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arXiv:2004.08341 · Physical Review A

High-fidelity multistate stimulated Raman adiabatic passage assisted by shortcut fields

Nikolay V. Vitanov

Published Aug 10, 2020• 24 citations
arXivHTMLPDF

Abstract

Multistate stimulated Raman adiabatic passage (STIRAP) is a process which allows for adiabatic population transfer between the two ends of a chainwise-connected quantum system. The process requires large temporal areas of the driving pulsed fields (pump and Stokes) in order to suppress the nonadiabatic couplings and thereby to make adiabatic evolution possible. To this end, in the present paper a variation of multistate STIRAP, which accelerates and improves the population transfer, is presented. In addition to the usual pump and Stokes fields it uses shortcut fields applied between the states, which form the dark state of the system. The shortcuts cancel the couplings between the dark state and the other adiabatic states thereby resulting (in the ideal case) in a unit transition probability between the two end states of the chain. Specific examples of five-state systems formed of the magnetic sublevels of the transitions between two degenerate levels with angular momenta ${J}_{g}=2$ (of ground or lower level) and ${J}_{e}=1$ or ${J}_{e}=2$ (of excited or upper level) are considered in detail, for which the shortcut fields are derived analytically. The proposed method is simpler than the usual ``shortcuts to adiabaticity'' recipe, which prescribes shortcut fields between all states of the system, while the present proposal uses shortcut fields between the sublevels forming the dark state only. The results are of potential interest in applications where high-fidelity quantum control is essential, e.g., quantum information, atom optics, formation of ultracold molecules, cavity QED, etc.

DOI
10.1103/physreva.102.023515

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Multistate stimulated Raman adiabatic passage (STIRAP) is a process which allows for adiabatic population transfer between the two ends of a chainwise-connected quantum system. The process requires large temporal areas of the driving pulsed fields (pump and Stokes) in order to suppress the nonadiabatic couplings and thereby to make adiabatic evolution possible. To this end, in the present paper a variation of multistate STIRAP, which accelerates and improves the population transfer, is presented. In addition to the usual pump and Stokes fields it uses shortcut fields applied between the states, which form the dark state of the system. The shortcuts cancel the couplings between the dark state and the other adiabatic states thereby resulting (in the ideal case) in a unit transition probability between the two end states of the chain. Specific examples of five-state systems formed of the magnetic sublevels of the transitions between two degenerate levels with angular momenta Jg=2{J}_{g}=2Jg​=2 (of ground or lower level) and Je=1{J}_{e}=1Je​=1 or Je=2{J}_{e}=2Je​=2 (of excited or upper level) are considered in detail, for which the shortcut fields are derived analytically. The proposed method is simpler than the usual ``shortcuts to adiabaticity'' recipe, which prescribes shortcut fields between all states of the system, while the present proposal uses shortcut fields between the sublevels forming the dark state only. The results are of potential interest in applications where high-fidelity quantum control is essential, e.g., quantum information, atom optics, formation of ultracold molecules, cavity QED, etc.
We propose a pulse-shaping method for improving population transfer in multistate stimulated Raman adiabatic passage (STIRAP) with nearest-neighbour couplings only. The method extends the quasiparallel-eigenenergy approach, previously used for two- and three-state systems, to multistate chains without introducing additional shortcut fields. The pump and Stokes fields are shaped so that the eigenenergies closest to the dark state remain nearly parallel to it during the central part of the interaction, where nonadiabatic transitions are most likely to occur. We derive analytic prescriptions for the required pulse shapes and apply them to five-, seven-, and nine-state chains formed by magnetic sublevels of degenerate manifolds with angular momenta Jg→Je=JgJ_g\rightarrow J_e=J_gJg​→Je​=Jg​ and Jg→Je=Jg−1J_g\rightarrow J_e=J_g-1Jg​→Je​=Jg​−1 driven by a pair of right- and left-circularly polarized pulses. Numerical simulations show that the optimized pulses can reduce the population transfer error by several orders of magnitude compared to standard Gaussian pulses. The same shapes also improve robustness against variations of the peak Rabi frequency, the single-photon detuning, and the multiphoton detuning. The comparison between the two angular-momentum families shows that the Jg→JgJ_g\rightarrow J_gJg​→Jg​ chains are generally more favourable, because their Clebsch-Gordan coefficients keep the relevant bright-state gap larger in the region where the dark state changes most rapidly. Finally, simulations with spontaneous emission show that the optimized resonant pulses remain advantageous in the lossy regime as well.
Abstract The multistate stimulated Raman adiabatic passage (STIRAP) is an efficient technique to achieve a selective and accurate population transfer in a chainwise-linked system. However, their efficiency is imperfect due to the nonadiabatic losses from the long runtime of the adiabatic evolution. Here, we focus on realizing a perfect and robust coherent control of the quantum states with optimal shortcut to adiabaticity in a realistic five-state hybrid quantum system. In particular, the optimal shortcut field requires minimal additional coupling (only one coupling strength) to accelerate the adiabatic evolution in this five-state system. Compared to the original STIRAP, the optimal shortcut shows the ultra-high fidelity of quantum state manipulations even though the control parameters of the Hamiltonians are changed in different ways. Furthermore, we study the efficiency of the optimal shortcut field technique in the presence of various experimental errors, such as systematic error, Rabi frequency error, and coupling strength error, and it features a broad range of high efficiencies above 99.9%, showing its robustness against the above errors. The results might shed insight on the further applications of shortcuts to adiabaticity on robust quantum information processing in multi-level quantum systems.
The technique of stimulated Raman adiabatic passage (STIRAP) is a highly efficient tool for coherent population transfer in a chainwise-connected three-state quantum system. It is widely accepted that the two-photon resonance between the two end states of the chain is a crucial condition for STIRAP. This assumption is indeed correct when the two driving fields, pump and Stokes, produce nearly equal couplings for their respective transitions. We show analytically, supported by numeric examples, that when the pump and Stokes couplings differ significantly, the two-photon population transfer profile is distorted and its center is shifted away from the two-photon resonance; hence, the optimal operation of STIRAP demands a two-photon detuning. We derive simple analytic estimates for the center and the width of the two-photon profile. The results are of potential importance in situations when the pump and Stokes fields are of different physical natures (e.g., laser and cavity fields) or when two-photon resonance is unwanted (e.g., in the presence of residual light).
The technique of stimulated Raman adiabatic passage (STIRAP) is an efficient and robust technique for population transfer in three-state chain-wise connected quantum systems, 1-2-3. Here we analyze the transition time in STIRAP, that is the time it takes for the population to be transferred from state 1 to state 3. We derive a very simple formula for this transition time, which shows that it is inversely proportional to the nonadiabatic coupling $\mathrm{\ensuremath{\vartheta}\ifmmode \dot{}\else \.{}\fi{}}({t}_{c})$, estimated at the time tc{t}_{c}tc​ when the pump and Stokes couplings have the same value. Explicit formulas for several pulse shapes of the pump and Stokes fields are derived. Contrary to the naive expectation that the transition time might be proportional to the delay between the pump and Stokes pulses, or to the width of their overlap region, we find that the transition time is inversely proportional to the delay, i.e., larger delays produce faster transitions. We also calculate the transition time in two important variations of the STIRAP technique---bright-STIRAP and STIRAP in multistate systems---where similar features are found.
Abstract Robust quantum control is essential for the development of quantum computers, which rely on precise manipulation of qubits. One form of quantum control is stimulated Raman adiabatic passage (STIRAP), which ordinarily is a state transfer protocol but was extended by Kis and Renzoni (2002 Phys. Rev. A 65 032318) to perform qubit rotations. Shortcut methods to adiabaticity for STIRAP have been shown to speed up adiabatic processes, beyond the adiabatic criterion, with high fidelity. Here, we apply shortcut to adiabaticity methods to the STIRAP qubit rotation scheme to improve the performance of quantum logic gates. The scheme can be implemented via direct connections between ground states in a 4-level Λ system or effective connections in a 5-level Λ system with modified pulses that implement transitionless quantum driving via the addition of a counterdiabatic driving term. We show that the extended shortcut to adiabaticity method serves to improve the fidelity of qubit rotations in the diabatic regime.
The technique of stimulated Raman shortcut to adiabatic passage (STIRSAP) is implemented to chainwise and N-pod systems. In chainwise systems, for large detuning conditions, the population of the middle states can be suppressed during the time evolution of the system and therefore, the Hamiltonian of an N-state system is reduced to an effective two-level system, using adiabatic elimination technique. Applying the STIRSAP method in two-level systems, the modified Rabi frequencies for fast population transfer are achieved. For N + 1-pod systems, assuming that N Stokes pulses have the same time dependence, we reduce the Hamiltonian of the original system to a three-state system. For both resonance and detuning conditions, we can reduce the three-state Hamiltonian to an effective two-state one. Using the STIRSAP technique, robust population transfer can be achieved from an initial ground state to an arbitrary coherent superposition of all ground states.