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arXiv:2607.07812

Bogolyubov excitons as a microscopic origin of two-level systems

Andrey Grankin, Victor M. Galitski

Published Jul 8, 2026• 0 citations
arXivHTMLPDF

Abstract

Two-level systems (TLS) are a leading source of decoherence and dielectric loss in Josephson-junction qubits, yet their microscopic origin remains unresolved. We propose an intrinsic, purely electronic TLS candidate: subgap bound states of Bogolyubov quasiparticles. We show that, in a model of a conventional superconductor with electron-electron attraction in the $s$-wave channel and repulsion in higher-angular-momentum channels, the latter produce an effective attraction between Bogolyubov quasiparticles, forming bound states. These Bogolyubov excitons resemble Bardasis--Schrieffer excitons but are driven by repulsive interactions. Bulk Bogolyubov excitons are not easily detectable through single-particle tunneling or other conventional probes, but we show that surface excitons couple to an external electric field and behave as two-level systems. We examine an idealized model of a bulk superconductor proximity-coupled to a two-dimensional repulsive metal, which could represent an external metallic or semiconductor layer or an underscreened region of the superconductor. The two levels correspond to the absence and presence of a single exciton, which carries an electric dipole moment and exhibits an avoided crossing with a resonator, as observed for TLS. Because this mechanism requires no defects and cannot be eliminated by screening or annealing, it suggests that TLS-like excitations may be intrinsic to superconductors.

DOI
10.48550/arxiv.2607.07812

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Two-level systems (TLS) are a leading source of decoherence and dielectric loss in Josephson-junction qubits, yet their microscopic origin remains unresolved. We propose an intrinsic, purely electronic TLS candidate: subgap bound states of Bogolyubov quasiparticles. We show that, in a model of a conventional superconductor with electron-electron attraction in the sss-wave channel and repulsion in higher-angular-momentum channels, the latter produce an effective attraction between Bogolyubov quasiparticles, forming bound states. These Bogolyubov excitons resemble Bardasis--Schrieffer excitons but are driven by repulsive interactions. Bulk Bogolyubov excitons are not easily detectable through single-particle tunneling or other conventional probes, but we show that surface excitons couple to an external electric field and behave as two-level systems. We examine an idealized model of a bulk superconductor proximity-coupled to a two-dimensional repulsive metal, which could represent an external metallic or semiconductor layer or an underscreened region of the superconductor. The two levels correspond to the absence and presence of a single exciton, which carries an electric dipole moment and exhibits an avoided crossing with a resonator, as observed for TLS. Because this mechanism requires no defects and cannot be eliminated by screening or annealing, it suggests that TLS-like excitations may be intrinsic to superconductors.
Abstract The anomalous low-temperature properties of glasses arise from intrinsic excitable entities, so-called tunneling Two-Level-Systems (TLS), whose microscopic nature has been baffling solid-state physicists for decades. TLS have become particularly important for micro-fabricated quantum devices such as superconducting qubits, where they are a major source of decoherence. Here, we present a method to characterize individual TLS in virtually arbitrary materials deposited as thin films. The material is used as the dielectric in a capacitor that shunts the Josephson junction of a superconducting qubit. In such a hybrid quantum system the qubit serves as an interface to detect and control individual TLS. We demonstrate spectroscopic measurements of TLS resonances, evaluate their coupling to applied strain and DC-electric fields, and find evidence of strong interaction between coherent TLS in the sample material. Our approach opens avenues for quantum material spectroscopy to investigate the structure of tunneling defects and to develop low-loss dielectrics that are urgently required for the advancement of superconducting quantum computers.
The sensitivity of superconducting qubits allows for spectroscopy and coherence measurements on individual two-level systems present in the disordered tunnel barrier of an Al/AlOx\mathrm{Al}/{\mathrm{AlO}}_{x}Al/AlOx​/Al Josephson junction. We report experimental evidence for the decoherence of two-level systems by Bogoliubov quasiparticles leaking into the insulating AlOx{\mathrm{AlO}}_{x}AlOx​ barrier. We control the density of quasiparticles in the junction electrodes either by the sample temperature or by injecting them using an on-chip dc superconducting quantum interference device driven to its resistive state. The decoherence rates were measured by observing the two-level system's quantum state evolving under application of resonant microwave pulses and were found to increase linearly with quasiparticle density, in agreement with theory. This interaction with electronic states provides a noise and decoherence mechanism that is relevant for various microfabricated devices such as qubits, single-electron transistors, and field-effect transistors. The presented experiments also offer a possibility to determine the location of the probed two-level systems across the tunnel barrier, providing clues about the fabrication step in which they emerge.
We propose a microscopic model of critical current noise in Josephson junctions based on individual trapping centers in the tunnel-barrier hybridized with electrons in the superconducting leads. We calculate the noise exactly in the limit of no on-site Coulomb repulsion. Our result reveals a noise spectrum that is dramatically different from the usual Lorentzian assumed in simple models. We show that the noise is dominated by sharp subgap resonances associated to the formation of pairs of Andreev bound states, thus providing a possible explanation for the spurious two-level systems (microresonators) observed in Josephson-junction qubits [R. W. Simmonds et al., Phys. Rev. Lett. 93, 077003 (2004).]. Another implication of our model is that each trapping center will contribute a sharp dielectric resonance only in the superconducting phase, providing an effective way to validate our results experimentally. We derive an effective Hamiltonian for a qubit interacting with Andreev bound states, establishing a direct connection between phenomenological models and the microscopic parameters of a Fermionic bath.
Controlling the states of quantum systems is a subject of major interest for both fundamental science and technological development. In this thesis, we carry out theoretical studies on how this can be achieved using light, both of classical and of quantum mechanical nature. We study a driven cavity system, where the driving field is classical and the cavity field is quantum mechanical. We demonstrate how virtual scattering of driving photons inside the cavity via two-photon processes can induce controllable long-range electron interactions in two-dimensional materials. We show that both the strength and the sign of the interactions can be tuned by the driving parameters and that the interactions are not screened effectively except at very low frequencies. For realistic cavity parameters, driving-induced heating of the electrons by inelastic photon scattering is suppressed and coherent electron interactions dominate. When the interactions are attractive, they cause an instability in the Cooper channel at a temperature proportional to the square root of the driving intensity. Our results open up a new avenue for engineering quantum materials on-demand and the possibility of studying the effect of long-range interactions in condensed matter systems. Following that, we take a more general approach to investigate the effect of long-range density-density electron attractive interactions on a superconductor. We show that the low-lying excitations of a 2D conventional superconductor can be significantly altered by these long-range interactions. Using BCS theory, we find that these interactions combine non-linearly with the intrinsic local attractions of the superconductor to increase the Bogoliubov quasiparticle excitation energies, thus enlarging the superconducting gap. Moreover, we show how the long-range nature of the driven-cavity-induced attractions qualitatively changes the collective excitations of the superconductor. Specifically, they lead to the appearance of additional collective excitations of the excitonic modes. They further push the Higgs mode "in gap": it lies below the Bogoliubov quasiparticle continuum such that it cannot decay through the quasiparticle excitations.
We theoretically study superconducting islands based on semiconductor-nanowire Josephson junctions and take into account the presence of subgap quasiparticle excitations in the spectrum of the junction. Our method extends the standard model Hamiltonian for a superconducting charge qubit and replaces the Josephson potential by the Bogoliubov--de Gennes Hamiltonian of the nanowire junction, projected onto the relevant low-energy subgap subspace. This allows us to fully incorporate the coherent dynamics of subgap levels in the junction. The combined effect of spin-orbit coupling and Zeeman energy in the nanowires forming the junction triggers a topological transition, where the subgap levels evolve from finite-energy Andreev bound states into near-zero-energy Majorana bound states. The interplay between the microscopic energy scales governing the nanowire junction (the Josephson energy, the Majorana coupling, and the Majorana energy splitting), with the charging energy of the superconducting island, gives rise to a great variety of physical regimes. Based on this interplay of different energy scales, we fully characterize the microwave response of the junction, from the Cooper pair box to the transmon regimes, and show how the presence of Majoranas can be detected through distinct spectroscopic features. In split-junction geometries, the plasma mode couples to the phase-dispersing subgap levels resulting from Majorana hybridization via a Jaynes--Cummings-like interaction. As a consequence of this interaction, higher order plasma excitations in the junction inherit Majorana properties, including the $4\ensuremath{\pi}$ effect.
By performing experiments with thin-film resonators of NbSi, we elucidate a decoherence mechanism at work in disordered superconductors. This decoherence is caused by charged Two Level Systems (TLS) which couple to the conduction electrons in the BCS ground state; it does not involve any out-of-equilibrium quasiparticles, vortices, etc. Standard theories of mesoscopic disordered conductors enable making predictions regarding this mechanism, notably that decoherence should increase as the superconductor cross section decreases. Given the omnipresence of charged TLS in solid-state systems, this decoherence mechanism affects, to some degree, all experiments involving disordered superconductors. In particular, we show it easily explains the poor coherence observed in quantum phase slip experiments and may contribute to lowering the quality factors in some disordered superconductor resonators.