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arXiv:2609.31865

Systematic errors from scalar slowing-down models in transient SERF magnetometry

Marek Kopciuch, Harini Raghavan, Morgan W. Mitchell

physics.atom-phquant-phSubmitted Sep 25, 2026• Announced Sep 29, 2026• 0 citations
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Abstract

Reduced Bloch models of spin-exchange-relaxation-free (SERF) magnetometers commonly describe the coupled electron--nuclear spin dynamics using a single nuclear slowing-down factor. We show that this scalar description becomes inaccurate when the polarization magnitude changes appreciably. We derive an effective Bloch equation with separate longitudinal and transverse slowing-down factors, $q_\parallel(P)$ and $q_\perp(P)$, governing changes in polarization magnitude and direction. For $^{87}\mathrm{Rb}$ under representative SERF conditions and undergoing free-induction decay (FID), comparison with master-equation simulations shows that the dynamic scalar model produces a magnetic-field estimation bias of up to $4.2\%$ at high initial polarization, while fixing the slowing-down factor at a reference value increases the error to $10.1\%$. Lowering the polarization suppresses this bias but also reduces the magnetic-field information contained in the FID signal. We further show that the anisotropic response modifies noncollinear optical pumping and introduces an additional nonlinear contribution to the harmonic response under periodic driving. The resulting model retains the simplicity of a three-component Bloch description while improving the quantitative accuracy of transient and driven SERF magnetometry.

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Reduced Bloch models of spin-exchange-relaxation-free (SERF) magnetometers commonly describe the coupled electron--nuclear spin dynamics using a single nuclear slowing-down factor. We show that this scalar description becomes inaccurate when the polarization magnitude changes appreciably. We derive an effective Bloch equation with separate longitudinal and transverse slowing-down factors, q∥(P)q_\parallel(P)q∥​(P) and q⊥(P)q_\perp(P)q⊥​(P), governing changes in polarization magnitude and direction. For 87Rb^{87}\mathrm{Rb}87Rb under representative SERF conditions and undergoing free-induction decay (FID), comparison with master-equation simulations shows that the dynamic scalar model produces a magnetic-field estimation bias of up to 4.2%4.2\%4.2% at high initial polarization, while fixing the slowing-down factor at a reference value increases the error to 10.1%10.1\%10.1%. Lowering the polarization suppresses this bias but also reduces the magnetic-field information contained in the FID signal. We further show that the anisotropic response modifies noncollinear optical pumping and introduces an additional nonlinear contribution to the harmonic response under periodic driving. The resulting model retains the simplicity of a three-component Bloch description while improving the quantitative accuracy of transient and driven SERF magnetometry.
Nuclear slowing-down factors account for the sharing of angular momentum between the electron and the nucleus in the effective Bloch description of alkali-metal spin dynamics in the spin-exchange-relaxation-free (SERF) regime. For collinear optical pumping and magnetic field, we find that longitudinal and transverse spin dynamics are characterized by different polarization-dependent slowing-down factors. Transverse dynamics are governed by the conventional factor q(p)q(p)q(p), with ppp the electron spin polarization, whereas longitudinal relaxation is governed by q(p)+p dq(p)/dpq(p)+p\,dq(p)/dpq(p)+pdq(p)/dp. The two factors coincide at zero polarization but differ substantially at high polarization, where the single-factor description overestimates the underlying pumping and relaxation rates inferred from longitudinal transients by factors approaching two to four, depending on the nuclear spin. We further derive closed-form expressions, valid at arbitrary polarization, for the residual spin-exchange relaxation of the transverse spin components at finite magnetic field along the pumping axis. This contribution is quadratic in the magnetic field and can become comparable to the zero-field linewidth at fields well within the SERF regime. The results are obtained by perturbation theory on the density-matrix dynamics linearized around the stationary state and are verified by numerical solutions of the microscopic density-matrix equation. These findings refine the effective Bloch description of alkali-metal spin dynamics and are directly relevant to atomic magnetometers and alkali-metal--noble-gas comagnetometers, including those used in precision searches for physics beyond the Standard Model.
It is demonstrated that a spin-exchange relaxation-free (SERF) atomic magnetometer can be used for scalar measurements with no additional hardware. Because of relaxation processes, an ensemble of alkali atoms needs a constant supply of polarized photons by a pump beam to maintain a polarized state. If the pump beam is shuttered off, the system decays to its equilibrium state. For a low enough relaxation rate and with a magnetic field present, the system will exhibit oscillations at its natural frequencies. In a SERF magnetometer, it happens at the Zeeman resonance frequency of the atoms (Larmor frequency). Thus, shuttering off the pump beam reveals oscillations at the Larmor frequency. From this frequency, one can deduce the scalar value of the applied magnetic field. As a result, all-optical scalar measurements can be performed. At the same time, either one or two vector components of the applied field can be measured by using one or two orthogonal probe beams, respectively. In a low-polarization SERF regime, the ground state can be well described by the Bloch equations for the electron spin polarization. By solving the time-dependent Bloch equations [neglecting the diffusion term and assuming that the nuclear slowing-down factor q(P) is constant], the oscillation frequency of the system is obtained. From this frequency, the scalar value of the applied magnetic field is derived. It is shown that applied fields down to 1 nT can be measured with a 0.1% relative uncertainty. Fields down to 50 pT can be measured with a 10% relative uncertainty. The time dependence acquired in the “off” periods is strongly correlated with the Zeeman sublevels population of the atomic ground state and reveals its spin dynamics.
Abstract Spin-exchange relaxation-free (SERF) co-magnetometers have promising applications in both inertial navigation and fundamental physics experiments. However, the fluctuation in the spin polarization caused by the probe beam has a non-negligible influence on the co-magnetometer signal. In this paper, a theoretical model containing three parameters of the probe beam is established by extending the coupled Bloch equation. Based on this model, the influence of probe power density on the transient and steady-state response of the SERF co-magnetometer is analyzed. According to the transient response model, a new measurement method for transverse optical pumping of the probe beam is proposed. Then, for the steady-state response model, a steady-state error suppression method is suggested by adjusting the degree of circular polarization of the probe beam. Eventually, the suppression method is used to refine the SERF co-magnetometer, achieving a suppression rate of 70.31% in transverse electron spin polarization fluctuations, thus improving the co-magnetometer to a stability of 0.0079∘ h−1. To our knowledge, this is better than what has been reported so far.
Abstract Spin-exchange (SE) and spin-destruction (SD) collisions play a central role in determining the coherence properties of alkali-metal vapors and the performance of alkali-metal magnetometers in external magnetic fields. In this work, we investigate how these collisions influence spin relaxation dynamics and magnetometric response using a generalized Bloch equation that fully accounts for the coupled evolution of spin polarizations in different hyperfine manifolds. Our results show that in the low-field regime, both SE and SD collisions contribute to the suppression of transverse spin relaxation and the slowdown of spin precession, whereas longitudinal relaxation depends weakly on the SE rate and is predominantly governed by SD interactions. Building on the established relationship between spin relaxation rates and magnetometric response, we further analyze how SE and SD collisions affect the performance of two representative magnetometer architectures: the spin-exchange relaxation-free (SERF) magnetometer and the magnetic-resonance Mx-type magnetometer. The SERF magnetometer’s response is found to be primarily determined by the SD rate, with only minor dependence on the nuclear spin quantum number. In contrast, the magnetic-resonance Mx-type magnetometer’s sensitivity is significantly affected by both the magnetic field strength and the SE rate. While the resonance linewidth decreases with reduced magnetic field, the associated measurement accuracy deteriorates markedly. Consequently, reliable magnetic field reconstruction is only achievable in the high-field regime, where the Larmor frequency greatly exceeds the SE rate.
The magnetic field gradient within optical pumping magnetometers (OPMs) suppresses sensitivity improvement. We investigated the effects of the magnetic field gradient along the x-, y-, and z-axes on the limiting factors of magnetometers under extremely low magnetic field conditions. We modified the magnetic field gradient relaxation model such that it can be applied to atoms in the spin exchange relaxation free (SERF) regime. The gradient relaxation time and spin polarizations, combined with fast spin-exchange interaction, were determined simultaneously using the oscillating cosine magnetic field excitation and amplitude spectrum analysis method. During the experiments, we eliminated the errors caused by the temperature and pumping power, and considered different isotope spin exchange collisions in naturally abundant Rb during the data analysis to improve the fitting accuracy. The experimental results agreed well with those of theoretical calculations and confirmed the accuracy of the improved model. The contribution of the transverse magnetic field gradient to the relaxation of the magnetic field gradient cannot be ignored in the case of small static magnetic fields. Our study provides a theoretical and experimental basis for eliminating magnetic gradient relaxation in atomic sensors in the SERF region.
The magnitude of the electron spin-relaxation rate Rrel of the atomic ensemble directly affects the sensitivity of the spin-exchange relaxation-free (SERF) atomic magnetometer (AM). The rapid and in-situ characterization of Rrel is of great importance. In this work, a fast extraction method of Rrel is proposed with a measurement period shorten to 0.5 s, merely detecting the transient response of SERF AM to a transverse DC excitation magnetic field after switching off the pump beam. In contrast to the conventional methods based on the measurement of the magnetic resonance linewidth, this method circumvents the involvement of optical pumping rate, and enables monitoring Rrel under arbitrary polarization, which is expected to improve the authenticity of Rrel measurement in a more convenient way.