Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2607.12665

Collective-State Preparation in a Subwavelength Triangular Trimer Using SUPER Excitation

Thomas Nunner, Johannes Kerber, Helmut Ritsch, Arpita Pal

physics.opticsquant-phSubmitted Jul 14, 2026• Announced Jul 15, 2026• 0 citations
v1 · Jul 14, 2026v2 · Sep 24, 2026
arXivHTMLPDF

Abstract

The Swing-UP of quantum EmitteR population (SUPER) scheme has recently been proposed as a deterministic method for the preparation of collective radiative states in two strongly dipole-coupled quantum emitters (Phys. Rev. Res. \textbf{8}, 013179 (2026)). Here, we extend this approach to an equilateral subwavelength triangular trimer of dipole-coupled two-level quantum emitters (QEs), loosely inspired by biological light-harvesting ring geometries. Using tailored, time-overlapping, red-detuned ultrashort SUPER pulses, we numerically investigate the selective preparation of collective target states. We find that both the state selectivity and the preparation efficiency depend strongly on the inter-emitter spacing. In particular, at deep-subwavelength separations, the symmetric collective state can be deterministically prepared with near-unity efficiency, whereas the inversion efficiency and state selectivity are significantly lower at larger inter-emitter separations. Furthermore, this state preparation technique inherits a certain degree of robustness against reasonable static position imperfections and on-site frequency inhomogeneities of the individual QEs. Our results demonstrate that deep-subwavelength triangular trimers and, more broadly, highly compact ring geometries are excellent candidates for the deterministic preparation of collective radiative states via SUPER excitation. These predictions could be realized with solid-state emitters and molecules. Our findings offer a route toward the direct probing of the `pure' electromagnetic layer of interaction in biological and bio-inspired synthetic nanophotonic ring configurations, with possible relevance in photonics, quantum information processing, and metrology.

Comments
9 pages including Appendices, 4 figures, and 1 table

Related papers

Selective preparation of collective states in coupled quantum emitters using the SUPER excitation scheme

Johannes Kerber, Laurin Ostermann, Vikas Remesh +2 more

The efficient preparation of collective eigenstates of subwavelength-spaced optical dipoles is a prerequisite for observing their signature radiative properties and for their applications in quantum information processing. We theoretically investigate the deterministic preparation of super- and subradiant states of two dipole-coupled two-level quantum emitters at deep-subwavelength separation using the Swing-UP of quantum EmitteR population (SUPER) excitation scheme. Utilizing suitable pulse parameters for two red-detuned, time-overlapping Gaussian pulses, the SUPER scheme enables close-to-unity population inversion in the targeted collective eigenstates. Furthermore, a tunable optical phase in the SUPER scheme enables the simultaneous inversions in both pure super- and subradiant states with finite populations, thereby resulting in the preparation of hybrid collective states. These results are possible to realize with or without an optical cavity. Our approach to populating the collective eigenstates in a cavity environment paves the way for the efficient preparation of these states in the presence of environmental decoherence. Our scheme enables single-photon generation, which is measured using the second-order correlation function. We also discuss in detail possible experimental realizations, in particular using solid-state emitters and molecules.

arXiv:2508.19692•Physical Review Research•Jan 20, 2026•1 citation

Harnessing quantum emitter rings for efficient energy transport and trapping

Raphael Holzinger, Jonah S. Peter, Stefan Ostermann +2 more

Efficient transport and harvesting of excitation energy under low light conditions is an important process in nature and quantum technologies alike. Here we formulate a quantum optics perspective to excitation energy transport in configurations of two-level quantum emitters with a particular emphasis on efficiency and robustness against disorder. We study a periodic geometry of emitter rings with subwavelength spacing, where collective electronic states emerge due to near-field dipole–dipole interactions. The system gives rise to collective subradiant states that are particularly suited to excitation transport and are protected from energy disorder and radiative decoherence. Comparing ring geometries with other configurations shows that the former are more efficient in absorbing, transporting, and trapping incident light. Because our findings are agnostic as to the specific choice of quantum emitters, they indicate general design principles for quantum technologies with superior photon transport properties and may elucidate potential mechanisms resulting in the highly efficient energy transport efficiencies in natural light-harvesting systems.

arXiv:2309.11376•Optica Quantum•Jan 30, 2024•21 citations

Efficient excitation transfer in an LH2-inspired nanoscale stacked ring geometry

Arpita Pal, Raphael Holzinger, Maria Moreno-Cardoner +1 more

Abstract Ring geometries of subwavelength-spaced quantum emitters exhibit outstanding radiation properties and are useful for antennas, excitation transport, and storage. Taking inspiration from the oligomeric geometry, in particular by considering only the position and dipole orientations of the bacteriochlorophylls in biological light-harvesting 2 complexes of (approximately 6 nm in diameter), we propose and predict highly efficient interlayer excitation transfer, achieving a maximum of 100% transfer for certain choices of dipole orientations in a three-dimensional (3D) concentric stacked ring geometry with C 9 symmetry and a diameter of 400 nm, formed by two-level atoms. Utilizing the quantum optical open system Lindblad master equation approach for estimating the collective dipole dynamics, we demonstrate that, depending on the system parameters, our bio-inspired 3D ring of quantum emitters enables efficient asymmetric excitation transfer between two ring layers, in particular from sparse to dense quantum emitter arrangements. The presented nanoscale geometry is expected to be realizable with diverse physical platforms operating at cryogenic temperatures, where the interacting dipole description remains applicable and, importantly, dominant over environmental decoherence.

arXiv:2409.15288•New Journal of Physics•Aug 22, 2025•1 citation

Cooperative subwavelength molecular quantum emitter arrays

R. Holzinger, S. A. Oh, Michael Reitz +2 more

Dipole-coupled subwavelength quantum emitter arrays respond cooperatively to external light fields as they may host collective delocalized excitations (a form of excitons) with super- or subradiant character. Deeply subwavelength separations typically occur in molecular ensembles, where in addition to photon-electron interactions, electron-vibron couplings and vibrational relaxation processes play an important role. We provide analytical and numerical results on the modification of super- and subradiance in molecular rings of dipoles including excitations of the vibrational degrees of freedom. While vibrations are typically considered detrimental to coherent dynamics, we show that molecular dimers or rings can be operated as platforms for the preparation of long-lived dark superposition states aided by vibrational relaxation. In closed ring configurations, we extend previous predictions for the generation of coherent light from ideal quantum emitters to molecular emitters, quantifying the role of vibronic coupling onto the output intensity and coherence.

arXiv:2203.04998•Physical Review Research•Aug 11, 2022•17 citations

Swing-up dynamics in quantum emitter cavity systems: Near ideal single photons and entangled photon pairs

Nils Heinisch, Nikolas Köcher, David Bauch +1 more

In the SUPER scheme (Swing-UP of the quantum EmitteR population), excitation of a quantum emitter is achieved with two off-resonant, red-detuned laser pulses. This allows the generation of high-quality single photons without the need of complex laser stray light suppression or careful spectral filtering. In the present work, we extend this promising method to quantum emitters, specifically semiconductor quantum dots, inside a resonant optical cavity. A significant advantage of the SUPER scheme is identified in that it eliminates re-excitation of the quantum emitter by suppressing photon emission during the excitation cycle. This, in turn, leads to almost ideal single-photon purity, overcoming a major factor typically limiting the quality of photons generated with quantum emitters in high-quality cavities. We further find that for cavity-mediated biexciton emission of degenerate photon pairs, the SUPER scheme leads to near-perfect biexciton initialization with very high values of polarization entanglement of emitted photon pairs. Published by the American Physical Society 2024

arXiv:2303.12604•Physical Review Research•Jan 19, 2024•14 citations

Selective protected state preparation of coupled dissipative quantum emitters

D. Plankensteiner, L. Ostermann, H. Ritsch +1 more

Inherent binary or collective interactions in ensembles of quantum emitters induce a spread in the energy and lifetime of their eigenstates. While this typically causes fast decay and dephasing, in many cases certain special entangled collective states with minimal decay can be found, which possess ideal properties for spectroscopy, precision measurements or information storage. We show that for a specific choice of laser frequency, power and geometry or a suitable configuration of control fields one can efficiently prepare these states. We demonstrate this by studying preparation schemes for strongly subradiant entangled states of a chain of dipole-dipole coupled emitters. The prepared state fidelity and its entanglement depth is further improved via spatial excitation phase engineering or tailored magnetic fields.

arXiv:1504.08148•Scientific Reports•Nov 9, 2015•68 citations
The Swing-UP of quantum EmitteR population (SUPER) scheme has recently been proposed as a deterministic method for the preparation of collective radiative states in two strongly dipole-coupled quantum emitters (Phys. Rev. Res. \textbf{8}, 013179 (2026)). Here, we extend this approach to an equilateral subwavelength triangular trimer of dipole-coupled two-level quantum emitters (QEs), loosely inspired by biological light-harvesting ring geometries. Using tailored, time-overlapping, red-detuned ultrashort SUPER pulses, we numerically investigate the selective preparation of collective target states. We find that both the state selectivity and the preparation efficiency depend strongly on the inter-emitter spacing. In particular, at deep-subwavelength separations, the symmetric collective state can be deterministically prepared with near-unity efficiency, whereas the inversion efficiency and state selectivity are significantly lower at larger inter-emitter separations. Furthermore, this state preparation technique inherits a certain degree of robustness against reasonable static position imperfections and on-site frequency inhomogeneities of the individual QEs. Our results demonstrate that deep-subwavelength triangular trimers and, more broadly, highly compact ring geometries are excellent candidates for the deterministic preparation of collective radiative states via SUPER excitation. These predictions could be realized with solid-state emitters and molecules. Our findings offer a route toward the direct probing of the `pure' electromagnetic layer of interaction in biological and bio-inspired synthetic nanophotonic ring configurations, with possible relevance in photonics, quantum information processing, and metrology.
The efficient preparation of collective eigenstates of subwavelength-spaced optical dipoles is a prerequisite for observing their signature radiative properties and for their applications in quantum information processing. We theoretically investigate the deterministic preparation of super- and subradiant states of two dipole-coupled two-level quantum emitters at deep-subwavelength separation using the Swing-UP of quantum EmitteR population (SUPER) excitation scheme. Utilizing suitable pulse parameters for two red-detuned, time-overlapping Gaussian pulses, the SUPER scheme enables close-to-unity population inversion in the targeted collective eigenstates. Furthermore, a tunable optical phase in the SUPER scheme enables the simultaneous inversions in both pure super- and subradiant states with finite populations, thereby resulting in the preparation of hybrid collective states. These results are possible to realize with or without an optical cavity. Our approach to populating the collective eigenstates in a cavity environment paves the way for the efficient preparation of these states in the presence of environmental decoherence. Our scheme enables single-photon generation, which is measured using the second-order correlation function. We also discuss in detail possible experimental realizations, in particular using solid-state emitters and molecules.
Efficient transport and harvesting of excitation energy under low light conditions is an important process in nature and quantum technologies alike. Here we formulate a quantum optics perspective to excitation energy transport in configurations of two-level quantum emitters with a particular emphasis on efficiency and robustness against disorder. We study a periodic geometry of emitter rings with subwavelength spacing, where collective electronic states emerge due to near-field dipole–dipole interactions. The system gives rise to collective subradiant states that are particularly suited to excitation transport and are protected from energy disorder and radiative decoherence. Comparing ring geometries with other configurations shows that the former are more efficient in absorbing, transporting, and trapping incident light. Because our findings are agnostic as to the specific choice of quantum emitters, they indicate general design principles for quantum technologies with superior photon transport properties and may elucidate potential mechanisms resulting in the highly efficient energy transport efficiencies in natural light-harvesting systems.
Abstract Ring geometries of subwavelength-spaced quantum emitters exhibit outstanding radiation properties and are useful for antennas, excitation transport, and storage. Taking inspiration from the oligomeric geometry, in particular by considering only the position and dipole orientations of the bacteriochlorophylls in biological light-harvesting 2 complexes of (approximately 6 nm in diameter), we propose and predict highly efficient interlayer excitation transfer, achieving a maximum of 100% transfer for certain choices of dipole orientations in a three-dimensional (3D) concentric stacked ring geometry with C 9 symmetry and a diameter of 400 nm, formed by two-level atoms. Utilizing the quantum optical open system Lindblad master equation approach for estimating the collective dipole dynamics, we demonstrate that, depending on the system parameters, our bio-inspired 3D ring of quantum emitters enables efficient asymmetric excitation transfer between two ring layers, in particular from sparse to dense quantum emitter arrangements. The presented nanoscale geometry is expected to be realizable with diverse physical platforms operating at cryogenic temperatures, where the interacting dipole description remains applicable and, importantly, dominant over environmental decoherence.
Dipole-coupled subwavelength quantum emitter arrays respond cooperatively to external light fields as they may host collective delocalized excitations (a form of excitons) with super- or subradiant character. Deeply subwavelength separations typically occur in molecular ensembles, where in addition to photon-electron interactions, electron-vibron couplings and vibrational relaxation processes play an important role. We provide analytical and numerical results on the modification of super- and subradiance in molecular rings of dipoles including excitations of the vibrational degrees of freedom. While vibrations are typically considered detrimental to coherent dynamics, we show that molecular dimers or rings can be operated as platforms for the preparation of long-lived dark superposition states aided by vibrational relaxation. In closed ring configurations, we extend previous predictions for the generation of coherent light from ideal quantum emitters to molecular emitters, quantifying the role of vibronic coupling onto the output intensity and coherence.
In the SUPER scheme (Swing-UP of the quantum EmitteR population), excitation of a quantum emitter is achieved with two off-resonant, red-detuned laser pulses. This allows the generation of high-quality single photons without the need of complex laser stray light suppression or careful spectral filtering. In the present work, we extend this promising method to quantum emitters, specifically semiconductor quantum dots, inside a resonant optical cavity. A significant advantage of the SUPER scheme is identified in that it eliminates re-excitation of the quantum emitter by suppressing photon emission during the excitation cycle. This, in turn, leads to almost ideal single-photon purity, overcoming a major factor typically limiting the quality of photons generated with quantum emitters in high-quality cavities. We further find that for cavity-mediated biexciton emission of degenerate photon pairs, the SUPER scheme leads to near-perfect biexciton initialization with very high values of polarization entanglement of emitted photon pairs. Published by the American Physical Society 2024
Inherent binary or collective interactions in ensembles of quantum emitters induce a spread in the energy and lifetime of their eigenstates. While this typically causes fast decay and dephasing, in many cases certain special entangled collective states with minimal decay can be found, which possess ideal properties for spectroscopy, precision measurements or information storage. We show that for a specific choice of laser frequency, power and geometry or a suitable configuration of control fields one can efficiently prepare these states. We demonstrate this by studying preparation schemes for strongly subradiant entangled states of a chain of dipole-dipole coupled emitters. The prepared state fidelity and its entanglement depth is further improved via spatial excitation phase engineering or tailored magnetic fields.