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ACS Photonics

Atom–Photon Interactions in Atomic Cladded Waveguides: Bridging Atomic and Telecom Technologies

Roy Zektzer, Eliran Talker, Yefim Barash, Noa Mazurski, Liron Stern, Uriel Levy

Published Feb 26, 2021• 16 citations
Publisher

Abstract

Accurate and stable frequency sources can be realized by locking lasers to well-known transitions between energy levels in isolated quantum systems such as alkali atoms. Unfortunately, current implementations of such frequency standards typically involve bulky optical setups and discrete optical components. Furthermore, the common transitions of alkali atoms are in the near-infrared, hindering their use as frequency references in the telecom regime. Our current work is focused on mitigating these deficiencies. In particular, we demonstrate the design, fabrication, and experimental characterization of an on-chip telecom frequency reference that is based on a ladder transition of rubidium atoms integrated with nanoscale optical waveguides. These atomic cladded waveguides are implemented in a serpentine geometry in order to optimize the chip area and maximize the interaction of light with the alkali atoms. Following its fabrication, the device is used to stabilize a telecom laser around a 1.5 μm wavelength to a precision better than 200 kHz at ∼250 s. Moreover, in spite of the fact that the natural lifetime of the excited state of the atom corresponding to only a few megahertz line widths, the nanoscale confinement of the optical mode dictates ultrashort interaction times and extreme photonic energy densities allowing us to demonstrate low power and faster (∼200 MHz) all-optical modulation of a near-infrared light with a telecom light. The results presented in this paper push forward the efforts toward fully integrated chip-scale stabilization system and provide an extremely efficient link between atomic based devices and silicon photonics platform in the telecom.

DOI
10.1021/acsphotonics.0c01895

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Accurate and stable frequency sources can be realized by locking lasers to well-known transitions between energy levels in isolated quantum systems such as alkali atoms. Unfortunately, current implementations of such frequency standards typically involve bulky optical setups and discrete optical components. Furthermore, the common transitions of alkali atoms are in the near-infrared, hindering their use as frequency references in the telecom regime. Our current work is focused on mitigating these deficiencies. In particular, we demonstrate the design, fabrication, and experimental characterization of an on-chip telecom frequency reference that is based on a ladder transition of rubidium atoms integrated with nanoscale optical waveguides. These atomic cladded waveguides are implemented in a serpentine geometry in order to optimize the chip area and maximize the interaction of light with the alkali atoms. Following its fabrication, the device is used to stabilize a telecom laser around a 1.5 μm wavelength to a precision better than 200 kHz at ∼250 s. Moreover, in spite of the fact that the natural lifetime of the excited state of the atom corresponding to only a few megahertz line widths, the nanoscale confinement of the optical mode dictates ultrashort interaction times and extreme photonic energy densities allowing us to demonstrate low power and faster (∼200 MHz) all-optical modulation of a near-infrared light with a telecom light. The results presented in this paper push forward the efforts toward fully integrated chip-scale stabilization system and provide an extremely efficient link between atomic based devices and silicon photonics platform in the telecom.
Alkali vapours, such as rubidium, are being used extensively in several important fields of research such as slow and stored light nonlinear optics quantum computation, atomic clocks and magnetometers. Recently, there is a growing effort towards miniaturizing traditional centimetre-size vapour cells. Owing to the significant reduction in device dimensions, light–matter interactions are greatly enhanced, enabling new functionalities due to the low power threshold needed for nonlinear interactions. Here, taking advantage of the mature platform of silicon photonics, we construct an efficient and flexible platform for tailored light–vapour interactions on a chip. Specifically, we demonstrate light–matter interactions in an atomic cladding waveguide, consisting of a silicon nitride nano-waveguide core with a rubidium vapour cladding. We observe the efficient interaction of the electromagnetic guided mode with the rubidium cladding and show that due to the high confinement of the optical mode, the rubidium absorption saturates at powers in the nanowatt regime. Alkali vapours are increasingly useful in photonic research and metrology applications, and they provide a useful test bed for investigating light–matter interaction. Stern et al. integrate silicon nitride waveguides with alkali vapours to study light–matter interactions on a chip-scale platform.
We study an integrated silicon photonic chip, composed of several sub-wavelength ridge waveguides, and immersed in a micro-cell with rubidium vapor. Employing two-photon excitation, including a telecom wavelength, we observe that the waveguide transmission spectrum gets modified when the photonic mode is coupled to rubidium atoms through its evanescent tail. Due to the enhanced electric field in the waveguide cladding, the atomic transition can be saturated at a photon number ≈80 times less than a free-propagating beam case. The non-linearity of the atom-clad Si-waveguide is about 4 orders of magnitude larger than the maximum achievable value in doped Si photonics. The measured spectra corroborate well with a generalized effective susceptibility model that includes the Casimir-Polder potentials, due to the dielectric surface, and the transient interaction between flying atoms and the evanescent waveguide mode. This work paves the way towards a miniaturized, low-power, and integrated hybrid atomic-photonic system compatible with CMOS technologies.
Photonic circuits are becoming very promising in many different applications, such as optical amplification, optical switching and wavelength division multiplexing optical networks, lab-on-chip in bioengineering, atom-light interaction in quantum information processing, wavelength selecting and filtering in astronomy, etc. Thanks to major developments in the nanofabrication technology, smaller but more powerful photonic circuits can be made to realize more complex applications. Here we propose two on-chip photonic circuits: one is for atom-light interaction in quantum information, and the other is for an optical spectrometer in astronomy. Part I The atom-light interaction can be used for a number of quantum based application, such as quantum information processing and atomic sensing. These significant applications make atom-light interaction a strong candidate for next-generation quantum computers and ultraprecise magnetic or navigation sensors. People have proposed various types of atom-photon interaction, and enhancing the interaction by using a small mode area has also been demonstrated in several platforms such as a hollow-core fiber, a hollow-core waveguide, a tapered fiber, and a nanowaveguide. In our work, we propose a nanowaveguide platform for collective atom-light interaction through the evanescent optical field coupling. We have demonstrated a centimeter-long silicon nitride nanowaveguide that has a sub-micrometer mode area and high fiber-to-waveguide coupling efficiencies for near-infrared wavelengths, working as evanescent field atom trapping/probing of an ensemble of 87Rb atoms. Inverse tapers are made at both ends of the waveguide that adiabatically transfer the weakly guided fiber-coupled mode to a strongly guided mode with an evanescent field for a better fiber-waveguide coupling efficiency. The coupling efficiency improves from around 2% to around 80% for both wavelengths. Trapping atoms by nanowaveguide modes is challenging because the small mode area generates high heat flux at the waveguide in an ultra-high vacuum. This platform has good thermal conductance and could transfer high enough optical powers to trap atoms in an ultra-high vacuum compared to a standalone photonic crystal waveguide with no substrate or an evanescent field coupled with a nanofiber. We have experimentally measured the optical absorption of thermal 87Rb atoms through the guided waveguide mode. We have also demonstrated an atom-chip mirror MOT with the same dimension of the platform that can be transferred to the proximity of the surface by magnetic field controls. Part II In astronomical applications, wavelength analysis is very important especially for the wavelength selecting and filtering. Here we focus on the wavelength range from 1µm to 1.7µm. There are many valuable applications that make this near infrared wavelength range so important. For example, the Lyman-alpha line of hydrogen is one of the very important emission lines of hydrogen for understanding the origin and creation of the universe. Since the universe has expanded for more than 10 billion years after the big bang, the Lyman-alpha line of hydrogen has redshifted from 121.5nm to the 1µm-to-1.7µm wavelength range according to Hubble’s Law. In addition, analysis of this wavelength range can also help us understand many other cosmic phenomena such as quasars, Gamma-ray bursts, etc. Therefore, a good spectrometer is needed to achieve this. Here we present an echelle grating which is based on an on-chip spectrometer that covers the near infrared wavelength range from 1.45um to 1.7um. To begin with, we use optical waveguides as the input and output channels. We have successfully achieved a reliable fabrication process to make the on-chip echelle-grating spectrometer. We have also achieved high fiber-waveguide coupling efficiency (94% per facet at 1550nm) and low propagation loss (-0.975dB/cm at 1550nm) for the input and output waveguides. In addition, we have characterized the bending loss of the waveguide. Finally, we have successfully measured the output spectrum of the echelle grating we designed and found it to be in good agreement with our simulation.
We combined experimental and theoretical investigations of an effective two-level atomic system operating in the near-infrared telecom wavelength regime, realized using hot rubidium vapor confined within a sub-micron-thick cell. In this strongly confined geometry, atomic coherence is profoundly influenced by wall-induced relaxation arising from frequent atom-surface collisions. By analyzing both absorption and fluorescence spectra, we demonstrate that the optical response is dominated by a closed cycling transition, which effectively isolates the atomic dynamics to a two-level configuration despite the presence of multiple hyperfine states. This confinement-induced selection suppresses optical pumping into uncoupled states and enables robust, controllable light-matter interaction at telecom wavelengths within a miniature atomic platform. Our results establish a practical route to realizing near-infrared atomic two-level systems in compact vapor-cell devices, opening new opportunities for integrated quantum photonic technologies, including on-chip quantum memories, telecom-band frequency references, and scalable quantum information processing.