in long-term quantum simulations, uniquely accessible to circular Rydberg atoms.
This thesis develops and exploits a room-temperature platform for quantum simulation with optically trapped circular Rydberg states of rubidium. The core of the work is a single-element hybrid architecture in which circular states encode the data degree of freedom, while optically accessible low-l Rydberg ancillae enable local addressing, conditional operations, and readout. These capabilities rely on operation near a Förster resonance. A first part of the thesis addresses a major scalability bottleneck of wide-field tweezer arrays: optical aberrations that degrade trap quality away from the optical axis. We present an atom-based method to calibrate a field-dependent wavefront-distortion model. This model is a central component of an array-generation algorithm developed previously within the team, enabling site-wise aberration correction at the programmed tweezer positions. Using the commercial aspheric lens integrated in our experimental setup, we obtain homogeneous, near-diffraction-limited traps over a 150 × 342 µm² field of view, ultimately limited by optical clipping. Building on these tools, we realize hybrid arrays combining bottle-beam traps for circular atoms and Gaussian tweezers for ancilla atoms. We then observe coherent resonant dipole-dipole spin-exchange (flip-flop) dynamics between two circular atoms prepared in |53C;54C⟩. The ancilla layer intervenes at three stages: it enables conditional preparation of the circular-atom pair state, contributes to a post-selection signal that identifies successful runs, and enables readout of the circular data-atom state. Because the ancilla is optically accessible, it provides local control and measurement of otherwise optically dark circular states. These results constitute a proof-of-principle for ancilla-enabled quantum simulation with circular Rydberg atoms in a hybrid platform. They motivate near-term upgrades that directly target the identified limitations, in particular cryogenic operation to access the long intrinsic lifetime of circular states, and efficient motional cooling to prepare atoms close to the motional ground state. By extending coherence times and reducing motion-induced damping, these upgrades would expand the accessible parameter regime and could enable the observation of hundreds of exchange oscillations with near-unit contrast. Combined with the site-resolved local control and non-destructive readout enabled by the ancilla layer, these upgrades would enable larger programmable arrays to probe slow many-body dynamics. With further improvements, for instance in fast and high-fidelity imaging, they would also pave the way for ancilla-assisted mid-circuit measurements.
Rydberg atoms are particularly well suited for quantum simulation, due to their strong dipole-dipole interactions over distances of a few microns. Defect-free arrays of Rydberg atoms are now being used in many experimental setups. However, these systems are typically constrained to simulation durations of only a few microseconds, limited by the lifetime of the laser-accessible states used. Circular Rydberg atoms (CRA), on the other hand, possess a natural lifetime up to a hundred times longer, extending to several tens of milliseconds. They offer the perspective to run quantum simulation over unprecedented timescales [1]. While the absence of optical transitions from circular Rydberg levels ensures their longevity, it also prevents their optical manipulation and readout required for local operations and measurements-key components of quantum simulation.
Large-scale Rydberg atom arrays are used for highly coherent analogue quantum simulations and for digital quantum computations. However, advanced quantum protocols, such as quantum error correction, require midcircuit qubit operations, including the replenishment, reset and read-out of a subset of qubits. A compelling strategy for unlocking these capabilities is a dual-species architecture in which a second atomic species is controlled independently and entangled with the first through Rydberg interactions. Here, we realize a dual-species Rydberg array consisting of rubidium and caesium atoms and explore regimes of interactions and dynamics not accessible in single-species architectures. We achieve enhanced interspecies interactions by electrically tuning the Rydberg states close to a Förster resonance. In this regime, we demonstrate an interspecies Rydberg blockade and implement a quantum state transfer from one species to another. We then generate a Bell state between Rb and Cs hyperfine qubits through an interspecies controlled-phase gate. Finally, we combine interspecies entanglement with a native midcircuit read-out to achieve quantum non-demolition measurements. Rydberg atoms in optical tweezers are a promising platform for quantum information science. A platform composed of dual-species Rydberg arrays has been realized, offering access to unexplored interaction regimes and crosstalk-free midcircuit control.
Arrays of neutral atoms excited to Rydberg levels have emerged as one of the most promising platforms for quantum computation and simulation. With the hope to outperform classical devices, the number of atoms has been increased by orders of magnitude. However, the interaction time, i.e., the maximum accumulated time during which an atom interacts with its neighbours, has been limited to a few microseconds only. This restrains the number of gates per atom or prevents the simulation of long-time dynamics of quantum many-body systems. Here, we observe the spin-exchange interaction between two spin 1/2s encoded in laser-trapped circular Rydberg atoms over more than 60μs60μs60μs and 40 spin-oscillation periods, improving the state of the art by an order of magnitude. These unprecedented timescales allow us to record for weak atomic trapping a collapse and revival of the spin-exchange oscillation contrast induced by spin-motion coupling. Our results constitute the first observation of this coupling with laser-trapped Rydberg atoms. To counteract its detrimental effect for quantum simulation, we demonstrate a novel dynamical decoupling method that prevents the collapse of the spin oscillations. This method exploits the advantages of our recently developed hybrid platform that enables the measurement and the optical manipulation of long-lived circular Rydberg atoms with auxiliary Rydberg atoms. This work opens a direct route to long-duration quantum simulation of strongly-interacting many-body systems.
Circular Rydberg atoms (CRAs), i.e., Rydberg atoms with maximal orbital momentum, are highly promising for quantum computation, simulation, and sensing. They combine long natural lifetimes with strong interatomic interactions and coupling to electromagnetic fields. Trapping individual CRAs is essential to harness these unique features. We report the first demonstration of CRAs laser trapping in a programmable array of optical bottle beams. We observe the decay of a trapped rubidium circular level over 5 ms using a novel optical detection method. This first optical detection of alkali CRAs is both spatially and level selective. We finally observe the mechanical oscillations of the CRAs in the traps. This work opens the route to the use of circular levels in quantum devices. It is also promising for quantum simulation and information processing using the full extent of Rydberg manifolds.
Summary form only given. Quantum simulation offers a highly promising way to understand large correlated quantum systems, and many experimental platforms are now being developed. Rydberg atoms are specially appealing thanks to their strong and short-range dipole-dipole interaction and to their long lifetime. Low-angular momentum Rydberg atoms have been successfully used recently to realize early quantum simulators. These experiments suffer, however, from the limited (despite long) lifetime of these levels and the fact that they cannot be efficiently trapped [1, 2].Here, we propose to use circular Rydberg atoms, i.e., Rydberg atoms with maximum angular momentum, to realize a quantum simulator: A chain of circular atoms is laser trapped inside a spontaneous emission inhibiting structure. A defect-free chain of 40 atoms could be prepared. It is expected to live several seconds inside the inhibition structure. Given the strong interaction frequencies between nearby Rydberg atoms, such a system would, thus, allow us to observe the dynamics of the spin chain over several 10 4 interaction cycles. In addition, the solid state Hamiltonian that would be simulated is fully tuneable experimentally. The proposed circular atoms quantum simulator should therefore open the way towards the simulations of systems and of their dynamics beyond the grasp of classical computation.