We present designs for the augmentation ``mirror'' pulses of large-momentum-transfer atom interferometers that maintain their fidelity as the wave-packet momentum difference is increased. These biselective pulses, tailored using optimal control methods to the evolving bimodal momentum distribution, should allow greater interferometer areas and hence increased inertial measurement sensitivity, without requiring elevated Rabi frequencies or extended frequency chirps. Using an experimentally validated model, we have simulated the application of our pulse designs to large-momentum-transfer atom interferometry using stimulated Raman transitions in a laser-cooled atomic sample of
85Rb at 1 $\ensuremath{\mu}\mathrm{K}$. After the wave packets have separated by 42 photon recoil momenta, our pulses maintain a fringe contrast of 90%, whereas, for adiabatic rapid passage and conventional $\ensuremath{\pi}$ pulses, the contrast is less than 10%. Furthermore, we show how these pulses may be adapted to be robust to laser intensity variations between pulses and to suppress the detrimental off-resonant excitation that limits other broadband pulse schemes.
Large-momentum-transfer (LMT) atom interferometry provides a route toward enhanced inertial sensitivity in compact quantum sensors, but its scalability is limited by the accumulation of pulse-transfer errors across long Raman pulse sequences. We investigate theoretically the use of stimulated Raman shortcut-to-adiabatic passage (STIRSAP) for high-fidelity LMT atom optics in a Mach--Zehnder interferometer geometry. The counterdiabatic correction is encoded directly into the Raman pulse envelopes, eliminating the need for auxiliary microwave or radio-frequency control fields. Numerical simulations based on an effective Raman model show that
1 μs STIRSAP pulses achieve single-pulse transfer fidelities of
Fπ=0.99902 while maintaining negligible pulse-time overhead even at high momentum order. We analyze the resulting tradeoff between interferometric phase enhancement and compound contrast decay and identify an unconstrained shot-noise optimum near
n≈270. The analysis further shows that practical operation at extreme LMT order is constrained by wave-packet separation, vibration noise, Doppler detuning, and accumulated systematic effects rather than by pulse duration itself. These results establish superadiabatic Raman control as a promising approach for scalable high-fidelity atom optics and clarify the physical limitations governing compact high-order atom interferometers.
We report here on the realization of light-pulse atom interferometers with large-momentum-transfer atom optics based on a sequence of Bragg transitions. We demonstrate momentum splitting up to 200 photon recoils in an ultracold atom interferometer. We highlight a new mechanism of destructive interference of the losses leading to a sizable efficiency enhancement of the beam splitters. We perform a comprehensive study of parasitic interferometers due to the inherent multiport feature of the quasi-Bragg pulses. Finally, we experimentally verify the phase shift enhancement and characterize the interferometer visibility loss.
We report a demonstration of composite Raman pulses that achieve broadband population inversion and are used to increase the momentum splitting of an atom interferometer up to 18ℏk (corresponding to an increase in the inertial signal by a factor of nine). Composite Raman pulses suppress the effects of pulse length and detuning errors, providing higher transfer efficiency and velocity acceptance than single square pulses. We implement two composite pulse sequences, π/20°−π90°−π/20° and π/20°−π180°−3π/20°, and use the latter composite pulse to demonstrate large-area atom interferometry with stimulated Raman transitions. In addition to enabling larger momentum transfer and higher sensitivity, we argue that composite pulses can improve the robustness of atom interferometers operating in dynamic environments.
Ushered forth by advances in time and frequency metrology, atom interferometry remains an indispensable measurement tool in atomic physics due to its precision and versatility. A sequence of four
pi/2 beam splitter pulses can create either an interferometer sensitive to the atom's recoil frequency when the momentum imparted by the light reverses direction between pulse pairs or, when constructed from pulses without such reversal, sensitive to the perturbing potential from an external optical field. Here, we demonstrate the first atom interferometer with laser-cooled lithium, advantageous for its low mass and simple atomic structure. We study both a recoil-sensitive Ramsey-Bord\\'e interferometer and interferometry sensitive to the dynamic polarizability of the ground state of lithium. Recoil-sensitive Ramsey-Bord\\'e interferometry benefits from lithium's high recoil frequency, a consequence of its low mass. At an interrogation time of 10 ms, a Ramsey-Bord\\'e lithium interferometer could achieve sensitivities comparable to those realized at much longer times with heavier alkali atoms. However, in contrast with other atoms that are used for atom interferometry, lithium's unresolved excited-state hyperfine structure precludes the the cycling transition necessary for efficient cooling. Without sub-Doppler cooling techniques. As as result, a lithium atomic gas is typically laser cooled to temperatures around 300
muK, above the Doppler limit, and well above the recoil temperature of 6
muK. This higher temperature gas expands rapidly during the operation of an atom interferometer, limiting the experimental interrogation time and preventing spatially resolved detection. In this work, a light-pulse lithium matter-wave interferometer is demonstrated in spite of these limitation. Two-photon Raman interferometer pulses coherently couple the atom's spin and momentum and are thus able to spectrally resolve the outputs. These fast pulses drive conjugate interferometers simultaneously which beat with a fast frequency component proportional to the atomic recoil frequency and an envelope modulated by the two-photon detuning of the Raman transition. We detect the summed signal at short experimental times, preventing perturbation of the signal from vibration noise. This demonstration of a sub-recoil measurement with a super-recoil sample opens the door to similar scheme with other particles that are difficult to trap and cool well, like electrons. An interferometer instead composed of
pi/2-pulses with a single direction of momentum transfer, can be sensitive to the dynamic polarizability of the atomic ground state. By scanning the frequency of an external driving field, such a measurement can be used to determine the atom's tune-out wavelength. This is the wavelength at which the frequency-dependent polarizability vanishes due to compensating ac-Stark shifts from other atomic states. Lithium's simple atomic structure allows for a precise computation of properties with only {\\em ab initio} wave functions and spectroscopic data. A direct interferometric measurement of lithium's red tune-out wavelength at 670.971626(1) nm, is a precise comparison to existing `all-order' atomic theory computations. It also provides another way to experimentally determine the
S− to
P− transitions matrix elements, for which large correlations and small values complicate computations. Finally, a future measurement of lithium's ultraviolet tune-out wavelength of at 324.192(2) nm would be sensitive to relativistic approximations in the atomic structure description.Atom interferometry simultaneously verifies existing atomic theory with measurements of atomic properties and searches for exotic physics lurking in plain sight. The techniques developed here broaden the applicability of interferometry and increase measurement sensitivity by simplifying cooling, increasing atom number and reducing the cycle time. Overcoming the current experimental limitations on interrogation time would allow for ultra-precise measurements of both the tune-out wavelength and the fine structure constant.
The use of cold atoms in any sensor operating in a dynamic environment requires that the measurement cycle be conducted before the atom cloud escapes the interaction region. Under multiple-g accelerations it is desirable to complete measurements in millisecond time scales, particularly when laser beams are used to interrogate the atoms. In this paper, we demonstrate high-contrast atom interferometry in a vapor cell using stimulated Raman transitions at millisecond interrogation times. Laser-cooled cesium atoms are interrogated with a sequence of three Raman pulses and the interferometer phase is read out in the same region in which the atoms are trapped. Our system achieved over 70% contrast with a Doppler insensitive interferometer and over 30% contrast with a Doppler sensitive interferometer, in an environment normally considered adverse to high-contrast atom interferometry (e.g., no retroreflector stabilization and no magnetic shielding). Demonstration of an inertially sensitive atom interferometer in this environment supports the feasibility of a high-bandwidth inertial sensor using light pulse atom interferometry. Finally, we show that Raman pulse population transfer efficiency in our system is primarily limited by nonuniformity of the Raman laser intensity across the atom cloud.