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arXiv:2607.09896

Dark Optical Trapping of Resonant Transition-Metal Dichalcogenide Particles

Patrick Illetschek, Gleb Fedorovich, Albert Seredin, Gleb Tselikov, Valentin S. Volkov, Nikolai Kiesel, Markus Aspelmeyer, Mihail Petrov, Anton V. Zasedatelev

physics.opticsquant-phSubmitted Jul 10, 2026• Announced Jul 14, 2026• 0 citations
arXivHTMLPDF

Abstract

Mitigating recoil events and minimizing optically induced heating are central challenges in the precise control and cooling of macroscopic particles. To overcome this, we propose trapping resonant dielectric particles for applications in ultra-high vacuum (UHV) levitodynamics. Contrary to other approaches, where suppressing the parasitic resonant scattering was achieved in a standing wave geometry, here we propose a single beam geometry in a dark trap regime. As a promising material platform, we focus on a class of transition-metal dichalcogenide (TMD) particles with high polarizability, characterized by refractive indices in the range $3.7$-$4.8$ and densities up to $9.3~\mathrm{g\,cm^{-3}}$. Using full Mie theory, we identify a range of TMD particle radii that support stable axial and radial magnetic quadrupole trapping in a bottle-beam configuration. We predict that for WS$_2$ particles with a mass of $0.5 \times 10^{12}\,\mathrm{amu}$, one can expect suppression of the scattering rate relative to the mechanical frequency down to $Γ/Ω\simeq 0.02$. This corresponds to a coherence time extended by approximately three orders of magnitude compared with silica particles of the same mass trapped in conventional bright optical traps at UHV. Combined with significantly reduced internal heating, remaining well below the melting point of the material, dark trapping of resonant TMD macroscopic particles emerges as a promising platform for exploring quantum physics with large masses.

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Mitigating recoil events and minimizing optically induced heating are central challenges in the precise control and cooling of macroscopic particles. To overcome this, we propose trapping resonant dielectric particles for applications in ultra-high vacuum (UHV) levitodynamics. Contrary to other approaches, where suppressing the parasitic resonant scattering was achieved in a standing wave geometry, here we propose a single beam geometry in a dark trap regime. As a promising material platform, we focus on a class of transition-metal dichalcogenide (TMD) particles with high polarizability, characterized by refractive indices in the range 3.73.73.7-4.84.84.8 and densities up to 9.3 g cm−39.3~\mathrm{g\,cm^{-3}}9.3 gcm−3. Using full Mie theory, we identify a range of TMD particle radii that support stable axial and radial magnetic quadrupole trapping in a bottle-beam configuration. We predict that for WS2_22​ particles with a mass of 0.5×1012 amu0.5 \times 10^{12}\,\mathrm{amu}0.5×1012amu, one can expect suppression of the scattering rate relative to the mechanical frequency down to Γ/Ω≃0.02Γ/Ω\simeq 0.02Γ/Ω≃0.02. This corresponds to a coherence time extended by approximately three orders of magnitude compared with silica particles of the same mass trapped in conventional bright optical traps at UHV. Combined with significantly reduced internal heating, remaining well below the melting point of the material, dark trapping of resonant TMD macroscopic particles emerges as a promising platform for exploring quantum physics with large masses.
Optically levitated and cooled nanoparticles are a new quantum system whose application to the creation of non-classical states of motion and quantum limited sensing is fundamentally limited by recoil and bulk heating. We study the creation of stable 3D optical traps using optical cylindrically polarized vortex beams with radial and azimuthal polarization and show that a significant reduction in recoil heating by up to an order of magnitude can be achieved when compared with conventional single Gaussian beam tweezers. Additionally these beams allow trapping of larger particles outside the Rayleigh regime using both bright and dark tweezer trapping with reduced recoil heating. By changing the wavelength of the trapping laser, or the size of the particles, non-linear and repulsive potentials of interest for the creation of non-classical states of motion can also be created.
High-refractive-index particles have recently attracted a growing interest in optical levitation experiments, offering the ability to further engineer optical forces through electromagnetic Mie resonances. Unlike standard silica particles, which are predominantly trapped in the dipole regime and exhibit trap frequencies mainly determined by material density, resonant meta-atoms formed by high-index particles enable qualitatively new trapping behaviors. In this work, we experimentally investigate the trapping of resonant silicon particles in an optical standing wave. A direct comparison of silicon and silica highlights the fundamental differences in their optical force scaling and trapping dynamics. Beyond conventional trapping at intensity-maxima, we demonstrate deterministic and stable three-dimensional trapping of silicon nanoparticles in optical intensity minima, a regime that remains inaccessible for silica particles. Drawing a mesoscopic analogy with blue-detuned atom trapping, our results establish meta-atoms as a versatile approach to further extend the optical manipulation tool box towards accessing novel trapping regimes e.g. in close proximity to a surface.
We demonstrate optical levitation and feedback cooling of a silica nanoparticle (radius = 78~nm) trapped within a radial vector beam (RVB) in high vacuum. Radial vector beams, when focused by a high-NA lens, produce a smaller focal spot than conventional Gaussian beams, yielding tighter optical potentials and potentially reduced photon-recoil heating rates. A vortex wave plate was used to generate the RVB using an aspheric lens (NA = 0.77) to form the trap. Cold-damping feedback was used to cool the center of mass motion in the radial and axial trap directions to temperatures in the mK range. At higher temperatures and pressures, additional trap frequencies arising from the nonlinear RVB optical potential are observed. This demonstration is a step toward exploiting structured light for levitated quantum optomechanics where these traps can be used to suppress bulk and motional heating.
This thesis reports on the design, setup, and operation of a new atom trap apparatus, which is developed to confine few rubidium atoms in ultrahigh vacuum by means of taylored and dynamically variable light potentials (dipole traps), thus making the atoms available for spectroscopy and controlled manipulations. To maintain low background pressure, atoms of a vapour cell are transferred into a cold atomic beam by laser cooling techniques, and accumulated by a magneto-optic trap (MOT) in a separate part of the vacuum system. The laser cooled atoms are then transferred into dipole traps made of focused far-off-resonant laser fields in single or crossed-beam geometry, which are superimposed with the center of the MOT. Gaussian as well as hollow Laguerre-Gaussian (LG01) beam profiles are used with red-detuned and blue-detuned light. Microfabricated dielectric phase objects allow the efficient and robust mode conversion of Gaussian into Laguerre-Gaussian laser beams. Trap geometries can easily be changed due to the highly flexible experimental setup. The dipole trap laser beams have powers up to several hundred milliwatts and are focused to around 10 m. At a detuning of several tens of nanometers from the atomic resonance, the resulting traps are a few millikelvin deep, and the trapped atoms exhibit motional frequencies near 30 kHz, trap light scattering rates of a few hundred photons per second per atom, and storage times of several seconds. The number of dipole-trapped atoms ranges from more than ten thousand to below ten. The dipole-trapped atoms are detected either by a photon counting system with efficient straylight discrimination, or by recapture into the MOT, which is imaged onto a sensitive photodiode and a CCD-camera. Due to the strong AC-Stark shift imposed by the high-intensity trapping light, energy-selective resonant excitation and detection of the stored atoms is possible. The measured energy distribution is consistent with a harmonic potential shape and allows for the determination of temperatures and heating rates. From initial measurements, the thermal energy is found to be about 10 % of the trap depth. Using a crossed-beam geometry with red-detuned laser light, efficient transfer of atoms between the beams is observed. Optimum transfer occurs when the two beams cross at a radial offset, which can qualitatively be understood when the particle energy and geometrical properties of the two-beam trapping potential are considered. Numerical simulations reproduce the general features of the measured transfer efficiency vs. radial beam offset. This experiment is a first step towards dynamically variable potentials. Atoms have been radially confined in a blue-detuned hollow beam, and their decay time has been determined. This configuration is currently extended to a three-dimensionally confining blue-detuned dipole trap. For advanced laser cooling, state manipulation and spectroscopy of trapped atoms, a system of two diode lasers has been set up which are phase-coherently locked with a difference frequency near 6.834 GHz, to drive Raman transitions between the hyperfine-split ground states of 87Rb atoms. Resonances of such a transition have been recorded in a buffer gas loaded rubidium vapour cell with linewidths below 100 Hz.
Many well theoretically motivated models of ultralight dark matter are expected to give rise to feeble oscillatory forces on macroscopic objects. Optically trapped sensors have high force sensitivities but have remained relatively unexplored in this context. In this work we propose a new, tunable, optically trapped sensor specifically designed to detect such forces. Our design features a high-mass (∼\sim∼ mg) plate whose high aspect ratio allows its weight to be supported by a vertical beam without excessive heating. We present the first systematic analysis and optimisation of quantum noises in optically trapped systems and show that our setup has the potential to operate at the standard quantum limit with current off-the-shelf technologies. We demonstrate that our sensor could offer unique access to large regions of uncharted parameter space of vector B-L dark matter, with projected sensitivities that could advance existing limits by several orders of magnitude over a broad range of frequencies.
The levitation of condensed matter in vacuum allows the study of its physical properties under extreme isolation from the environment. It also offers a venue to investigate quantum mechanics with large systems, at the transition between the quantum and classical worlds. In this work, we study a novel hybrid levitation platform that combines a Paul trap with a weak but highly focused laser beam, a configuration that integrates a deep potential with excellent confinement and motion detection. We combine simulations and experiments to demonstrate the potential of this approach to extend vacuum trapping and interrogation to a broader range of nanomaterials, such as absorbing particles. We study the stability and dynamics of different specimens, such as fluorescent dielectric crystals and gold nanorods, and demonstrate stable trapping down to pressures of 1 mbar.