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arXiv:2111.09572 · Optics Express

Enhancement of spin noise spectroscopy of rubidium atomic ensemble by using the polarization squeezed light

Lele Bai, Lulu Zhang, Yongbiao Yang, Rui Chang, Yao Qin, Jun He, Xin Wen, Junmin Wang

Published Dec 24, 2021• 12 citations
arXivHTMLPDF

Abstract

We measured the spin noise spectroscopy (SNS) of rubidium atomic ensemble with two different kinds of atomic vapor cells (filled with buffer gas or coated with paraffin film on the inner wall) and demonstrated the enhancement of the signal-to-noise ratio (SNR) by using polarization squeezed state (PSS) of 795-nm light field with Stokes operator S Λ 2 squeezed. The PSS is prepared by locking the relative phase between the squeezed vacuum state of light obtained with a sub-threshold optical parametric oscillator and the orthogonally polarized local oscillator beam by means of the quantum noise lock. Under the same conditions, the PSS can be employed not only to improve the SNR, but also to keep the full width at half maximum (FWHM) of SNS, compared with the case of using the polarization coherent state (PCS), enhancement of SNR is positively correlated with the squeezing level of the PSS. With increasing probe laser power and atomic number density, the SNR and FWHM of SNS will increase correspondingly. With the help of the PSS of the Stokes operator S Λ 2 , quantum improvements of both the SNR and FWHM of SNS signal has been demonstrated by controlling optical power of polarization squeezed light beam or atomic number density in our experiments.

DOI
10.1364/oe.448084

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Spin squeezing can suppress quantum projection noise via interparticle entanglement, therefore enabling measurement sensitivities beyond the standard quantum limit. In practice, however, the Gaussian and finite intensity profiles of the optical probe beam induce spatially inhomogeneous atom-light interactions. As polarized atoms move within a vapor cell, they experience position-dependent optical intensities, generating transit noise that limits spin squeezing performance. Here, we investigate the transit noise in a coated rubidium vapor cell through combined theoretical analysis and experimental measurements. By varying the probe beam diameter, we quantify the dependence of transit noise on beam size and atomic Larmor frequency. Our results show that, for a vapor cell with fixed dimensions, the transit noise increases as the probe beam spot area decreases. Moreover, when the Larmor frequency is below the characteristic linewidth of the transit noise, the noise contribution becomes larger. We further calculated and measured spin squeezing for different beam sizes and found an experimental difference of $2.7 \pm 0.2$ dB between 2~mm and 0.6~mm, similar to the theoretical prediction of $3.0 \pm 0.3$ dB. Theoretical analysis under conditions of stronger squeezing shows that transit noise becomes an even more critical limiting factor. These results provide practical guidance for optimizing probe beam parameters and suppressing transit noise in spin squeezing experiments.

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We measured the spin noise spectroscopy (SNS) of rubidium atomic ensemble with two different kinds of atomic vapor cells (filled with buffer gas or coated with paraffin film on the inner wall) and demonstrated the enhancement of the signal-to-noise ratio (SNR) by using polarization squeezed state (PSS) of 795-nm light field with Stokes operator S Λ 2 squeezed. The PSS is prepared by locking the relative phase between the squeezed vacuum state of light obtained with a sub-threshold optical parametric oscillator and the orthogonally polarized local oscillator beam by means of the quantum noise lock. Under the same conditions, the PSS can be employed not only to improve the SNR, but also to keep the full width at half maximum (FWHM) of SNS, compared with the case of using the polarization coherent state (PCS), enhancement of SNR is positively correlated with the squeezing level of the PSS. With increasing probe laser power and atomic number density, the SNR and FWHM of SNS will increase correspondingly. With the help of the PSS of the Stokes operator S Λ 2 , quantum improvements of both the SNR and FWHM of SNS signal has been demonstrated by controlling optical power of polarization squeezed light beam or atomic number density in our experiments.
Abstract With the help of Stokes operator Ŝ 2 squeezed state (also called polarization squeezed state (PSS)) of 795 nm light, rubidium-87 ( 87 Rb) atomic magnetometer based on Faraday rotation (FR) has been implemented and characterized. The PSS of Stokes operator Ŝ 2 of 795 nm light has been prepared by means of coherently combining the polarization coherent state (PCS) of a linearly p-polarized bright 795 nm light beam and a linearly s-polarized squeezed vacuum state (SVS) generated by a 397.5 nm ultraviolet laser pumped sub-threshold optical parametric oscillator (OPO) with a PPKTP bulk crystal inside the OPO cavity. PSS with a squeezing level of −3.7 ± 0.3 dB has been achieved around the analysis frequency of 10 kHz. At different transitions of D 1 line, various frequency detuning, and reasonable atomic vapor cell’s temperature, FR has been measured and compared. To decrease absorption (scattering) losses and the back-action from atomic spin noise to the probe beam’s polarization noise for maintaining the quantum properties of PSS of Stokes operator Ŝ 2 of 795 nm light, we had to run our magnetometer with 87 Rb vapor cell’s temperature below 60 °C, at which the PSS was almost destroyed. The sensitivities of magnetic field measurement were characterized via measuring signal-to-noise ratio of the alternating current calibrated magnetic field signal with a balanced polarimeter. Under the conditions of the atomic number density of ∼5.8 × 10 10 cm −3 ( T ∼ 40 °C) and the probe beam with a detuning of ∼−400 MHz relative to the 5S 1/2 ( F g = 2) − 5P 1/2 ( F e = 1) transition of 87 Rb D 1 line, a typical sensitivity of ∼19.5 pT (Hz 1/2 ) −1 has been achieved employing PSS of Stokes operator Ŝ 2 as the probe, compared with a sensitivity of ∼28.3pT (Hz 1/2 ) −1 using PCS as the probe. We preliminarily demonstrated that the quantum-enhanced sensitivity in a Faraday-rotation-based 87 Rb atomic magnetometer with the help of PSS of 795 nm light.
We report quantum enhancement of Faraday rotation spin noise spectroscopy by polarization squeezing of the probe beam. Using natural abundance Rb in 100 Torr of N2{\mathrm{N}}_{2}N2​ buffer gas and squeezed light from a subthreshold optical parametric oscillator stabilized 20 GHz to the blue of the D1{D}_{1}D1​ resonance, we observe that an input squeezing of 3.0 dB improves the signal-to-noise ratio by 1.5 to 2.6 dB over the combined (power)$\ensuremath{\bigotimes}$(number density) ranges (0.5--4.0 mW)$\ensuremath{\bigotimes}(1.5\ifmmode\times\else\texttimes\fi{}{10}^{12}\phantom{\rule{0.16em}{0ex}}{\mathrm{cm}}^{\ensuremath{-}3}$ to $1.3\ifmmode\times\else\texttimes\fi{}{10}^{13} {\mathrm{cm}}^{\ensuremath{-}3}$), covering the ranges used in optimized spin noise spectroscopy experiments. We also show that squeezing improves the tradeoff between statistical sensitivity and broadening effects, a previously unobserved quantum advantage.
Squeezed states are important sources in quantum physics, which have potential applications in fields such as quantum teleportation, quantum information networks, quantum memory, and quantum metrology and precise measurements. For our interest, the squeezed vacuum will be used in the quantum-enhanced optical atomic magnetometers, filling the vacuum port of the probe beam to improve measurement sensitivity. Based on the sub-threshold optical parametric oscillator (OPO) with PPKTP crystal, the squeezed vacuum at rubidium D1 line of 795 nm is obtained. In our work, we investigate the noise sources in an OPO system. By carefully controlling the classical noise source, the squeezing band extends to the analysis frequency of 2.6 kHz. The flat squeezing trace is 2.8 dB below the shot noise limit. In our work, we focus on the difference between the squeezing results at the analysis frequency of kilohertz regime at two different wavelengths, 1064 nm and 795 nm. The difference mainly comes from the absorption of 795 nm laser and its second harmonic at 397.5 nm in crystal (397.5 nm laser is at the edge of transparent window of PPKTP crystal that has an absorption index much higher than at other wavelength). The absorption induced nonlinear loss and thermal instability greatly affect the squeezing results, which is discussed in our work. Squeezing level at 795 nm is worse than at 1064 nm due to the above-mentioned factors. Noise coupling to the detection system limits the squeezing band. In the audio frequency band, squeezing is easily submerged in roll-up noises and the measured squeezing level is limited. Two factors limit the obtained squeezing:the technical noise induced in the detection and the squeezing degradation by the noise coupling of the control beams. In experiment, we carefully control the classical noise at analytical frequency of kilohertz by means of a vacuum-injected OPO, a counter-propagating cavity locking beam with orthogonal polarization, low noise homodyne detector, stable experimental system and quantum noise locking method for squeezing phase locking. Firstly, to preclude the classical noise from coupling the laser source, we use the vacuum injected OPO. A signal beam helps optimize the parametric gain and is blocked in the squeezing measurement process. In order to maintain the OPO, a counter-propagating beam with orthogonal polarization is used for locking the cavity. Then, a low noise balanced homodyne detector with a common-mode rejection ratio of 45 dB helps improve the audio frequency detection. Finally, the quantum noise locking provides a method to lock the relative phase between the coherent beam and the squeezed vacuum field. With the combination of these technical improvements, a squeezed vacuum of 2.8 dB is obtained at the analysis frequency of 2.6-100 kHz. The obtained squeezing level is mainly limited by the relatively large loss in OPO, which is induced by ultra-violet absorption in PPKTP crystal. The generated squeezed field is used to reduce the polarization noise of probe beam in an optical magnetometer, in order to increase detection sensitivity.
line (795 nm) is achieved, with the lowest squeezing band at an audio frequency of 2.6 kHz. It is synthetized by a bright coherent beam and a squeezed vacuum, which are orthogonally polarized and share same frequency. Two methods are applied to support the optical parametric oscillator: an orthogonally-polarized locking beam that precludes residual unwanted interference and quantum noise locking method that locks the squeezing phase. Besides, the usage of low noise balanced detector, mode cleaner and the optical isolator helped to improve the audio frequency detection. The squeezing level is limited by absorption-induced losses at short wavelengths, which is 397.5 nm. The generated polarization squeezed light can be used in a quantum enhanced magnetometer to increase the measurement sensitivity.
Spin squeezing can suppress quantum projection noise via interparticle entanglement, therefore enabling measurement sensitivities beyond the standard quantum limit. In practice, however, the Gaussian and finite intensity profiles of the optical probe beam induce spatially inhomogeneous atom-light interactions. As polarized atoms move within a vapor cell, they experience position-dependent optical intensities, generating transit noise that limits spin squeezing performance. Here, we investigate the transit noise in a coated rubidium vapor cell through combined theoretical analysis and experimental measurements. By varying the probe beam diameter, we quantify the dependence of transit noise on beam size and atomic Larmor frequency. Our results show that, for a vapor cell with fixed dimensions, the transit noise increases as the probe beam spot area decreases. Moreover, when the Larmor frequency is below the characteristic linewidth of the transit noise, the noise contribution becomes larger. We further calculated and measured spin squeezing for different beam sizes and found an experimental difference of 2.7±0.22.7 \pm 0.22.7±0.2 dB between 2~mm and 0.6~mm, similar to the theoretical prediction of 3.0±0.33.0 \pm 0.33.0±0.3 dB. Theoretical analysis under conditions of stronger squeezing shows that transit noise becomes an even more critical limiting factor. These results provide practical guidance for optimizing probe beam parameters and suppressing transit noise in spin squeezing experiments.