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arXiv:2608.14343

Analytical Theory of Higher-Order Collective Spin Interactions in Cavity Quantum Electrodynamics

Leilani Ainsworth, Chase Gomes, Joseph Prescott, Kaley Wilcox, Jack Sullivan, Esteban Teran, Manav Bilakhia, Simone Colombo

quant-phphysics.atom-phSubmitted Aug 14, 2026• Announced Aug 17, 2026• 0 citations
v1 · Aug 14, 2026v2 · Aug 17, 2026
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Abstract

Cavity-mediated collective-spin interactions are commonly described by a quadratic one-axis twisting Hamiltonian. However, the underlying atom-light interaction naturally generates nonlinearities to arbitrary order. Here, we derive a closed-form analytical expression for the complete hierarchy of cavity-mediated collective-spin interactions. We show that the nonlinear coefficients $χ_k$ are governed by Chebyshev polynomials, with $k$ the order of nonlinearity. This yields a universal scaling $χ_k\proptoη^k$ with the single-atom cooperativity $η$ and a description of their dependence on cavity detuning. The result provides a systematic framework for determining when higher-order nonlinearities become relevant and when the quadratic approximation breaks down. We identify experimentally relevant regimes in which higher-order terms substantially modify collective-spin dynamics, accelerating the generation of quantum correlations and quantum Fisher information, and demonstrate that finite-order expansions can accurately reproduce the full cavity-mediated evolution. Our results establish a general framework for understanding higher-order nonlinearities in cavity quantum electrodynamics and their role in collective entanglement and quantum-enhanced sensing.

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Cavity-mediated collective-spin interactions are commonly described by a quadratic one-axis twisting Hamiltonian. However, the underlying atom-light interaction naturally generates nonlinearities to arbitrary order. Here, we derive a closed-form analytical expression for the complete hierarchy of cavity-mediated collective-spin interactions. We show that the nonlinear coefficients χkχ_kχk​ are governed by Chebyshev polynomials, with kkk the order of nonlinearity. This yields a universal scaling χk∝ηkχ_k\proptoη^kχk​∝ηk with the single-atom cooperativity ηηη and a description of their dependence on cavity detuning. The result provides a systematic framework for determining when higher-order nonlinearities become relevant and when the quadratic approximation breaks down. We identify experimentally relevant regimes in which higher-order terms substantially modify collective-spin dynamics, accelerating the generation of quantum correlations and quantum Fisher information, and demonstrate that finite-order expansions can accurately reproduce the full cavity-mediated evolution. Our results establish a general framework for understanding higher-order nonlinearities in cavity quantum electrodynamics and their role in collective entanglement and quantum-enhanced sensing.
In an ensemble of two-level atoms that can be described in terms of a collective spin, entangled states can be used to enhance the sensitivity of interferometric precision measurements. While non-Gaussian spin states can produce larger quantum enhancements than spin-squeezed Gaussian states, their use requires the measurement of observables that are nonlinear functions of the three components of the collective spin. In this paper we develop strategies that achieve the optimal quantum enhancements using non-Gaussian states produced by a nonlinear one-axis-twisting Hamiltonian, and show that measurement-after-interaction techniques, known to amplify the output signals in quantum parameter estimation protocols, are effective in measuring nonlinear spin observables. Including the presence of the relevant decoherence processes from atomic experiments, we determine analytically the quantum enhancement of non-Gaussian over-squeezed states as a function of the noise parameters for arbitrary atom numbers.
In an ensemble of two-level atoms that can be described in terms of a collective spin, entangled states can be used to enhance the sensitivity of interferometric precision measurements. While non-Gaussian spin states can produce larger quantum enhancements than spin-squeezed Gaussian states, their use requires the measurement of observables that are nonlinear functions of the three components of the collective spin. In this paper we develop strategies that achieve the optimal quantum enhancements using non-Gaussian states produced by a nonlinear one-axis-twisting Hamiltonian, and show that measurement-after-interaction techniques, known to amplify the output signals in quantum parameter estimation protocols, are effective in measuring nonlinear spin observables. Including the presence of the relevant decoherence processes from atomic experiments, we determine analytically the quantum enhancement of non-Gaussian over-squeezed states as a function of the noise parameters for arbitrary atom numbers.
The interaction between an atomic ensemble and a light mode in a high-finesse optical cavity can easily reach the strong-coupling regime, where quantum effects dominate.In this regime, the interaction can be used to generate both atom-light and atom-atom entanglement.We analyze the dominant effects on the collective atomic state and the light field, and derive a unified approach that can account for atomic entanglement induced both by measurements on the light field, and by ignoring the state of the light field altogether.We present analytical expressions for the entanglement induced by the interaction, and determine the conditions that maximize the entanglement-induced gain over the standard quantum limit in quantum sensors and atomic clocks.
Cavity quantum electrodynamics with atomic ensembles is typically associated with collective spin phenomena, such as superradiance and spin squeezing, in which the atoms evolve collectively as a macroscopic spin (S∼N/2S\sim N/2S∼N/2) on the Bloch sphere. Surprisingly, we show that the tendency toward a collective spin description need not imply collective spin phenomena; rather, it can be exploited to generate new forms of strongly correlated quantum matter. The key idea is to use uniform cavity-mediated interactions to energetically project the system into the total-spin singlet sector (S=0S=0S=0) - a highly entangled subspace where the physics is governed entirely by cavity fluctuations. Focusing on Rydberg atom arrays coupled to a single-mode cavity, we show that global cavity fluctuations can effectively squeeze classical antiferromagnets into quantum spin liquids, characterized by non-local entanglement, fractionalized excitations, and emergent gauge fields. This work suggests that cavity QED can be a surprising resource for inducing strongly correlated phenomena, which could be explored in the new generation of hybrid tweezer-cavity platforms.
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The idea of making photons effectively interact has attracted a lot of interest in recent years, for several reasons. Firstly, since photons do not naturally interact with each other, it is of fundamental physical interest to see what kind of medium can mediate interactions between these fundamental and non-interacting particles, and to what extent. Secondly, photonics is a major candidate for future quantum technology, due to the easy manipulation, readout, and transport of photons, which makes them ideal for quantum information processing. Finally, achieving strong and tunable interactions among photons would open up an avenue for exploring the many-body physics of a fluid of light. In this thesis, we will see how a cavity formed of subwavelength lattices of two-level atoms can confine photons to a nonlinear environment for a long time, such that emitted photons have accumulated strong correlations both among their momenta and in their temporal statistics. This speaks of a strong photon-photon interaction within the cavity. The nonlinearity originates in the saturability of individual atoms, and the lattice structure results in a strong and low-loss collective interaction with light. While a single atomic lattice has a largely linear nature, as the effect of individual atoms washes out in the collective response, the confining geometry of the cavity means the photons are exposed to the underlying saturability of the atoms for such a long time that the nonlinearity is revived. We will analyse this system both using a standard input-output formalism, where the nonlinear physics of the system is handled numerically, and a powerful Green's function-based approach that allows for exact analytical results with no additional approximations. This analytical description has the potential to lead to an exact study of the many-body physics of interacting photons in a two-dimensional setting.