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arXiv:2605.04914 · Photonics

Transit Noise in Spin Squeezing Experiments with Coated Rubidium Vapor Cell

Yujie Ji, Peiying Li, Yanhong Xiao, Yuzhuo Wang, Junlei Duan

quant-phSubmitted May 6, 2026• Announced May 7, 2026• 0 citations
arXivHTMLPDF

Abstract

Spin squeezing can suppress quantum projection noise via interparticle entanglement, therefore enabling measurement sensitivities beyond the standard quantum limit. In practice, however, the Gaussian and finite intensity profiles of the optical probe beam induce spatially inhomogeneous atom-light interactions. As polarized atoms move within a vapor cell, they experience position-dependent optical intensities, generating transit noise that limits spin squeezing performance. Here, we investigate the transit noise in a coated rubidium vapor cell through combined theoretical analysis and experimental measurements. By varying the probe beam diameter, we quantify the dependence of transit noise on beam size and atomic Larmor frequency. Our results show that, for a vapor cell with fixed dimensions, the transit noise increases as the probe beam spot area decreases. Moreover, when the Larmor frequency is below the characteristic linewidth of the transit noise, the noise contribution becomes larger. We further calculated and measured spin squeezing for different beam sizes and found an experimental difference of $2.7 \pm 0.2$ dB between 2~mm and 0.6~mm, similar to the theoretical prediction of $3.0 \pm 0.3$ dB. Theoretical analysis under conditions of stronger squeezing shows that transit noise becomes an even more critical limiting factor. These results provide practical guidance for optimizing probe beam parameters and suppressing transit noise in spin squeezing experiments.

Journal reference
Photonics 2026, 13(5), 456
DOI
10.3390/photonics13050456
Comments
16 pages,7 figures, 3 appendix figures

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Spin squeezing can suppress quantum projection noise via interparticle entanglement, therefore enabling measurement sensitivities beyond the standard quantum limit. In practice, however, the Gaussian and finite intensity profiles of the optical probe beam induce spatially inhomogeneous atom-light interactions. As polarized atoms move within a vapor cell, they experience position-dependent optical intensities, generating transit noise that limits spin squeezing performance. Here, we investigate the transit noise in a coated rubidium vapor cell through combined theoretical analysis and experimental measurements. By varying the probe beam diameter, we quantify the dependence of transit noise on beam size and atomic Larmor frequency. Our results show that, for a vapor cell with fixed dimensions, the transit noise increases as the probe beam spot area decreases. Moreover, when the Larmor frequency is below the characteristic linewidth of the transit noise, the noise contribution becomes larger. We further calculated and measured spin squeezing for different beam sizes and found an experimental difference of 2.7±0.22.7 \pm 0.22.7±0.2 dB between 2mm and 0.6mm, similar to the theoretical prediction of 3.0±0.33.0 \pm 0.33.0±0.3 dB. Theoretical analysis under conditions of stronger squeezing shows that transit noise becomes an even more critical limiting factor. These results provide practical guidance for optimizing probe beam parameters and suppressing transit noise in spin squeezing experiments.
Quantum control of many body atomic spins is often pursued in the context of an atom-light quantum interface, where a quantized light field acts as a "quantum bus" that can be used to entangle distant atoms. One key challenge is to improve the coherence of the atom-light interface and the amount of atom-light entanglement it can generate, given the constraints of working with multilevel atoms and optical fields in a 3D geometry. We have explored new ways to achieve this, through rigorous optimization of the spatial geometry, and through control of the internal atomic state. Our basic setup consists of a quantized probe beam passing through an atom cloud held in a dipole trap, first generating spin-probe entanglement through the Faraday interaction, and then using backaction from a measurement of the probe polarization to squeeze the collective atomic spin. The relevant figure of merit is the metrologically useful spin squeezing determined by the enhancement in the resolution of rotations of the collective spin, relative to the commonly used spin coherent state. With an optimized free-space geometry, and by using a 2-color probe scheme to suppress tensor light shifts, we achieve 3(2) dB of metrologically useful spin squeezing. We can further increase atom-light coupling by implementing internal state control to prepare spin states with larger initial projection noise relative to the spin coherent state. Under the right conditions this increase in projection noise can lead to stronger measurement backaction and increased atom-atom entanglement. With further internal state control the increased atom-atom entanglement can then be mapped to a basis where it corresponds to improved squeezing of, e.g., the physical spin-angular momentum or the collective atomic clock pseudospin. In practice, controlling the collective spin of N ~ 10⁶ atoms in this fashion is an extraordinarily difficult challenge because errors in the control of individual atoms tend to be highly correlated. By employing precise internal state control, we have prepared and detected projection noise limited "cat" states (which have initial projection noise that is larger by a factor of 2f = 8 for Cs relative to the spin coherent state) and estimate that we can generate up to 6.0(5) dB of metrologically useful spin squeezing, demonstrating the advantage of using the internal atomic structure as a resource for ensemble control.
We measured the spin noise spectroscopy (SNS) of rubidium atomic ensemble with two different kinds of atomic vapor cells (filled with buffer gas or coated with paraffin film on the inner wall) and demonstrated the enhancement of the signal-to-noise ratio (SNR) by using polarization squeezed state (PSS) of 795-nm light field with Stokes operator S Λ 2 squeezed. The PSS is prepared by locking the relative phase between the squeezed vacuum state of light obtained with a sub-threshold optical parametric oscillator and the orthogonally polarized local oscillator beam by means of the quantum noise lock. Under the same conditions, the PSS can be employed not only to improve the SNR, but also to keep the full width at half maximum (FWHM) of SNS, compared with the case of using the polarization coherent state (PCS), enhancement of SNR is positively correlated with the squeezing level of the PSS. With increasing probe laser power and atomic number density, the SNR and FWHM of SNS will increase correspondingly. With the help of the PSS of the Stokes operator S Λ 2 , quantum improvements of both the SNR and FWHM of SNS signal has been demonstrated by controlling optical power of polarization squeezed light beam or atomic number density in our experiments.
High precision optical detection is fundamentally limited by quantum noise. This limit can be bypassed with the use of squeezed states of light with modified quantum noise. We study squeezed states of light with a focus on optimization of squeezing generated via polarization self-rotation (PSR) in hot rubidium vapor. The goal of our research is to reduce quantum noise by optimizing cell temperature and beam shape of the input pump field. We find that computerized spatial optimization algorithms (combined with manual optimization of temperature and laser detuning) are successful in improving squeezing levels, with one spatial mask yielding over 1.0 dB of squeezing improvement under certain conditions. We have achieved quantum noise suppression of 2.3 ± 0.1 dB below shot noise.
We report the measurement of the intensity difference squeezing via the non-degenerate four-wave mixing process in a rubidium atomic vapor medium. Two pairs of balanced detection systems are employed to measure the probe and the conjugate beams, respectively. It is convenient to get the quantum shot noise limit, the squeezed and the amplified noise power spectra. We also investigate the influence of the input extra quadrature amplitude noise of the probe beam. The influence of the extra noise can be minimized and the squeezing can be optimized under the proper parameter condition. We measure the −3.7-dB intensity difference squeezing when the probe beam has a 3-dB extra quadrature amplitude noise. This result is slightly smaller than −4.1 dB when the ideal coherent light (no extra noise) for the probe beam is used.
We study the fundamental limits of noise spectroscopy using estimation theory, Faraday rotation probing of an atomic spin system, and squeezed light. We find a simple and general expression for the Fisher information, which quantifies the sensitivity to spectral parameters such as resonance frequency and linewidth. For optically detected spin noise spectroscopy, we find that shot noise imposes ``local'' standard quantum limits for any given probe power and atom number, and also ``global'' standard quantum limits when the probe power and atom number are taken as free parameters. We confirm these estimation theory results using nondestructive Faraday rotation probing of hot Rb vapor, observing the predicted optima, and finding good quantitative agreement with a first-principles calculation of the spin noise spectra. Finally, we show sensitivity beyond the atom- and photon-number-optimized global standard quantum limit using squeezed light.
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