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arXiv:2608.09234

Stroboscopic Raman Spectroscopy of Atom Optics in Quasi-Bragg Regime

Joel Gomes Baptista, Louis Pagot, Sébastien Merlet, Leonid A. Sidorenkov, Franck Pereira dos Santos

Published Aug 10, 2026• 0 citations
arXivHTMLPDF

Abstract

Quasi-Bragg regime is a good compromise for large-momentum-transfer atom interferometry, allowing for scaling up the interferometric area, while constraining the population of unwanted states. Separation of momentum states via standard time of flight methods, however, can be challenging when using laser-cooled atoms, rather than ultracold atoms with sub-recoil velocity distribution. To overcome this limit, we use Raman spectroscopy for stroboscopic sampling of the atomic state evolution in momentum space during the interrogating laser pulses. We quantitatively characterize atom optics employing two-photon (2___k) and multi-photon (6___k) Bragg transitions, the latter being optionally enhanced with optimal control protocol. We closely match the observed dynamics of the atomic state with simulations. Finally, we perform momentum spectroscopy of the output states in a 6___k Bragg gravimeter.

DOI
10.48550/arxiv.2608.09234

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Quasi-Bragg regime is a good compromise for large-momentum-transfer atom interferometry, allowing for scaling up the interferometric area, while constraining the population of unwanted states. Separation of momentum states via standard time of flight methods, however, can be challenging when using laser-cooled atoms, rather than ultracold atoms with sub-recoil velocity distribution. To overcome this limit, we use Raman spectroscopy for stroboscopic sampling of the atomic state evolution in momentum space during the interrogating laser pulses. We quantitatively characterize atom optics employing two-photon (2___k) and multi-photon (6___k) Bragg transitions, the latter being optionally enhanced with optimal control protocol. We closely match the observed dynamics of the atomic state with simulations. Finally, we perform momentum spectroscopy of the output states in a 6___k Bragg gravimeter.
We demonstrate light-pulse atom interferometry with large-momentum-transfer atom optics based on stimulated Raman transitions and frequency-swept adiabatic rapid passage. Our atom optics have produced momentum splittings of up to 30 photon recoil momenta in an acceleration-sensitive interferometer for laser cooled atoms. We experimentally verify the enhancement of phase shift per unit acceleration and characterize interferometer contrast loss. By forgoing evaporative cooling and velocity selection, this method lowers the atom shot-noise-limited measurement uncertainty and enables large-area atom interferometry at higher data rates.
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Spin squeezing in atomic ensembles enables atom interferometry with sensitivities below the shot-noise limit, but the associated entanglement is highly susceptible to loss, making imperfections in atom optics a central limitation. Bragg diffraction is an established technique for driving transitions between atomic momentum states and enables large-momentum transfer through higher-order diffraction while preserving the internal state. However, it is intrinsically limited by two competing mechanisms: Short light pulses induce parasitic diffraction into off-resonant orders beyond an effective two-level description, while long pulses face velocity selectivity. We derive analytical expressions in a second-quantized framework for the atom optics and phase uncertainty of a Mach-Zehnder interferometer including these effects. We demonstrate that sub-shot-noise scaling is achieved only in a regime of intermediate pulse duration. Furthermore, we show that deleterious effects of higher-order diffraction are partially mitigated by optimizing the input quantum state.
We report here on the realization of light-pulse atom interferometers with large-momentum-transfer atom optics based on a sequence of Bragg transitions. We demonstrate momentum splitting up to 200 photon recoils in an ultracold atom interferometer. We highlight a new mechanism of destructive interference of the losses leading to a sizable efficiency enhancement of the beam splitters. We perform a comprehensive study of parasitic interferometers due to the inherent multiport feature of the quasi-Bragg pulses. Finally, we experimentally verify the phase shift enhancement and characterize the interferometer visibility loss.
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