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Journal of Modern Optics

Stimulated Raman shortcut to adiabatic passage in chainwise and N-pod systems

N. Irani, M. Amniat-Talab, M. Saadati-Niari

Published Oct 22, 2021• 3 citations
Publisher

Abstract

The technique of stimulated Raman shortcut to adiabatic passage (STIRSAP) is implemented to chainwise and N-pod systems. In chainwise systems, for large detuning conditions, the population of the middle states can be suppressed during the time evolution of the system and therefore, the Hamiltonian of an N-state system is reduced to an effective two-level system, using adiabatic elimination technique. Applying the STIRSAP method in two-level systems, the modified Rabi frequencies for fast population transfer are achieved. For N + 1-pod systems, assuming that N Stokes pulses have the same time dependence, we reduce the Hamiltonian of the original system to a three-state system. For both resonance and detuning conditions, we can reduce the three-state Hamiltonian to an effective two-state one. Using the STIRSAP technique, robust population transfer can be achieved from an initial ground state to an arbitrary coherent superposition of all ground states.

DOI
10.1080/09500340.2021.1989512

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The technique of stimulated Raman shortcut to adiabatic passage (STIRSAP) is implemented to chainwise and N-pod systems. In chainwise systems, for large detuning conditions, the population of the middle states can be suppressed during the time evolution of the system and therefore, the Hamiltonian of an N-state system is reduced to an effective two-level system, using adiabatic elimination technique. Applying the STIRSAP method in two-level systems, the modified Rabi frequencies for fast population transfer are achieved. For N + 1-pod systems, assuming that N Stokes pulses have the same time dependence, we reduce the Hamiltonian of the original system to a three-state system. For both resonance and detuning conditions, we can reduce the three-state Hamiltonian to an effective two-state one. Using the STIRSAP technique, robust population transfer can be achieved from an initial ground state to an arbitrary coherent superposition of all ground states.
The stimulated Raman adiabatic passage (STIRAP) shows an efficient technique that accurately transfers population between two discrete quantum states with the same parity, in three-level quantum systems based on adiabatic evolution. This technique has widely theoretical and experimental applications in many fields of physics, chemistry, and beyond. Here, we present a generally robust approach to speed up STIRAP with invariant-based shortcut to adiabaticity. By controlling the dynamical process, we inversely design a family of Hamiltonians that can realize fast and accurate population transfer from the first to the third level, while the systematic error is largely suppressed in general. Furthermore, a detailed trade-off relation between the population of the intermediate state and the amplitudes of Rabi frequencies in the transfer process is illustrated. These results provide an optimal route toward manipulating the evolution of three-level quantum systems in future quantum information processing.
Multistate stimulated Raman adiabatic passage (STIRAP) is a process which allows for adiabatic population transfer between the two ends of a chainwise-connected quantum system. The process requires large temporal areas of the driving pulsed fields (pump and Stokes) in order to suppress the nonadiabatic couplings and thereby to make adiabatic evolution possible. To this end, in the present paper a variation of multistate STIRAP, which accelerates and improves the population transfer, is presented. In addition to the usual pump and Stokes fields it uses shortcut fields applied between the states, which form the dark state of the system. The shortcuts cancel the couplings between the dark state and the other adiabatic states thereby resulting (in the ideal case) in a unit transition probability between the two end states of the chain. Specific examples of five-state systems formed of the magnetic sublevels of the transitions between two degenerate levels with angular momenta Jg=2{J}_{g}=2Jg​=2 (of ground or lower level) and Je=1{J}_{e}=1Je​=1 or Je=2{J}_{e}=2Je​=2 (of excited or upper level) are considered in detail, for which the shortcut fields are derived analytically. The proposed method is simpler than the usual ``shortcuts to adiabaticity'' recipe, which prescribes shortcut fields between all states of the system, while the present proposal uses shortcut fields between the sublevels forming the dark state only. The results are of potential interest in applications where high-fidelity quantum control is essential, e.g., quantum information, atom optics, formation of ultracold molecules, cavity QED, etc.
We study the stimulated Raman adiabatic passage technique in an NNN-pod system driven by NNN pulsed fields when $N\ensuremath{-}2$ and $N\ensuremath{-}1$ pulses not connected to the initial state have the same shape. We show that, for properly timed pulses, robust population transfer from an initial ground state to an arbitrary coherent superposition of the ground states can be achieved in a single step. The case of $N\ensuremath{-}2$ pulses of the same shape involves a geometric phase of the same type as the one appearing in tripod systems.
Chainwise stimulated Raman adiabatic passage (C-STIRAP) in a M-type molecular system is a good alternative in creating ultracold deeply bound molecules when the typical STIRAP in a $\mathrm{\ensuremath{\Lambda}}$-type system does not work due to weak Frank-Condon factors between states. However, its creation efficiency under smooth evolution is generally low. During the process, the population in the intermediate states may decay out quickly and the strong laser pulses may induce multiphoton processes. In this paper, we find that the shortcut to adiabaticity (STA) fits very well in improving the performance of the C-STIRAP. Currently, related discussions on the so-called chainwise stimulated Raman shortcut-to-adiabatic passage (C-STIRSAP) are rare. Here, we investigate this topic under adiabatic elimination. Given a relation among the four incident pulses, it is quite interesting that the M-type system can be generalized into an effective $\mathrm{\ensuremath{\Lambda}}$-type structure with the simplest resonant coupling. Consequently, all possible methods of STA for the three-state system can be borrowed. We take the counterdiabatic driving and ``chosen path'' methods as instances to demonstrate our treatment of the molecular system. Although the chosen path method does not work well in a real three-state system if there is strong decay in the excited state, our C-STIRSAP protocol under both methods can create ultracold deeply bound molecules with high efficiency in the M-type system. The evolution time is shortened without strong laser pulses and the robustness of STA is well preserved. Finally, the detection of ultracold deeply bound molecules is discussed.
The stimulated Raman adiabatic passage shows an efficient technique that accurately transfers population between two discrete quantum states with the same parity in three-level quantum systems based on adiabatic evolution. This technique has widely theoretical and experimental applications in many fields of physics, chemistry, and beyond. Here, we present a general approach to robust stimulated Raman shortcut-to-adiabatic passage with invariant-based optimal control. By controlling the dynamical process, we inversely design a family of Hamiltonians with non-divergent Rabi frequencies that can realize fast and accurate population transfer from the first to the third level, while the systematic errors are largely suppressed in general. Furthermore, a detailed trade-off relation between the population of the intermediate state and the amplitudes of Rabi frequencies in the transfer process is illustrated. These results provide an optimal route toward manipulating the evolution of three-level quantum systems in future quantum information processing.
Shortcuts to adiabaticity in various quantum systems have attracted much attention with their wide applications in quantum information processing and quantum control. In this paper, we concentrate on a stimulated Raman shortcut-to-adiabatic passage in quantum three-level systems. To implement counterdiabatic driving but without additional coupling, we first reduce the quantum three-level systems to effective two-level problems at large intermediate-level detuning, or on resonance, apply counterdiabatic driving along with the unitary transformation and eventually modify the pump and Stokes pulses for achieving fast and high-fidelity population transfer. The required laser intensity and stability against parameter variation are further discussed, to demonstrate the advantage of shortcuts to adiabaticity.