Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

Journal of Physics D Applied Physics

Probe beam influence on spin polarization in spin-exchange relaxation-free co-magnetometers

Yao Wei, Xing Li, Yueyang Zhai, Wenfeng Fan, Chi Fang, Feng Liu, Wei Quan

Published Feb 20, 2023• 5 citations
Publisher

Abstract

Abstract Spin-exchange relaxation-free (SERF) co-magnetometers have promising applications in both inertial navigation and fundamental physics experiments. However, the fluctuation in the spin polarization caused by the probe beam has a non-negligible influence on the co-magnetometer signal. In this paper, a theoretical model containing three parameters of the probe beam is established by extending the coupled Bloch equation. Based on this model, the influence of probe power density on the transient and steady-state response of the SERF co-magnetometer is analyzed. According to the transient response model, a new measurement method for transverse optical pumping of the probe beam is proposed. Then, for the steady-state response model, a steady-state error suppression method is suggested by adjusting the degree of circular polarization of the probe beam. Eventually, the suppression method is used to refine the SERF co-magnetometer, achieving a suppression rate of 70.31% in transverse electron spin polarization fluctuations, thus improving the co-magnetometer to a stability of 0.0079∘ h−1. To our knowledge, this is better than what has been reported so far.

DOI
10.1088/1361-6463/acbd60

Related papers

Transverse light-shift in a spin-exchange relaxation-free co-magnetometer: measurement, decoupling, and suppression

Sixun Liu, Ruigang Wang, Linlin Yuan +6 more

The transverse light-shift can induce non-negligible polarization error in the output signal of spin-exchange relaxation-free (SERF) co-magnetometer. In this paper, a novel method for rapid measurement of transverse light-shift based on the error of steady-state response of co-magnetometer is proposed firstly, then the sources of transverse light-shift in a compact SERF co-magnetometer is modeled and analyzed from three aspects: the non-ideal linear polarization of probe laser, the circular dichroism of the atomic spin ensembles, and the stress-induced birefringence effect of the cell wall. Furthermore, the decoupling and suppression methods of transverse light-shift based on a degree of circular polarization (DOCP) regulation scheme is presented, to realize the decoupling measurement of the transverse light-shift introduced by the whole co-magnetometer cell, and cancel it out with the non-ideal linear polarization of the probe laser. Eventually, the DOCP regulation scheme suggested in this paper achieves more than a 67% suppression ratio in transverse light-shift, and the short- and long-term performance of SERF co-magnetometer are improved due to the reduction of the coupling effect between the probe laser power and transverse field. Moreover, the measurement, decoupling and suppression methods provided in this paper also have the potential to be applied to other atomic sensors, such as the SERF magnetometers and nuclear spin co-magnetometers.

Optics Express•Apr 8, 2022•32 citations

Nonlinear Effect Analysis and Sensitivity Improvement in Spin Exchange Relaxation Free Atomic Magnetometers

Bozheng Xing, Ning Ma, Haoran Lv +1 more

Abstract In this study, the influence of the nonlinear magneto–optical rotation effect on a spin‐exchange relaxation‐free (SERF) atomic magnetometer is analyzed. The nonlinear effect is described by saturation parameters obtained from the density matrix model considering the Rabi oscillation of the probe light. For better sensitivity, the nonlinear effect is suppressed, and larger output signals are achieved. Based on the nonlinear effect analysis, the relationship between the probe sensitivity and light power density is obtained, and the optimal probe light power density is measured with best probe sensitivity. The best probe sensitivity improves by ≈6 times at the optimal probe light power density compared with that in the conventional linear optical rotation detection. The proposed method can be applied to SERF magnetometers, co‐magnetometers, and atomic spin gyroscopes.

Advanced Quantum Technologies•Jul 25, 2024•7 citations

Comprehensive analysis of the impact of optical magnetic misalignment on the performance of the SERF co-magnetometer

Ze Yu Cai, Lihong Duan, Shimiao Fan +2 more

The ultra-sensitive atomic co-magnetometer based on the spin-exchange relaxation-free (SERF) regime is a valuable tool for inertial measurements and fundamental physics research. However, the optical magnetic misalignment effect is a significant source of error in SERF co-magnetometers, limiting their magnetic field suppression ability and long-term stability. This paper establishes a response model of angular velocity and magnetic field for the SERF co-magnetometer. The impact of optical magnetic misalignment on the scale factor, magnetic field amplitude-frequency response, and angular velocity errors caused by magnetic noise is systematically investigated. The results indicate that the scale factor and magnetic field suppression ability decrease as the optical magnetic misalignment angle increases, while the angular velocity errors caused by magnetic noise increase as the misalignment angle increases. Finally, experimental results demonstrate that the optical-magnetic misalignment effect significantly compromises the long-term stability of SERF co-magnetometers, underscoring its substantial influence on the overall performance. This work contributes to understanding the mechanism of optical magnetic misalignment effects on the SERF co-magnetometer and enhances its performance.

Optics Express•Apr 10, 2025•4 citations

Polarization measurement of Cs using the pump laser beam

Jiancheng Fang, Rujie Li, Lihong Duan +2 more

In the optical pumping systems based on the pump-probe arrangement, the spin polarization of the atoms is generally monitored utilizing the probe laser beam, in which way an extra perturbation must be introduced and thus affects the normal operation of the sensors. By investigating the absorption rate of the circularly polarized pump laser, here we demonstrate the feasibility of extracting the electron-spin polarization from the transmitted pump laser intensity. We experimentally validate the method in a spin-exchange relaxation free (SERF) magnetometer and the results are in excellent agreement with the theory. The scheme operates in a silent mode and features a real-time observation. We also study the corresponding magnetic field response of the SERF magnetometer and a term arising from the diffusion effects has been added to the original model to explain the discrepancy of the response.

arXiv:1510.00885•Oct 3, 2015•0 citations

Measurement of Equilibrium Spin Polarization in Spin-Exchange Relaxation-Free Atomic Magnetometers via the Steady-State Response to the Triaxial Magnetic Field

Faming Wang, Xiujie Fang, Bozheng Xing +5 more

This study proposes an in situ method for measuring the equilibrium spin polarization and its longitudinal spatial distribution in a spin-exchange relaxation-free (SERF) atomic magnetometer. The total relaxation rate was determined by analyzing the steady-state response of the magnetometer to the triaxial magnetic field. The transfer coefficient between spin polarization along the probe beam axis and the steady-state response was derived from the optical depth of the probe light and the incident/transmitted power through the vapor cell. By applying a DC magnetic field along the sensitive axis and combining the total relaxation rate with the transfer coefficient, the equilibrium spin polarization value under zero-field conditions was obtained. The equilibrium spin polarization distribution along the pump beam propagation direction was measured, showing consistent trends with simulation results, with a maximum relative error of less than 5%. The expanded uncertainty of the proposed equilibrium spin polarization measurement method ranges from 0.8% to 9.7%. The advantages of this method include no requirement for additional optical field or magnetic field modulation, immunity to temperature and temperature gradients, and the capability to directly determine the equilibrium spin polarization value.

IEEE Transactions on Instrumentation and Measurement•Jan 1, 2025•7 citations

Effect of Optical Nonorthogonality on Dynamic Response in Dual-Beam Atomic Magnetometer

Bozheng Xing, Siran Li, Xiujie Fang +2 more

In this article, we analyze the amplitude-frequency and phase-frequency responses of a spin-exchange relaxation-free (SERF) atomic magnetometer with the nonorthogonal angle between the pump and probe beam. The optical nonorthogonality leads to a change in the photon spin direction of circularly polarized pump light, which decides the polarization direction of the atomic ensemble, causing significant differences in dynamic responses to the magnetic field. We theoretically analyze relationships between dynamic response solutions of the Bloch equation with different pump lights and magnetic field directions based on which the equations are linearized. The equations are solved with the Fourier transform method, and three-axis dynamic responses are obtained under the influences of optical nonorthogonality and residual static magnetic field. In the experiment, we verify the linear superposition characteristics between different response components. According to the results, we propose a novel method to quickly calibrate the nonorthogonal angle, which could reduce the optical nonorthogonal angle by 20 times, reaching 0.54°, and effectively enhance the dynamic magnetic field response signal in atomic magnetometers.

IEEE Transactions on Instrumentation and Measurement•Nov 25, 2024•7 citations
Abstract Spin-exchange relaxation-free (SERF) co-magnetometers have promising applications in both inertial navigation and fundamental physics experiments. However, the fluctuation in the spin polarization caused by the probe beam has a non-negligible influence on the co-magnetometer signal. In this paper, a theoretical model containing three parameters of the probe beam is established by extending the coupled Bloch equation. Based on this model, the influence of probe power density on the transient and steady-state response of the SERF co-magnetometer is analyzed. According to the transient response model, a new measurement method for transverse optical pumping of the probe beam is proposed. Then, for the steady-state response model, a steady-state error suppression method is suggested by adjusting the degree of circular polarization of the probe beam. Eventually, the suppression method is used to refine the SERF co-magnetometer, achieving a suppression rate of 70.31% in transverse electron spin polarization fluctuations, thus improving the co-magnetometer to a stability of 0.0079∘ h−1. To our knowledge, this is better than what has been reported so far.
The transverse light-shift can induce non-negligible polarization error in the output signal of spin-exchange relaxation-free (SERF) co-magnetometer. In this paper, a novel method for rapid measurement of transverse light-shift based on the error of steady-state response of co-magnetometer is proposed firstly, then the sources of transverse light-shift in a compact SERF co-magnetometer is modeled and analyzed from three aspects: the non-ideal linear polarization of probe laser, the circular dichroism of the atomic spin ensembles, and the stress-induced birefringence effect of the cell wall. Furthermore, the decoupling and suppression methods of transverse light-shift based on a degree of circular polarization (DOCP) regulation scheme is presented, to realize the decoupling measurement of the transverse light-shift introduced by the whole co-magnetometer cell, and cancel it out with the non-ideal linear polarization of the probe laser. Eventually, the DOCP regulation scheme suggested in this paper achieves more than a 67% suppression ratio in transverse light-shift, and the short- and long-term performance of SERF co-magnetometer are improved due to the reduction of the coupling effect between the probe laser power and transverse field. Moreover, the measurement, decoupling and suppression methods provided in this paper also have the potential to be applied to other atomic sensors, such as the SERF magnetometers and nuclear spin co-magnetometers.
Abstract In this study, the influence of the nonlinear magneto–optical rotation effect on a spin‐exchange relaxation‐free (SERF) atomic magnetometer is analyzed. The nonlinear effect is described by saturation parameters obtained from the density matrix model considering the Rabi oscillation of the probe light. For better sensitivity, the nonlinear effect is suppressed, and larger output signals are achieved. Based on the nonlinear effect analysis, the relationship between the probe sensitivity and light power density is obtained, and the optimal probe light power density is measured with best probe sensitivity. The best probe sensitivity improves by ≈6 times at the optimal probe light power density compared with that in the conventional linear optical rotation detection. The proposed method can be applied to SERF magnetometers, co‐magnetometers, and atomic spin gyroscopes.
The ultra-sensitive atomic co-magnetometer based on the spin-exchange relaxation-free (SERF) regime is a valuable tool for inertial measurements and fundamental physics research. However, the optical magnetic misalignment effect is a significant source of error in SERF co-magnetometers, limiting their magnetic field suppression ability and long-term stability. This paper establishes a response model of angular velocity and magnetic field for the SERF co-magnetometer. The impact of optical magnetic misalignment on the scale factor, magnetic field amplitude-frequency response, and angular velocity errors caused by magnetic noise is systematically investigated. The results indicate that the scale factor and magnetic field suppression ability decrease as the optical magnetic misalignment angle increases, while the angular velocity errors caused by magnetic noise increase as the misalignment angle increases. Finally, experimental results demonstrate that the optical-magnetic misalignment effect significantly compromises the long-term stability of SERF co-magnetometers, underscoring its substantial influence on the overall performance. This work contributes to understanding the mechanism of optical magnetic misalignment effects on the SERF co-magnetometer and enhances its performance.
In the optical pumping systems based on the pump-probe arrangement, the spin polarization of the atoms is generally monitored utilizing the probe laser beam, in which way an extra perturbation must be introduced and thus affects the normal operation of the sensors. By investigating the absorption rate of the circularly polarized pump laser, here we demonstrate the feasibility of extracting the electron-spin polarization from the transmitted pump laser intensity. We experimentally validate the method in a spin-exchange relaxation free (SERF) magnetometer and the results are in excellent agreement with the theory. The scheme operates in a silent mode and features a real-time observation. We also study the corresponding magnetic field response of the SERF magnetometer and a term arising from the diffusion effects has been added to the original model to explain the discrepancy of the response.
This study proposes an in situ method for measuring the equilibrium spin polarization and its longitudinal spatial distribution in a spin-exchange relaxation-free (SERF) atomic magnetometer. The total relaxation rate was determined by analyzing the steady-state response of the magnetometer to the triaxial magnetic field. The transfer coefficient between spin polarization along the probe beam axis and the steady-state response was derived from the optical depth of the probe light and the incident/transmitted power through the vapor cell. By applying a DC magnetic field along the sensitive axis and combining the total relaxation rate with the transfer coefficient, the equilibrium spin polarization value under zero-field conditions was obtained. The equilibrium spin polarization distribution along the pump beam propagation direction was measured, showing consistent trends with simulation results, with a maximum relative error of less than 5%. The expanded uncertainty of the proposed equilibrium spin polarization measurement method ranges from 0.8% to 9.7%. The advantages of this method include no requirement for additional optical field or magnetic field modulation, immunity to temperature and temperature gradients, and the capability to directly determine the equilibrium spin polarization value.
In this article, we analyze the amplitude-frequency and phase-frequency responses of a spin-exchange relaxation-free (SERF) atomic magnetometer with the nonorthogonal angle between the pump and probe beam. The optical nonorthogonality leads to a change in the photon spin direction of circularly polarized pump light, which decides the polarization direction of the atomic ensemble, causing significant differences in dynamic responses to the magnetic field. We theoretically analyze relationships between dynamic response solutions of the Bloch equation with different pump lights and magnetic field directions based on which the equations are linearized. The equations are solved with the Fourier transform method, and three-axis dynamic responses are obtained under the influences of optical nonorthogonality and residual static magnetic field. In the experiment, we verify the linear superposition characteristics between different response components. According to the results, we propose a novel method to quickly calibrate the nonorthogonal angle, which could reduce the optical nonorthogonal angle by 20 times, reaching 0.54°, and effectively enhance the dynamic magnetic field response signal in atomic magnetometers.