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arXiv:2106.13234 · PRX Quantum

Collective Spin-Light and Light-Mediated Spin-Spin Interactions in an Optical Cavity

Zeyang Li, Boris Braverman, Simone Colombo, Chi Shu, Akio Kawasaki, Albert F. Adiyatullin, Edwin Pedrozo-Peñafiel, Enrique Mendez, Vladan Vuletić

Published Apr 12, 2022• 49 citations
arXivHTMLPDF

Abstract

The interaction between an atomic ensemble and a light mode in a high-finesse optical cavity can easily reach the strong-coupling regime, where quantum effects dominate.In this regime, the interaction can be used to generate both atom-light and atom-atom entanglement.We analyze the dominant effects on the collective atomic state and the light field, and derive a unified approach that can account for atomic entanglement induced both by measurements on the light field, and by ignoring the state of the light field altogether.We present analytical expressions for the entanglement induced by the interaction, and determine the conditions that maximize the entanglement-induced gain over the standard quantum limit in quantum sensors and atomic clocks.

DOI
10.1103/prxquantum.3.020308

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The interaction between an atomic ensemble and a light mode in a high-finesse optical cavity can easily reach the strong-coupling regime, where quantum effects dominate.In this regime, the interaction can be used to generate both atom-light and atom-atom entanglement.We analyze the dominant effects on the collective atomic state and the light field, and derive a unified approach that can account for atomic entanglement induced both by measurements on the light field, and by ignoring the state of the light field altogether.We present analytical expressions for the entanglement induced by the interaction, and determine the conditions that maximize the entanglement-induced gain over the standard quantum limit in quantum sensors and atomic clocks.
Macroscopic arrays of cold atoms trapped in optical cavities can reach the strong atom-light collective coupling regime thanks to the simultaneous interactions of the cavity mode with the atomic ensemble. In a recent work [R. J. Lewis-Swan, D. Barberena, J. A. Muniz, J. R. K. Cline, D. Young, J. K. Thompson, and A. M. Rey, Phys. Rev. Lett. 124, 193602 (2020)] we reported a protocol that takes advantage of the strong and collective atom-light interactions in cavity QED systems for precise electric-field sensing in the optical domain. We showed that it can provide between 10 and 20 dB of metrological gain over the standard quantum limit in current cavity QED experiments operating with long-lived alkaline-earth atoms. Here, we give a more in depth discussion of the protocol using both exact analytical calculations and numerical simulations, and describe the precise conditions under which the predicted enhancement holds after thoroughly accounting for both photon loss and spontaneous emission, natural decoherence mechanisms in current experiments. The analysis presented here not only serves to benchmark the protocol and its utility in cavity QED arrays but also sets the conditions required for its applicability in other experimental platforms such as arrays of trapped ions.
We consider the optical generation and characterization of entanglement in atomic ensembles under nonuniform interaction between the ensemble and an optical mode. We show that for a wide range of parameters a system of nonuniformly coupled atomic spins can be described as an ensemble of uniformly coupled spins with a reduced effective atom-light coupling and a reduced effective atom number, with a reduction factor of order unity given by the ensemble-mode geometry. This description is valid even for complex entangled states with arbitrary phase-space distribution functions as long as the average total spin remains large, and the detection does not resolve single spins. Furthermore, we derive an analytic formula for determining the observable entanglement in the case, of relevance in practice, where the ensemble-mode coupling differs between state generation and measurement.
The quantum nature of light makes it a basic component for models of quantum measurement and information exchange between disparate quantum modes, pioneered in the field of cavity quantum electrodynamics. The interaction of atomic ensembles with the mode of an optical cavity provides a flexible platform for exploring the coherent interaction of light with diverse macroscopic dynamics, such as collective motion and spin. This dissertation presents experimental results and theoretical models for continuous measurement and control of the center of mass motion and collective spin precession of an atomic ensemble, mediated by coupling to a high-finesse optical cavity. First, the theory of dispersive coupling between the cavity mode and the collective motion and spin of an atomic ensemble is derived, and then a general time-domain formalism is developed for theoretical analysis of multi-mode optodynamical systems. Single-mode optodynamical effects are introduced through experimental demonstrations of measurement and control of the collective atomic spin, providing a close analogy to cavity optomechanics.Next, multiple collective atomic modes are considered within a single cavity, in order to assemble optically mediated interactions within multi-mode optodynamical systems. A demonstration of optodynamical interactions between the center of mass motion of two atomic ensembles is presented, coupled through an optical spring mediated by the cavity mode. Then simultaneous coupling of the center of mass motion and total spin precession of a single ensemble of atoms is described, yielding an experimental realization of a negative-mass instability, facilitated by the novel resource of the spin ensembles inverted state. A theoretical analysis of the negative-mass instability is presented, which indicates the possibility of generating two-mode squeezed states in the absence of excess incoherent noise. Finally, linear state retrodiction from the optodynamical signals is discussed, providing background and supplemental material for a forthcoming manuscript.
In the context of quantum metrology, optical cavity-QED platforms have primarily been focused on the generation of entangled atomic spin states useful for next-generation frequency and time standards. Here, we report a complementary application: the use of optical cavities to generate nonclassical states of light for electric field sensing below the standard quantum limit. We show that cooperative atom-light interactions in the strong collective coupling regime can be used to engineer generalized atom-light cat states which enable quantum enhanced sensing of small displacements of the cavity field even in the presence of photon loss. We demonstrate that metrological gains of 10-20 dB below the standard quantum limit are within reach for current cavity-QED systems operating with long-lived alkaline-earth atoms.
Abstract An ensemble of atoms can operate as a quantum sensor by placing atoms in a superposition of two different states. Upon measurement of the sensor, each atom is individually projected into one of the two states. Creating quantum correlations between the atoms, that is entangling them, could lead to resolutions surpassing the standard quantum limit 1–3 set by projections of individual atoms. Large amounts of entanglement 4–6 involving the internal degrees of freedom of laser-cooled atomic ensembles 4–16 have been generated in collective cavity quantum-electrodynamics systems, in which many atoms simultaneously interact with a single optical cavity mode. Here we report a matter-wave interferometer in a cavity quantum-electrodynamics system of 700 atoms that are entangled in their external degrees of freedom. In our system, each individual atom falls freely under gravity and simultaneously traverses two paths through space while entangled with the other atoms. We demonstrate both quantum non-demolition measurements and cavity-mediated spin interactions for generating squeezed momentum states with directly observed sensitivity 3 . 4−0.9+1.13\,.\,{4}_{-0.9}^{+1.1}3.4−0.9+1.1​ 3 . 4 − 0.9 + 1.1 dB and 2 . 5−0.6+0.62\,.\,{5}_{-0.6}^{+0.6}2.5−0.6+0.6​ 2 . 5 − 0.6 + 0.6 dB below the standard quantum limit, respectively. We successfully inject an entangled state into a Mach–Zehnder light-pulse interferometer with directly observed sensitivity 1 . 7−0.5+0.51\,.\,{7}_{-0.5}^{+0.5}1.7−0.5+0.5​ 1 . 7 − 0.5 + 0.5 dB below the standard quantum limit. The combination of particle delocalization and entanglement in our approach may influence developments of enhanced inertial sensors 17,18 , searches for new physics, particles and fields 19–23 , future advanced gravitational wave detectors 24,25 and accessing beyond mean-field quantum many-body physics 26–30 .
We propose a simple and efficient method for generating metrologically useful quantum entanglement in an ensemble of spin-1 atoms that interacts with a high-finesse optical cavity mode. It requires straightforward preparation of N atoms in the m_{F}=0 sublevel, tailoring of the atom-field interaction to give an effective Tavis-Cummings model for the collective spin-1 ensemble, and a photon counting measurement on the cavity output field. The photon number provides a projective measurement of the collective spin length S, which, for the chosen initial state, is heavily weighted around values S≃sqrt[N], for which the corresponding spin states are strongly entangled and exhibit Heisenberg scaling of the metrological sensitivity with N, as quantified by the quantum Fisher information.