Photonic integrated circuits (PICs) generate, route, and process light with high efficiency, scalability, and functional density on a single chip. Yet the tightly confined on-chip modes can not easily access or effectively interact with atomic vapors, fluids, gain media, and biological samples. Existing approaches require bringing the medium onto the chip or into a weak, tightly confined evanescent field, which restricts the interaction volume and the range of accessible media. Here, we demonstrate a re-entrant chip-free-space interface in which a thin-film lithium niobate circuit frequency-doubles telecom light, emits the 780~nm field through a Rubidium vapor cell, and recollects the reflected probe on the same chip. This emit-interact-recollect loop resolves the saturated absorption spectrum and stabilizes the telecom laser to within $\pm 280$~kHz over 2 hours. Our study paves an route to embed external media into PICs through the re-entrant photonic interface.
Photonic integrated circuits (PICs) generate, route, and process light with high efficiency, scalability, and functional density on a single chip. Yet the tightly confined on-chip modes can not easily access or effectively interact with atomic vapors, fluids, gain media, and biological samples. Existing approaches require bringing the medium onto the chip or into a weak, tightly confined evanescent field, which restricts the interaction volume and the range of accessible media. Here, we demonstrate a re-entrant chip-free-space interface in which a thin-film lithium niobate circuit frequency-doubles telecom light, emits the 780~nm field through a Rubidium vapor cell, and recollects the reflected probe on the same chip. This emit-interact-recollect loop resolves the saturated absorption spectrum and stabilizes the telecom laser to within ±280~kHz over 2 hours. Our study paves an route to embed external media into PICs through the re-entrant photonic interface.
Devices based on spectroscopy of atomic vapors can measure physical quantities such as magnetic fields, RF electric fields, time and length, and rotation and have applications in a broad range of fields including communications, medicine, and navigation. We present a type of photonic device that interfaces single-mode silicon nitride optical waveguides with warm atomic vapors, enabling precision spectroscopy in an extremely compact (<1 cm3) package. We perform precision spectroscopy of rubidium confined in a micro-machined, 27 mm3 volume, vapor cell using a collimated free-space 120 μm diameter laser beam derived directly from a single-mode silicon nitride waveguide. With this optical-fiber integrated photonic spectrometer, we demonstrate an optical frequency reference at 780 nm with a stability of 10−11 from 1 to 104 s. This device harnesses the benefits of both photonic integration and precision spectroscopy for the next generation of quantum sensors and devices based on atomic vapors.
We study an integrated silicon photonic chip, composed of several sub-wavelength ridge waveguides, and immersed in a micro-cell with rubidium vapor. Employing two-photon excitation, including a telecom wavelength, we observe that the waveguide transmission spectrum gets modified when the photonic mode is coupled to rubidium atoms through its evanescent tail. Due to the enhanced electric field in the waveguide cladding, the atomic transition can be saturated at a photon number ≈80 times less than a free-propagating beam case. The non-linearity of the atom-clad Si-waveguide is about 4 orders of magnitude larger than the maximum achievable value in doped Si photonics. The measured spectra corroborate well with a generalized effective susceptibility model that includes the Casimir-Polder potentials, due to the dielectric surface, and the transient interaction between flying atoms and the evanescent waveguide mode. This work paves the way towards a miniaturized, low-power, and integrated hybrid atomic-photonic system compatible with CMOS technologies.
The integration of quantum emitters with integrated photonics enables complex quantum photonic circuits that are necessary for photonic implementation of quantum simulators, computers, and networks. Thin-film lithium niobate is an ideal material substrate for quantum photonics because it can tightly confine light in small waveguides and has a strong electro-optic effect that can switch and modulate single photons at low power and high speed. However, lithium niobate lacks efficient single-photon emitters, which are essential for scalable quantum photonic circuits. We demonstrate deterministic coupling of single-photon emitters with a lithium niobate photonic chip. The emitters are composed of InAs quantum dots embedded in an InP nanobeam, which we transfer to a lithium niobate waveguide with nanoscale accuracy using a pick-and-place approach. An adiabatic taper transfers single photons emitted into the nanobeam to the lithium niobate waveguide with high efficiency. We verify the single photon nature of the emission using photon correlation measurements performed with an on-chip beamsplitter. Our results demonstrate an important step toward fast, reconfigurable quantum photonic circuits for quantum information processing.
Integrating alkali atomic vapors with nanophotonic devices offers a scalable route to quantum technologies that leverage strong atom–photon interactions. While there have been many approaches to such integration, the general reliance on traditional glass vapor cells, distilled alkali metals, and epoxy sealing limits reproducibility and scalability. Moreover, mitigating adverse Rb-photonics interactions is essential, particularly as devices become more compact and the alkali source lies in close proximity to the photonic elements. Here, we demonstrate the successful operation of compact and fully integrated devices that combine silicon nitride photonic integrated circuits (PICs) with microfabricated borosilicate vapor cells and pill-type rubidium (Rb) dispensers through hermetic seals via anodic bonding. We show how successful operation hinges on optically activating the dispenser in a low-power pulsed mode, releasing controlled amounts of Rb vapor on demand while mitigating photonic degradation. Simultaneously, a counter-propagating desorption laser completely suppresses Rb-induced losses and enables waveguide-based atomic vapor spectroscopy. Using this approach, we demonstrate repeatable control of vapor density by tuning activation pulse length, duty cycle, and device temperature. These results establish a compact, manufacturable, and scalable vapor–PIC device, and set the stage for future demonstrations in cavity quantum electrodynamics, quantum nonlinear optics, and chip-scale atomic sensors.
Integrating alkali atomic vapors with nanophotonic devices offers a scalable route to quantum technologies that leverage strong atom-photon interactions. While there have been many approaches to such integration, the general reliance on traditional glass vapor cells, distilled alkali metals, and epoxy sealing limits reproducibility and scalability. Moreover, mitigating adverse Rb-photonics interactions is essential, particularly as devices become more compact and the alkali source lies in close proximity to the photonic elements. Here, we demonstrate the successful operation of compact and fully integrated devices that combine silicon nitride photonic integrated circuits (PICs) with microfabricated borosilicate vapor cells and pill-type rubidium (Rb) dispensers through hermetic seals via anodic bonding. We show how successful operation hinges on optically activating the dispenser in a low-power pulsed mode, releasing controlled amounts of Rb vapor on demand while mitigating photonic degradation. Simultaneously, a counter-propagating desorption laser completely suppresses Rb-induced losses and enables waveguide-based atomic vapor spectroscopy. Using this approach, we demonstrate repeatable control of vapor density by tuning activation pulse length, duty cycle, and device temperature. These results establish a compact, manufacturable, and scalable vapor-PIC device, and set the stage for future demonstrations in cavity quantum electrodynamics, quantum nonlinear optics, and chip-scale atomic sensors.
Long-range quantum network nodes require the combination of strong light-matter coupling, long coherence times and in situ spectral control at telecom wavelengths. The coherence of erbium in integrated devices is held back by its hosts, which do not simultaneously provide the weakly magnetic nuclear-spin environment and the well-defined substitutional sites found in coherence-optimised bulk crystals. Here we bring such an optimised crystal onto a photonic chip, by bonding an Er3+:CaWO4 host without an adhesive interlayer to a high-Q electro-optically tuneable thin-film lithium niobate microring resonator. At an effective temperature of 75 mK and a field of only 0.2 T, the bonded ensemble retains an effective homogeneous linewidth of 289±34 Hz (TM=1.10±0.13 ms), with spectral diffusion proceeding at 86±18 Hz and saturating at 1.5±0.2 kHz. Electro-optically tuning the resonator through the erbium optical transition resolves an avoided crossing with a collective cooperativity of C=6.7±0.4. Exploiting superhyperfine coupling to the host's 183W nuclear spins, we store and retrieve optical phase information over 5 s with a visibility of 0.935±0.015. Strong collective coupling, millisecond coherence and in situ spectral tuning in a single device thus establish heterogeneous integration leveraging coherence-optimised hosts as a route to scalable telecom quantum networks.