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arXiv:2005.05486 · Nano Letters

Extending Vacuum Trapping to Absorbing Objects with Hybrid Paul-Optical Traps

Gerard P. Conangla, Raúl A. Rica, Romain Quidant

Published Jul 21, 2020• 46 citations
arXivHTMLPDF

Abstract

The levitation of condensed matter in vacuum allows the study of its physical properties under extreme isolation from the environment. It also offers a venue to investigate quantum mechanics with large systems, at the transition between the quantum and classical worlds. In this work, we study a novel hybrid levitation platform that combines a Paul trap with a weak but highly focused laser beam, a configuration that integrates a deep potential with excellent confinement and motion detection. We combine simulations and experiments to demonstrate the potential of this approach to extend vacuum trapping and interrogation to a broader range of nanomaterials, such as absorbing particles. We study the stability and dynamics of different specimens, such as fluorescent dielectric crystals and gold nanorods, and demonstrate stable trapping down to pressures of 1 mbar.

DOI
10.1021/acs.nanolett.0c02025

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The levitation of condensed matter in vacuum allows the study of its physical properties under extreme isolation from the environment. It also offers a venue to investigate quantum mechanics with large systems, at the transition between the quantum and classical worlds. In this work, we study a novel hybrid levitation platform that combines a Paul trap with a weak but highly focused laser beam, a configuration that integrates a deep potential with excellent confinement and motion detection. We combine simulations and experiments to demonstrate the potential of this approach to extend vacuum trapping and interrogation to a broader range of nanomaterials, such as absorbing particles. We study the stability and dynamics of different specimens, such as fluorescent dielectric crystals and gold nanorods, and demonstrate stable trapping down to pressures of 1 mbar.
We present a hybrid trapping platform that allows us to levitate a charged nanoparticle in high vacuum using either optical fields, radio-frequency fields, or a combination thereof. Our hybrid approach combines an optical dipole trap with a linear Paul trap while maintaining a large numerical aperture (0.77 NA). We detail a controlled transfer procedure that allows us to use the Paul trap as a “safety net” to recover particles lost from the optical trap at high vacuum. The presented hybrid platform adds to the toolbox of levitodynamics and represents an important step towards fully controllable “dark” potentials, providing control in the absence of decoherence because of photon recoil. Published by the American Physical Society 2024
In this M.Phil thesis, a hybrid trap for optomechanical studies of mesoscopic particle is investigated. It uses a Planar Paul Trap (PPT) for electrical confinement and a parabolic mirror for optical confinement. The PPT is compatible with the printed circuit board (PCB) technology making it easier to integrate with the mirror trap. This compatibility also simplifies particle loading, enhances ground state cooling and improves optical interrogation within the trap. It can create various potential landscapes of a quartic potential, including double well or inverted harmonic, and is a potential tool for investigating macroscopic quantum superposition states. This planar geometry of the Paul trap allows large optical access required for optical confinement and detection of the particle. The parabolic mirror provides the benefits of virtually no chromatic aberration, high numerical aperture and functioning as an additional RF electrode of the hybrid trap. The work includes simulations and experiments to characterize the hybrid trap by analyzing the effective trapping potential. From the numerical simulations, the ratio of axial to radial secular frequencies of the trapped particle under the RF drive is = 0.98, implying the chosen parameters of the PPT + mirror RF trap has approximately the same stiffness and hence confinement in the axial and radial directions. It is also observed that the dynamics of a single particle under the RF drive is not affected by damping and random forces in a high vacuum (∼ 10-6 mbar).
Levitodynamics is a fast growing field that studies the levitation and manipulation of micro- and nanoobjects, fuelled by both fundamental physics questions and technological applications. Due to the isolated nature of trapped particles, levitated systems are highly decoupled from the environment, and offer experimental possibilities that are absent in clamped nanomechanical oscillators. In particular, a central question in quantum physics is how the transition between the classical and quantum world materializes, and levitated objects represent a promising avenue to study this intermediate regime. In the last years, most levitation experiments have been restricted to optically trapped silica nanoparticles in vacuum, controlling the particle's position with intensity modulated laser beams. However, the use of optical traps severely constrains the experiments that can be performed, because few particle materials can withstand the optical absorption and resulting heating in vacuum. This completely prevents the use of objects with internal degrees of freedom, which---coupled to mechanical variables---offer a clear path towards the study of quantum phenomena at the macroscale. In this thesis, we address these issues by considering other types of trap and feedback schemes, achieving excellent control on the dynamics of optically active nanoparticles. With stochastic calculus, simulations and experiments, we study the dynamics of trapped particles in different regimes, considering also a hybrid quadrupole-optical trapping scheme. Then, using a Paul trap of our own design, we demonstrate the trapping, interrogation and feedback cooling of a nanodiamond hosting a single NV center in vacuum, a clear candidate to perform quantum physics experiments at the single spin level. Finally, we discuss and implement an optimal controller to cool the center of mass motion of an optically levitated nanoparticle. The feedback is realized by exerting a Coulomb force on a charged particle with a pair of electrodes, and thus requires no optics. La levitodinàmica és un camp de la física en ràpida expansió que estudia la levitació i manipulació de micro- i nano-objectes, empesa per la possibilitat de solucionar trencaclosques de física fonamental i de desenvolupar noves aplicacions tecnològiques. Gràcies al gran aïllament de les partícules en levitació, l’evolució dels sistemes levitodinàmics està molt desacoplada del seu entorn. Per consegüent, permeten fer experiments que no serien possibles en nanooscil·ladors mecànics sobre substrat. En particular, una qüestió central en física consisteix en entendre com es produeix la transició entre els mons clàssic i quàntic; els objectes en levitació permeten estudiar aquest règim intermedi de manera innovadora. En els últims anys, la majoria d’experiments de levitodinàmica s’han limitat a atrapar òpticament partícules de sílice en el buit, tot controlant la posició de la partícula amb feixos làser modulats. Tot i així, l’ús de trampes òptiques suposa un obstacle a l’hora d’exportar aquests experiments a règims més diversos perquè, a baixes pressions, pocs materials són capaços de suportar les altes temperatures resultants de l’absorció de llum làser. Això impedeix l’ús d’objectes amb graus de llibertat interns, que –acoplats a variables mecàniques– suposen un full de ruta clar per estudiar fenòmens quàntics a escala macroscòpica En aquesta tesi, adrecem aquestes qüestions tot considerant altres tipus de trampa i tècniques de feedback, i assolim un control excel·lent de la dinàmica de nanopartícules òpticament actives en levitació. Mitjançant càlcul estocàstic, simulacions i experiments, estudiem la dinàmica de les partícules en règims diversos, àdhuc considerant un esquema híbrid de trampa de Paul-òptica. A continuació, utilitzant una trampa de Paul, demostrem experimentalment l’atrapament, interrogació i feedback-cooling en el buit d’un nanodiamant que conté un únic NV− center, un clar candidat per a la realització d’experiments de física quàntica amb un únic spin. Finalment, estudiem i implementem un controlador òptim per a refredar el centre de massa d’una partícula òpticament levitada. El feedback es realitza exercint una força de Coulomb sobre una partícula carregada positivament mitjançant un parell d’elèctrodes, i per tant no requereix elements òptics
Nanoparticles levitated in high vacuum are isolated from the surrounding environment and thus can be used in various applications, including quantum physics research. We demonstrated optical levitation of a nanoparticle, which was trapped without cooling at a pressure of 4.5 × 10 −3 Pa, using a single aspheric lens with a large numerical aperture (= 0.9) and 1030-nm laser. We also activated parametric feedback cooling to trap the particle at a pressure of 5.8 × 10 −4 Pa. This experimental system will be useful for studying nanoparticles in ultrahigh vacuum and for building a mixed system with laser-cooled atoms.