Circular Rydberg atoms (CRAs), i.e., Rydberg atoms with maximal orbital momentum, are highly promising for quantum computation, simulation, and sensing. They combine long natural lifetimes with strong interatomic interactions and coupling to electromagnetic fields. Trapping individual CRAs is essential to harness these unique features. We report the first demonstration of CRAs laser trapping in a programmable array of optical bottle beams. We observe the decay of a trapped rubidium circular level over 5 ms using a novel optical detection method. This first optical detection of alkali CRAs is both spatially and level selective. We finally observe the mechanical oscillations of the CRAs in the traps. This work opens the route to the use of circular levels in quantum devices. It is also promising for quantum simulation and information processing using the full extent of Rydberg manifolds.
Circular Rydberg atoms (CRAs), i.e., Rydberg atoms with maximal orbital momentum, are highly promising for quantum computation, simulation, and sensing. They combine long natural lifetimes with strong interatomic interactions and coupling to electromagnetic fields. Trapping individual CRAs is essential to harness these unique features. We report the first demonstration of CRAs laser trapping in a programmable array of optical bottle beams. We observe the decay of a trapped rubidium circular level over 5 ms using a novel optical detection method. This first optical detection of alkali CRAs is both spatially and level selective. We finally observe the mechanical oscillations of the CRAs in the traps. This work opens the route to the use of circular levels in quantum devices. It is also promising for quantum simulation and information processing using the full extent of Rydberg manifolds.
Circular Rydberg atoms (CRAs), i.e., Rydberg atoms with maximal orbital momentum, ideally combine long coherence times and strong interactions, a key property of quantum systems, in particular for the development of quantum technologies. However, the dipole-dipole interaction between CRAs has not been observed so far. We report the measurement and characterization of the resonant dipole-dipole interaction between two CRAs, individually trapped in optical tweezers, and find excellent agreement with theoretical predictions. We demonstrate a dynamic control over the strength of the interaction by tuning the orientation of an electric field. We use the interaction between the CRAs as a meter for the interatomic distance, and record the relative motion between two atoms in their traps. This motion, that we induce through the interaction between Rydberg levels with permanent electric dipoles, transiently populated during the preparation of the circular states, is a signature of spin-motion coupling.
Circular Rydberg atoms, with their long lifetimes and adjustable strong dipolar interactions, are promising candidates for the implementation of quantum simulations in regimes that were previously out of reach. A new quantum simulator paradigm, based on qubits encoded in circular states, would implement an XXZ spin-1/2 Hamiltonian with dynamically adjustable parameters over a wide range of values. This thesis addresses the preliminary steps in constructing such a quantum simulator. First, we present the realization of two-dimensional arrays of optically-trapped circular Rydberg atoms with arbitrary geometries. For this purpose, we prepare arrays of ultra-cold rubidium atoms, individually trapped in optical tweezers. An additional beam with adjustable position allows us to rearrange the atoms within the array to implement the desired geometry in a deterministic manner. We then excite the atoms to the circular state with principal quantum number n=52, while trapping them in hollow beams using the ponderomotive force. These experimental capabilities allowed us to control and characterize, for the first time, the dipolar interactions between circular states, within pairs of individually trapped atoms. We showed the good agreement of these measurements with theoretical expectations and highlighted their dependence on the system's geometry. This experimental study is coupled to an investigation of the motion of the circular atoms within their traps.
Stability achieved by large angular momentum is ubiquitous in nature, with examples ranging from classical mechanics, over optics and chemistry, to nuclear physics. In atoms, angular momentum can protect excited electronic orbitals from decay due to selection rules. This manifests spectacularly in highly excited Rydberg states. Low angular momentum Rydberg states are at the heart of recent breakthroughs in quantum computing, simulation and sensing with neutral atoms. For these applications the lifetime of the Rydberg levels sets fundamental limits for gate fidelities, coherence times, or spectroscopic precision. The quest for longer Rydberg state lifetimes has motivated the generation, coherent control and trapping of circular Rydberg atoms, which are characterized by the maximally allowed electron orbital momentum and were key to seminal experiments with single atoms and photons. Here, we report the observation of individually trapped circular Rydberg atoms with lifetimes of more than 10 milliseconds, two orders of magnitude longer-lived than the established low angular momentum orbitals. This is achieved via Purcell suppression of blackbody modes at room temperature. We coherently control individual circular Rydberg levels at so far elusive principal quantum numbers of up to n = 103, and observe tweezer trapping of the Rydberg atoms on the hundred millisecond scale. Our results pave the way for quantum information processing and sensing utilizing the combination of extreme lifetimes and giant Rydberg blockade.
Stability achieved by large angular momentum is ubiquitous in nature, with examples ranging from classical mechanics, over optics and chemistry, to nuclear physics. In atoms, angular momentum can protect excited electronic orbitals from decay due to selection rules. This manifests spectacularly in highly excited Rydberg states. Low angular momentum Rydberg states are at the heart of recent breakthroughs in quantum computing, simulation and sensing with neutral atoms. For these applications the lifetime of the Rydberg levels sets fundamental limits for gate fidelities, coherence times, or spectroscopic precision. The quest for longer Rydberg state lifetimes has motivated the generation, coherent control and trapping of circular Rydberg atoms, which are characterized by the maximally allowed electron orbital momentum and were key to seminal experiments with single atoms and photons. Here, we report the observation of individually trapped circular Rydberg atoms with lifetimes of more than 10 milliseconds, two orders of magnitude longer-lived than the established low angular momentum orbitals. This is achieved via Purcell suppression of blackbody modes at room temperature. We coherently control individual circular Rydberg levels at so far elusive principal quantum numbers of up to n = 103, and observe tweezer trapping of the Rydberg atoms on the hundred millisecond scale. Our results pave the way for quantum information processing and sensing utilizing the combination of extreme lifetimes and giant Rydberg blockade.
In recent years, advances in optical tweezers arrays have enabled the trapping and control of individual atoms. This makes it possible to simulate condensed matter systems by arranging atoms in an array that mimics the crystalline structure of real materials. This approach, known as quantum simulation, was first envisioned by R. Feynman and is now being implemented by several research groups worldwide. In order to induce interactions between atoms, they are prepared in highly excited atomic states, known as Rydberg states. In particular, circular Rydberg states, which possess maximal angular momentum, exhibit lifetimes of several milliseconds, much longer than those of other Rydberg states. This property makes them particularly interesting for the development of new quantum technologies. In this work, we present the first building blocks of a quantum simulator based on circular Rydberg states of strontium atoms. This includes the development of a new cryogenic apparatus in which individual strontium atoms are trapped in optical tweezers. Using an alkaline-earth element allows us to exploit its two valence electrons for different tasks. One electron is excited to the circular state with principal quantum number n = 52, while the ionic core behaves as a Sr+ ion, which can be directly trapped by the tweezers. Moreover, we observe coherent oscillations between singlet and triplet spin states, due to the spin-orbit coupling of the electron in the circular state. These oscillations allow us to measure, with high precision, QED corrections to the Landé g5S1/2 factor of the ground state of Sr+.
Quantum simulation offers interesting perspectives for the understanding of complex systems that are out of reach for numerical approaches. In this line, a new quantum simulation platform has recently been proposed. A spin-1/2 XXZ hamiltonian is thus realized in which the parameters can be controlled over a large range. The spin states are encoded by circular Rydberg states coupled through dipole-dipole interaction. These states benefit from longer lifetimes compared to the low angular momentum states used for current quantum simulations. In addition, they can be laser-trapped through the ponderomotive effect, and their lifetime can be further enhanced by spontaneous emission inhibition. We present in this thesis the first step towards the implementation of the proposed quantum simulator. We first prepare an array of rubidium 87 atoms trapped individually in optical tweezers. These atoms are subsequently excited to the circular Rydberg state n = 52 and transferred to hollow bottle-beam traps. We thus demonstrate the ponderomotive trapping of these states over durations of several milliseconds. We take advantage of the optical detection of the states thus prepared with various experiments. We characterize the trapping potential by measuring its transverse frequency. We finally conclude with the coherent manipulation of these trapped circular states through Rabi oscillations and Ramsey interferometry to determine their coherence.