Efficient transport and harvesting of excitation energy under low light conditions is an important process in nature and quantum technologies alike. Here we formulate a quantum optics perspective to excitation energy transport in configurations of two-level quantum emitters with a particular emphasis on efficiency and robustness against disorder. We study a periodic geometry of emitter rings with subwavelength spacing, where collective electronic states emerge due to near-field dipole–dipole interactions. The system gives rise to collective subradiant states that are particularly suited to excitation transport and are protected from energy disorder and radiative decoherence. Comparing ring geometries with other configurations shows that the former are more efficient in absorbing, transporting, and trapping incident light. Because our findings are agnostic as to the specific choice of quantum emitters, they indicate general design principles for quantum technologies with superior photon transport properties and may elucidate potential mechanisms resulting in the highly efficient energy transport efficiencies in natural light-harvesting systems.
Efficient transport and harvesting of excitation energy under low light conditions is an important process in nature and quantum technologies alike. Here we formulate a quantum optics perspective to excitation energy transport in configurations of two-level quantum emitters with a particular emphasis on efficiency and robustness against disorder. We study a periodic geometry of emitter rings with subwavelength spacing, where collective electronic states emerge due to near-field dipole–dipole interactions. The system gives rise to collective subradiant states that are particularly suited to excitation transport and are protected from energy disorder and radiative decoherence. Comparing ring geometries with other configurations shows that the former are more efficient in absorbing, transporting, and trapping incident light. Because our findings are agnostic as to the specific choice of quantum emitters, they indicate general design principles for quantum technologies with superior photon transport properties and may elucidate potential mechanisms resulting in the highly efficient energy transport efficiencies in natural light-harvesting systems.
Decoherence is mostly detrimental in quantum information and quantum optics applications. However, the interplay between environment-induced incoherent dynamics and unitary evolution can give rise to novel quantum many-body phenomena that can be harnessed as a useful resource. As is well known, in dense subwavelength atomic arrays only a single collective eigenmode in the single-excitation manifold couples strongly to free-space radiation, exhibiting superradiant spontaneous emission. Most of the remaining eigenstates form a manifold of weakly radiative modes, giving rise to long-lived subradiant excitations. Here we demonstrate that populating these subradiant modes via additional decoherence mechanisms, such as dephasing or coupling to phonons, can significantly enhance single-photon absorption in a nanoring of quantum emitters. Such nanoring geometry is particularly appealing due to its unique optical properties and its resemblance to natural light-harvesting complexes, which serve as efficient antennas in photosynthesis. Our findings may shed light on fundamental aspects of energy absorption in nature; despite the much greater complexity of biological systems, they may nonetheless operate according to similar underlying optical principles.
Abstract Ring geometries of subwavelength-spaced quantum emitters exhibit outstanding radiation properties and are useful for antennas, excitation transport, and storage. Taking inspiration from the oligomeric geometry, in particular by considering only the position and dipole orientations of the bacteriochlorophylls in biological light-harvesting 2 complexes of (approximately 6 nm in diameter), we propose and predict highly efficient interlayer excitation transfer, achieving a maximum of 100% transfer for certain choices of dipole orientations in a three-dimensional (3D) concentric stacked ring geometry with C 9 symmetry and a diameter of 400 nm, formed by two-level atoms. Utilizing the quantum optical open system Lindblad master equation approach for estimating the collective dipole dynamics, we demonstrate that, depending on the system parameters, our bio-inspired 3D ring of quantum emitters enables efficient asymmetric excitation transfer between two ring layers, in particular from sparse to dense quantum emitter arrangements. The presented nanoscale geometry is expected to be realizable with diverse physical platforms operating at cryogenic temperatures, where the interacting dipole description remains applicable and, importantly, dominant over environmental decoherence.
Subwavelength arrays of quantum emitters feature unique and largely design-able nonlinear optical properties. As a generic example we study a sub-wavelength sized ring of identical dipoles with an extra identical absorbing emitter at the center. For a 9-ring one finds the most efficient antenna configuration to direct single incoming photons to the center without re-emission. Interestingly, for very tiny structures sizes below a tenth of a wavelength, a full quantum description predicts an even larger absorption enhancement than a mean field model using a classical dipole approximation. We identify the origin of the enhancement in the appearance of a collective dark state with dominant center occupation. By special design of the center absorber one thus can harness the same efficiency enhancement also at different wavelengths and for other geometric structures. On the one hand this idea could be the basis of a new generation of highly efficient and selective nano antennas, while on the other hand, it could be an important piece towards understanding the surprising efficiency of natural light harvesting molecules. Adding gain via active dipoles in such nano ring systems allows to design minimalist laser like classical light sources. In the nonlinear operating regime at stronger pump fields these systems transform to non-classical light sources with tailor-able spatio-temporal emission upon coherent illumination.
Collective excitations in ordered subwavelength atomic arrays can exhibit strongly suppressed radiative decay due to interference between light scattered by neighboring emitters. These so-called subradiant states make these systems a promising platform for storing and manipulating photonic excitations. The external geometry of the array, combined with dynamical control of the atomic dipole orientation, enables localized trapping and coherent transport of these subradiant excitations. Here, we theoretically demonstrate these capabilities in ring-shaped atomic arrays. Specifically, we show adiabatic transport of a localized excitation around a single ring, coherent transfer of a single excitation between two neighboring rings with geometry-controlled selectivity, and interaction-induced conditional phase shifts between two simultaneously trapped excitations in neighboring rings. The latter can be interpreted as effective controlled-phase operations between stored excitations. Together, these results demonstrate the potential of ordered atomic arrays as a platform for coherent photonic quantum information processing with dissipation-protected collective excitations.
A ring of dipole-coupled quantum emitters positioned at subwavelength distances possesses only a few radiant but many subradiant collective excitations with lifetimes growing exponentially with the atom number. These exhibit a three-dimensionally confined spatial radiation field pattern and form nanoscale high-Q optical resonators. Tailoring size, orientation, and distance between two rings allows for increasing the ratio of coherent ring-to-ring energy transfer versus free-space emission by orders of magnitude. In particular, the more dark and delocalized over several sites are excitons, the higher is their fidelity for transport to a second ring.
The Swing-UP of quantum EmitteR population (SUPER) scheme has recently been proposed as a deterministic method for the preparation of collective radiative states in two strongly dipole-coupled quantum emitters (Phys. Rev. Res. \textbf{8}, 013179 (2026)). Here, we apply this approach to an equilateral subwavelength triangular trimer of dipole-coupled two-level quantum emitters (QEs), loosely inspired by biological light-harvesting ring geometries, and demonstrate that tailored, time-overlapping, red-detuned ultrashort SUPER pulses can selectively prepare collective states in a C3-symmetric system, including energetically degenerate eigenstates that are resolved through site-dependent optical phases. We find that both the state selectivity and the preparation efficiency depend strongly on the inter-emitter spacing. In particular, at deep-subwavelength separations, the symmetric collective state can be deterministically prepared with near-unity efficiency (approximately 94%), whereas the inversion efficiency and state selectivity are significantly lower at larger inter-emitter separations. Furthermore, this state preparation technique inherits a certain degree of robustness against reasonable static position imperfections and on-site frequency inhomogeneities of the individual QEs. Our results demonstrate that deep-subwavelength triangular trimers and, more broadly, highly compact ring geometries are excellent candidates for the deterministic preparation of collective radiative states via SUPER excitation. These predictions could be realized with solid-state emitters and molecules. Our findings offer a route toward the direct probing of the `pure' electromagnetic layer of interaction in biological and bio-inspired synthetic nanophotonic ring configurations, with possible relevance in photonics, quantum information processing, and metrology.