We have developed a low temperature (LT), ultra-high-vacuum (UHV) system that combines two complementary techniques, scanning probe microscopy (SPM) and electrical transport measurements, within a single platform. By providing simultaneous access to the atomic-scale surface landscape and the macroscopic device response of the same sample, the setup enables direct correlations between local structural/spectroscopic signatures and global electronic transport behavior in two-dimensional (2D) devices. The system allows experiments where atomic-scale modifications or controlled manipulations are performed while continuously monitoring their impact on device-scale performance. The setup consists of two interconnected UHV chambers: a dedicated preparation chamber and a separate measurement chamber that houses a liquid-helium cryostat and the SPM/transport stage. Base pressure is 1x10^-11 Torr. A key feature is direct optical access to the sample, enabling rapid and reliable tip positioning with an accuracy of 5 microns x 5 microns within 10 minutes. The SPM, operated using custom-built electronics, can track the exact same sample region across a temperature range from 2.9 K to 400 K, with mechanical stability below 1 pm. System performance is demonstrated on graphene devices, and bulk Pb is used to determine energy resolution. Using superconducting tips, scanning tunneling spectroscopy measures the superconducting gap with an energy resolution of 30 microV. Transport measurements track the temperature dependence of both resistivity and critical current across the superconducting transition of an in-situ prepared Pb nanowire.
We have developed a low temperature (LT), ultra-high-vacuum (UHV) system that combines two complementary techniques, scanning probe microscopy (SPM) and electrical transport measurements, within a single platform. By providing simultaneous access to the atomic-scale surface landscape and the macroscopic device response of the same sample, the setup enables direct correlations between local structural/spectroscopic signatures and global electronic transport behavior in two-dimensional (2D) devices. The system allows experiments where atomic-scale modifications or controlled manipulations are performed while continuously monitoring their impact on device-scale performance. The setup consists of two interconnected UHV chambers: a dedicated preparation chamber and a separate measurement chamber that houses a liquid-helium cryostat and the SPM/transport stage. Base pressure is 1x10^-11 Torr. A key feature is direct optical access to the sample, enabling rapid and reliable tip positioning with an accuracy of 5 microns x 5 microns within 10 minutes. The SPM, operated using custom-built electronics, can track the exact same sample region across a temperature range from 2.9 K to 400 K, with mechanical stability below 1 pm. System performance is demonstrated on graphene devices, and bulk Pb is used to determine energy resolution. Using superconducting tips, scanning tunneling spectroscopy measures the superconducting gap with an energy resolution of 30 microV. Transport measurements track the temperature dependence of both resistivity and critical current across the superconducting transition of an in-situ prepared Pb nanowire.
Quantum electron microscopy is an emerging research field at the intersection of electron microscopy, quantum optics, and nanophotonics. Free electrons can serve as powerful quantum probes, on par with photons in their ability to carry and transfer quantum information, generate entanglement within and with a specimen, and reveal previously inaccessible details on nanoscale quantum phenomena [1]. However, quantum experiments are generally highly sensitive to decoherence arising from interactions with residual gas particles, making ultra-high vacuum (UHV) conditions sometimes essential. UHV environments are also required in transmission electron microscopes (TEMs) for the investigation of contamination-sensitive materials [2, 3]. In our project, we aim to combine a trapped-ion quantum computer with a TEM to realise Quantum-Computer-Enhanced Electron Microscopy (QCEM) (www.qcem.info). In this scheme, coherent interactions between free electrons and a trapped ion require vacuum conditions beyond the standard TEM operation [4]. Although UHV-TEM systems have previously been realised [2,3, 5-7], achieving base pressures in the 10⁻⁹ mbar range or better typically involves significant financial investment, long implementation times, and close collaboration with manufacturers. We present a cost-effective, minimally invasive modification to the vacuum system of a JEOL JEM-2100F to reduce the base pressure at the sample position to below 5 × 10⁻⁹ mbar. Our approach is to integrate two additional 50 L/s NEG-ion pumps mounted on flanges near the sample region, with no structural modifications to the microscope. The NEG pumps are integrated into the microscope workflow through controlled activation and regeneration cycles compatible with standard TEM operation. This work represents a practical step toward enabling the realisation of QCEM, and the concept enables a relatively rapid implementation at a moderate cost, which can, in principle, be adapted to any TEM that provides suitable flange access to the sample chamber.
We present a custom-designed ultrahigh vacuum (UHV) cluster tool developed for studying shallow nitrogen-vacancy (NV) centers in diamond, enabling in situ diamond surface preparation, characterization, and single NV center dynamics measurements within a single connected platform. The system combines a surface science chamber for controlled surface modification and analysis with a cryogenic confocal microscope chamber dedicated to NV spin and optical measurements. This integrated approach enables a direct correlation between diamond surface chemistry and the resulting NV spin and charge properties. The instrument provides a versatile platform for systematic studies of surface-induced decoherence mechanisms and charge dynamics for shallow NV centers, and establishes a pathway toward reproducible surface engineering for quantum sensing applications.
The investigation of novel electronic phases in low-dimensional quantum materials demands for the concurrent development of measurement techniques that combine surface sensitivity with high spatial resolution and high measurement accuracy. We propose a new quantum sensing imaging modality based on superconducting charge qubits to study dissipative charge carrier dynamics with nanometer spatial and high temporal resolution. Using analytical and numerical calculations we show that superconducting charge qubit microscopy (SCQM) has the potential to resolve temperature and resistivity changes in a sample as small as ΔT≤0.1mK and Δρ≤1⋅104Ω⋅cm, respectively. Among other applications, SCQM will be especially suited to study the microscopic mechanisms underlying resistive phase transition, such as the superconductor-insulator-transition in twisted bilayer graphene, to investigate novel topological boundary modes found in higher order topological insulators and to optimize the transport properties of nano- and mesoscopic devices.
A novel cryogenic scanning laser microscope with a spatial resolution of less than 5 μm has been designed for on-chip in situ investigations of the working properties of normal and superconducting circuits and devices. The instrument relies on the detection of the electrical response of the circuit to a very localized heating induced by irradiation with 675 nm wavelength light from a semiconductor laser. The hot spot is moved by a specially designed piezoelectric scanner sweeping the tip of a single-mode optical fiber a few μm above the circuit. Depending on the scanner design the scanning area can be as large as 50×500 μm2 at 4.2 K. The microscope can be operated in the temperature range 2–300 K using a standard temperature controller. The central microscope body is mounted inside the vacuum can of a dip-stick-type cryoprobe. A damped spring system is used to reduce interference from extraneous mechanical vibrations. The microscope is integrated in a personal-computer-based data acquisition and control setup.
Mechanically ultrastable environments within maintenance-free dry cryostats are needed for high-precision surface probe microscopy experiments, as well as next-generation quantum technologies. The most demanding applications require picometre-scale precision combined with multi-axis and millimetre-scale scanning range, while offering access to optical, microwave, and radiofrequency control and a vector magnetic field. We demonstrate a versatile platform for such systems based on passive and active vibration control for a commercial dry cryostat. Using a tunable optical microcavity as a sensor, we report vibration levels of 4.2 pm root mean square at 2.3 K over one hour without postselection. We further demonstrate drift-free long-term operation with stability below 8.6 pm RMS over 12 hours. Our system enables continuous and automated operation for next-generation high-throughput applications without the need for liquid helium infrastructure. Requiring only standard machining facilities and commercially available hardware, the design can be readily adapted for cryogenic optical, electrical and magnetic high-precision measurements across quantum science, surface science, and nanotechnology.
Ultracold atomic gases can be utilised as extremely sensitive probes of their surrounding environment. In particular, samples of ultracold atoms confined using chip-based microtraps are an ideal tool for mapping electric and magnetic field landscapes. Over the course of this thesis, a new experiment capable of performing surface microscopy using magnetically trapped clouds of cold rubidium-87 atoms has been built. The focus of the work is on the design and construction of the experimental system, which must incorporate many different aspects for manipulating thermal atomic gases, with a view to positioning them at sub-micron distances from special surfaces. This reduced atom-surface separation is necessary for implementing a high resolution, high sensitivity magnetic field sensor with cold atoms. Although current microfabrication techniques easily enable trapping at distances on the order of micrometres, several distance-dependent surface effects - such as the Casimir-Polder force, Johnson-Nyquist noise, and stray potentials - eventually impede magnetic trapping at the sub-micron level. These surface effects can greatly modify the confining potentials, which reduces the trap depth and consequently leads to an additional loss rate of atoms from the trap. We have explored the possibility of using special surfaces such as nano-membranes of silicon nitride and graphene, which have reduced atom- surface interactions, to enable trapping distances at the sub-micron level. A multilayer printed circuit board chip has been designed to form an initial magnetic trap and then transport the cloud of atoms to a desired location over the samples. This chip, along with various samples, is mounted on a custom-made electrical feedthrough designed to make connections to all conductor that are inside the vacuum chamber. The initial cloud of cold atoms can then be prepared in the central region of the chip and delivered to the location of the samples on either side. The experimental system is able to routinely capture over 10^8 rubidium-87 atoms at a temperature of 80 micro-Kelvin in a magneto-optical trap using a novel scheme of five laser beams. A method is demonstrated for enhancing the atom number in the magneto-optical traps by a factor of two by using laser beams with two slightly different frequencies. Atoms from the magneto-optical trap are then transferred to a purely magnetic trap formed by the wires on the printed circuit board chip. Time-dependent currents in the chip wires then create a dynamic potential, which is shown to successfully transport the atomic sample over a distance of 12 millimetre with minimal atom loss. This thesis describes the development of the apparatus in detail, along with careful characterisation of the cold cloud at various stages of the experimental sequence. Initial results on the long distance atom transport are presented. Finally, the experimental results of the two frequency magneto-optical trap for atom number improvement are discussed.