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arXiv:2003.04753 · Optics Express

Integrating two-photon nonlinear spectroscopy of rubidium atoms with silicon photonics

Artur Skljarow, Nico Gruhler, Wolfram Pernice, Harald Kübler, Tilman Pfau, Robert Löw, Hadiseh Alaeian

Published May 15, 2020• 15 citations
arXivHTMLPDF

Abstract

We study an integrated silicon photonic chip, composed of several sub-wavelength ridge waveguides, and immersed in a micro-cell with rubidium vapor. Employing two-photon excitation, including a telecom wavelength, we observe that the waveguide transmission spectrum gets modified when the photonic mode is coupled to rubidium atoms through its evanescent tail. Due to the enhanced electric field in the waveguide cladding, the atomic transition can be saturated at a photon number ≈80 times less than a free-propagating beam case. The non-linearity of the atom-clad Si-waveguide is about 4 orders of magnitude larger than the maximum achievable value in doped Si photonics. The measured spectra corroborate well with a generalized effective susceptibility model that includes the Casimir-Polder potentials, due to the dielectric surface, and the transient interaction between flying atoms and the evanescent waveguide mode. This work paves the way towards a miniaturized, low-power, and integrated hybrid atomic-photonic system compatible with CMOS technologies.

DOI
10.1364/oe.389644

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We study an integrated silicon photonic chip, composed of several sub-wavelength ridge waveguides, and immersed in a micro-cell with rubidium vapor. Employing two-photon excitation, including a telecom wavelength, we observe that the waveguide transmission spectrum gets modified when the photonic mode is coupled to rubidium atoms through its evanescent tail. Due to the enhanced electric field in the waveguide cladding, the atomic transition can be saturated at a photon number ≈80 times less than a free-propagating beam case. The non-linearity of the atom-clad Si-waveguide is about 4 orders of magnitude larger than the maximum achievable value in doped Si photonics. The measured spectra corroborate well with a generalized effective susceptibility model that includes the Casimir-Polder potentials, due to the dielectric surface, and the transient interaction between flying atoms and the evanescent waveguide mode. This work paves the way towards a miniaturized, low-power, and integrated hybrid atomic-photonic system compatible with CMOS technologies.
We investigate an integrated optical chip immersed in atomic vapor providing several waveguide geometries for spectroscopy applications. The narrow-band transmission through a silicon nitride waveguide and interferometer is altered when the guided light is coupled to a vapor of rubidium atoms via the evanescent tail of the waveguide mode. We use grating couplers to couple between the waveguide mode and the radiating wave, which allow for addressing arbitrary coupling positions on the chip surface. The evanescent atom-light interaction can be numerically simulated and shows excellent agreement with our experimental data. This work demonstrates a next step towards miniaturization and integration of alkali atom spectroscopy and provides a platform for further fundamental studies of complex waveguide structures.
We investigate an integrated optical chip immersed in atomic vapor providing several waveguide geometries for spectroscopy applications. The narrow-band transmission through a silicon nitride waveguide and interferometer is altered when the guided light is coupled to a vapor of rubidium atoms via the evanescent tail of the waveguide mode. We use grating couplers to couple between the waveguide mode and the radiating wave, which allow for addressing arbitrary coupling positions on the chip surface. The evanescent atom-light interaction can be numerically simulated and shows excellent agreement with our experimental data. This work demonstrates a next step towards miniaturization and integration of alkali atom spectroscopy and provides a platform for further fundamental studies of complex waveguide structures.
Alkali vapours, such as rubidium, are being used extensively in several important fields of research such as slow and stored light nonlinear optics quantum computation, atomic clocks and magnetometers. Recently, there is a growing effort towards miniaturizing traditional centimetre-size vapour cells. Owing to the significant reduction in device dimensions, light–matter interactions are greatly enhanced, enabling new functionalities due to the low power threshold needed for nonlinear interactions. Here, taking advantage of the mature platform of silicon photonics, we construct an efficient and flexible platform for tailored light–vapour interactions on a chip. Specifically, we demonstrate light–matter interactions in an atomic cladding waveguide, consisting of a silicon nitride nano-waveguide core with a rubidium vapour cladding. We observe the efficient interaction of the electromagnetic guided mode with the rubidium cladding and show that due to the high confinement of the optical mode, the rubidium absorption saturates at powers in the nanowatt regime. Alkali vapours are increasingly useful in photonic research and metrology applications, and they provide a useful test bed for investigating light–matter interaction. Stern et al. integrate silicon nitride waveguides with alkali vapours to study light–matter interactions on a chip-scale platform.
Accurate and stable frequency sources can be realized by locking lasers to well-known transitions between energy levels in isolated quantum systems such as alkali atoms. Unfortunately, current implementations of such frequency standards typically involve bulky optical setups and discrete optical components. Furthermore, the common transitions of alkali atoms are in the near-infrared, hindering their use as frequency references in the telecom regime. Our current work is focused on mitigating these deficiencies. In particular, we demonstrate the design, fabrication, and experimental characterization of an on-chip telecom frequency reference that is based on a ladder transition of rubidium atoms integrated with nanoscale optical waveguides. These atomic cladded waveguides are implemented in a serpentine geometry in order to optimize the chip area and maximize the interaction of light with the alkali atoms. Following its fabrication, the device is used to stabilize a telecom laser around a 1.5 μm wavelength to a precision better than 200 kHz at ∼250 s. Moreover, in spite of the fact that the natural lifetime of the excited state of the atom corresponding to only a few megahertz line widths, the nanoscale confinement of the optical mode dictates ultrashort interaction times and extreme photonic energy densities allowing us to demonstrate low power and faster (∼200 MHz) all-optical modulation of a near-infrared light with a telecom light. The results presented in this paper push forward the efforts toward fully integrated chip-scale stabilization system and provide an extremely efficient link between atomic based devices and silicon photonics platform in the telecom.
Devices based on spectroscopy of atomic vapors can measure physical quantities such as magnetic fields, RF electric fields, time and length, and rotation and have applications in a broad range of fields including communications, medicine, and navigation. We present a type of photonic device that interfaces single-mode silicon nitride optical waveguides with warm atomic vapors, enabling precision spectroscopy in an extremely compact (<1  cm3) package. We perform precision spectroscopy of rubidium confined in a micro-machined, 27  mm3 volume, vapor cell using a collimated free-space 120 μm diameter laser beam derived directly from a single-mode silicon nitride waveguide. With this optical-fiber integrated photonic spectrometer, we demonstrate an optical frequency reference at 780 nm with a stability of 10−11 from 1 to 104  s. This device harnesses the benefits of both photonic integration and precision spectroscopy for the next generation of quantum sensors and devices based on atomic vapors.