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arXiv:2606.24939 · Physical Review A

Bright-state source cancellation in dissipative shortcut Raman atom optics

Asad Ali, Saif Al-Kuwari, M. I. Hussain, H. Kuniyil, M. T. Rahim, Saeed Haddadi

quant-phphysics.atom-phphysics.opticsSubmitted Jun 22, 2026• Announced Jun 24, 2026• 0 citations
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Abstract

Spontaneous Raman scattering limits shortcut-assisted atom optics, but its microscopic origin is obscured once the lossy excited state is adiabatically eliminated. We organize the problem around a single quantity: in the instantaneous dark-bright basis the lower-manifold optical source is carried entirely by the bright-state amplitude, $S=Ωb$, so that primary spontaneous scattering reduces to the compact functional. This recovers the known dissipative-STIRAP loss in transparent form and makes the action of a shortcut explicit: ideal counterdiabatic STIRSAP cancels the bright-state \emph{source}, not the optical decay coefficient. We show this cancellation is exact in the full three-level model at the counterdiabatic point, for arbitrary one-photon detuning, Rabi frequency, and pulse duration. The residual source splits into orthogonal quadratures -- shortcut mismatch (real) and two-photon Doppler detuning (imaginary) -- which invites a velocity-selective protocol that nulls the Doppler quadrature for a chosen momentum class with a second, phase-shifted lower-state field. Our central result is that this source nulling is never superior to simply chirping the two-photon detuning: the two coincide only when the selected class $δ_c$ is small compared with the bright-state gap, and the nulling degrades and then fails as $δ_c\to|μ|$ -- precisely the regime of launched or warm clouds and high-order large-momentum-transfer (LMT) optics that motivates velocity selection. The controlling quantity is the magnitude of the residual Hamiltonian perturbation a scheme leaves behind, not the residual source it cancels. As a complement to existing multi-pulse decay budgets, we cast a single-pulse mode-error budget for LMT interferometry entirely in terms of the bright-state source, and delineate when shortcut-assisted Raman control reduces the total scattering cost.

Comments
12 pages, 4 figures

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Spontaneous Raman scattering limits shortcut-assisted atom optics, but its microscopic origin is obscured once the lossy excited state is adiabatically eliminated. We organize the problem around a single quantity: in the instantaneous dark-bright basis the lower-manifold optical source is carried entirely by the bright-state amplitude, S=ΩbS=ΩbS=Ωb, so that primary spontaneous scattering reduces to the compact functional. This recovers the known dissipative-STIRAP loss in transparent form and makes the action of a shortcut explicit: ideal counterdiabatic STIRSAP cancels the bright-state \emph{source}, not the optical decay coefficient. We show this cancellation is exact in the full three-level model at the counterdiabatic point, for arbitrary one-photon detuning, Rabi frequency, and pulse duration. The residual source splits into orthogonal quadratures -- shortcut mismatch (real) and two-photon Doppler detuning (imaginary) -- which invites a velocity-selective protocol that nulls the Doppler quadrature for a chosen momentum class with a second, phase-shifted lower-state field. Our central result is that this source nulling is never superior to simply chirping the two-photon detuning: the two coincide only when the selected class δcδ_cδc​ is small compared with the bright-state gap, and the nulling degrades and then fails as δc→∣μ∣δ_c\to|μ|δc​→∣μ∣ -- precisely the regime of launched or warm clouds and high-order large-momentum-transfer (LMT) optics that motivates velocity selection. The controlling quantity is the magnitude of the residual Hamiltonian perturbation a scheme leaves behind, not the residual source it cancels. As a complement to existing multi-pulse decay budgets, we cast a single-pulse mode-error budget for LMT interferometry entirely in terms of the bright-state source, and delineate when shortcut-assisted Raman control reduces the total scattering cost.
Large-momentum-transfer (LMT) atom interferometry provides a route toward enhanced inertial sensitivity in compact quantum sensors, but its scalability is limited by the accumulation of pulse-transfer errors across long Raman pulse sequences. We investigate theoretically the use of stimulated Raman shortcut-to-adiabatic passage (STIRSAP) for high-fidelity LMT atom optics in a Mach--Zehnder interferometer geometry. The counterdiabatic correction is encoded directly into the Raman pulse envelopes, eliminating the need for auxiliary microwave or radio-frequency control fields. Numerical simulations based on an effective Raman model show that 1 μs1~μ\mathrm{s}1 μs STIRSAP pulses achieve single-pulse transfer fidelities of Fπ=0.99902F_π= 0.99902Fπ​=0.99902 while maintaining negligible pulse-time overhead even at high momentum order. We analyze the resulting tradeoff between interferometric phase enhancement and compound contrast decay and identify an unconstrained shot-noise optimum near n≈270n\approx270n≈270. The analysis further shows that practical operation at extreme LMT order is constrained by wave-packet separation, vibration noise, Doppler detuning, and accumulated systematic effects rather than by pulse duration itself. These results establish superadiabatic Raman control as a promising approach for scalable high-fidelity atom optics and clarify the physical limitations governing compact high-order atom interferometers.
Multistate stimulated Raman adiabatic passage (STIRAP) is a process which allows for adiabatic population transfer between the two ends of a chainwise-connected quantum system. The process requires large temporal areas of the driving pulsed fields (pump and Stokes) in order to suppress the nonadiabatic couplings and thereby to make adiabatic evolution possible. To this end, in the present paper a variation of multistate STIRAP, which accelerates and improves the population transfer, is presented. In addition to the usual pump and Stokes fields it uses shortcut fields applied between the states, which form the dark state of the system. The shortcuts cancel the couplings between the dark state and the other adiabatic states thereby resulting (in the ideal case) in a unit transition probability between the two end states of the chain. Specific examples of five-state systems formed of the magnetic sublevels of the transitions between two degenerate levels with angular momenta Jg=2{J}_{g}=2Jg​=2 (of ground or lower level) and Je=1{J}_{e}=1Je​=1 or Je=2{J}_{e}=2Je​=2 (of excited or upper level) are considered in detail, for which the shortcut fields are derived analytically. The proposed method is simpler than the usual ``shortcuts to adiabaticity'' recipe, which prescribes shortcut fields between all states of the system, while the present proposal uses shortcut fields between the sublevels forming the dark state only. The results are of potential interest in applications where high-fidelity quantum control is essential, e.g., quantum information, atom optics, formation of ultracold molecules, cavity QED, etc.
We investigate collective chirped stimulated Raman adiabatic passage (STIRAP) in a pair of identical three-level atoms using a symmetric six-state model. Numerical simulations reveal a pronounced oscillatory dependence of the population transfer to the doubly excited Rydberg state on the peak Rabi frequency, indicating dynamics beyond the conventional single-dark-state description of STIRAP. To identify the underlying mechanism, we develop a dressed-manifold description based on gauge-invariant projections onto nearly degenerate instantaneous dressed manifolds. The analysis demonstrates that the wavefunction remains predominantly confined to a two-dimensional dark manifold while becoming transiently coupled to a neighboring bright manifold during the pulse-overlap interval. We further show that in the dressed-manifold representation, the Rydberg-Rydberg interaction modifies the collective resonance structure while preserving the dark-bright manifold dynamics responsible for the oscillatory transfer; an appropriately chosen frequency chirp compensates the interaction-induced detuning and restores efficient population transfer. This dressed-manifold picture provides a consistent interpretation of oscillatory collective transfer and establishes a framework for controlling adiabatic dynamics in interacting multilevel systems by linearly chirped STIRAP, opening a route toward manifold-based control of Rydberg-mediated quantum gates, correlated-state preparation, and other coherent operations in interacting atomic systems.
Despite the fact that atom interferometry has been a successful application of quantum sensing, a major topic of interest is the further improvement of the sensitivity of these devices. In particular, the area enclosed by the interferometer (which controls the sensitivity) can be increased by providing a larger momentum kick to the atom cloud, increasing the extent of the momentum axis. One such atom optics technique involves increasing the number of central π−π-π−Raman pulses. This technique, while providing the prerequisite additional momentum boost, also causes the atom to remain in the intermediate high energy state for longer periods of time. This additional length of time is often neglected in many treatments due to the adiabatic elimination of the higher energy state enabled by the large optical detuning. The increased time in the intermediate high energy state results in a higher probability of undesired spontaneous decay and a loss of quantum information, thereby adding error to the atom interferometer. In this work, we consider an open quantum system using the Lindblad master equation to devise a model for the atomic state dynamics that includes the undesired spontaneous decay from the intermediate high energy state. We formulate an error figure of merit to analyze limitations of an atom interferometer configured for acceleration measurements. Our theoretical results show the error figure of merit will be dominated by a NR−2N_{R}^{-2}NR−2​ scaling factor for low numbers of π−π-π−Raman pulses, but will be dominated by a monotonic increase in error for high number of π−π-π−Raman pulses. We determined the number of πππ-Raman pulses that accomplishes maximal momentum transfer with a the minimal error, depending on major system parameters.
The technique of stimulated Raman shortcut to adiabatic passage (STIRSAP) is implemented to chainwise and N-pod systems. In chainwise systems, for large detuning conditions, the population of the middle states can be suppressed during the time evolution of the system and therefore, the Hamiltonian of an N-state system is reduced to an effective two-level system, using adiabatic elimination technique. Applying the STIRSAP method in two-level systems, the modified Rabi frequencies for fast population transfer are achieved. For N + 1-pod systems, assuming that N Stokes pulses have the same time dependence, we reduce the Hamiltonian of the original system to a three-state system. For both resonance and detuning conditions, we can reduce the three-state Hamiltonian to an effective two-state one. Using the STIRSAP technique, robust population transfer can be achieved from an initial ground state to an arbitrary coherent superposition of all ground states.
We propose a pulse-shaping method for improving population transfer in multistate stimulated Raman adiabatic passage (STIRAP) with nearest-neighbour couplings only. The method extends the quasiparallel-eigenenergy approach, previously used for two- and three-state systems, to multistate chains without introducing additional shortcut fields. The pump and Stokes fields are shaped so that the eigenenergies closest to the dark state remain nearly parallel to it during the central part of the interaction, where nonadiabatic transitions are most likely to occur. We derive analytic prescriptions for the required pulse shapes and apply them to five-, seven-, and nine-state chains formed by magnetic sublevels of degenerate manifolds with angular momenta Jg→Je=JgJ_g\rightarrow J_e=J_gJg​→Je​=Jg​ and Jg→Je=Jg−1J_g\rightarrow J_e=J_g-1Jg​→Je​=Jg​−1 driven by a pair of right- and left-circularly polarized pulses. Numerical simulations show that the optimized pulses can reduce the population transfer error by several orders of magnitude compared to standard Gaussian pulses. The same shapes also improve robustness against variations of the peak Rabi frequency, the single-photon detuning, and the multiphoton detuning. The comparison between the two angular-momentum families shows that the Jg→JgJ_g\rightarrow J_gJg​→Jg​ chains are generally more favourable, because their Clebsch-Gordan coefficients keep the relevant bright-state gap larger in the region where the dark state changes most rapidly. Finally, simulations with spontaneous emission show that the optimized resonant pulses remain advantageous in the lossy regime as well.