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arXiv:1610.02356 · Physical Review A

Sensitivity, quantum limits, and quantum enhancement of noise spectroscopies

Vito Giovanni Lucivero, Aleksandra Dimić, Jia Kong, Ricardo Jiménez-Martínez, Morgan W. Mitchell

Published Apr 21, 2017• 25 citations
arXivHTMLPDF

Abstract

We study the fundamental limits of noise spectroscopy using estimation theory, Faraday rotation probing of an atomic spin system, and squeezed light. We find a simple and general expression for the Fisher information, which quantifies the sensitivity to spectral parameters such as resonance frequency and linewidth. For optically detected spin noise spectroscopy, we find that shot noise imposes ``local'' standard quantum limits for any given probe power and atom number, and also ``global'' standard quantum limits when the probe power and atom number are taken as free parameters. We confirm these estimation theory results using nondestructive Faraday rotation probing of hot Rb vapor, observing the predicted optima, and finding good quantitative agreement with a first-principles calculation of the spin noise spectra. Finally, we show sensitivity beyond the atom- and photon-number-optimized global standard quantum limit using squeezed light.

DOI
10.1103/physreva.95.041803

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We study the fundamental limits of noise spectroscopy using estimation theory, Faraday rotation probing of an atomic spin system, and squeezed light. We find a simple and general expression for the Fisher information, which quantifies the sensitivity to spectral parameters such as resonance frequency and linewidth. For optically detected spin noise spectroscopy, we find that shot noise imposes local'' standard quantum limits for any given probe power and atom number, and also global'' standard quantum limits when the probe power and atom number are taken as free parameters. We confirm these estimation theory results using nondestructive Faraday rotation probing of hot Rb vapor, observing the predicted optima, and finding good quantitative agreement with a first-principles calculation of the spin noise spectra. Finally, we show sensitivity beyond the atom- and photon-number-optimized global standard quantum limit using squeezed light.
We report quantum enhancement of Faraday rotation spin noise spectroscopy by polarization squeezing of the probe beam. Using natural abundance Rb in 100 Torr of N2{\mathrm{N}}_{2}N2​ buffer gas and squeezed light from a subthreshold optical parametric oscillator stabilized 20 GHz to the blue of the D1{D}_{1}D1​ resonance, we observe that an input squeezing of 3.0 dB improves the signal-to-noise ratio by 1.5 to 2.6 dB over the combined (power)$\ensuremath{\bigotimes}$(number density) ranges (0.5--4.0 mW)$\ensuremath{\bigotimes}(1.5\ifmmode\times\else\texttimes\fi{}{10}^{12}\phantom{\rule{0.16em}{0ex}}{\mathrm{cm}}^{\ensuremath{-}3}$ to $1.3\ifmmode\times\else\texttimes\fi{}{10}^{13} {\mathrm{cm}}^{\ensuremath{-}3}$), covering the ranges used in optimized spin noise spectroscopy experiments. We also show that squeezing improves the tradeoff between statistical sensitivity and broadening effects, a previously unobserved quantum advantage.
We study the effect of optical squeezing on the performance of a sensitive, quantum-noise-limited optically-pumped magnetometer. We use Bell-Bloom optical pumping to excite a 87^{87}87Rb vapor and Faraday rotation to detect spin precession. The sub-pT/Hz\mathrm{pT}/\sqrt{\mathrm{Hz}}pT/Hz​ sensitivity is limited by spin projection noise (photon shot noise) at low (high) frequencies. Probe polarization squeezing both improves high-frequency sensitivity and increases signal bandwidth. The accompanying polarization anti-squeezing perturbs only an unmeasured spin component, so there is no loss of sensitivity at any frequency. The method is compatible with high-density and multi-pass techniques that reach extreme sensitivity.
Quantum metrology enables us to estimate optical phase shifts beyond the shot noise limit. Applications include quantum-enhanced biological measurement [1], microscopy [2] and gravitational wave detection[3]. For two-mode N-photon system, the NOON state can achieve the highest possible phase sensitivity where multi-photon coherence between two states significantly contributes to improving the phase sensitivity. Another alternative approach to improve the phase sensitivity by use of squeezed states. Squeezing is usually characterized by reducing the quantum noise of desired observable at the expense of increasing the quantum noise for its non-commute partner. Because shot-noise limits the phase sensitivity of any classical states, the reduced quantum noise can be used for improving the phase sensitivity. Here we experimentally study the phase sensitivity of an optical spin-squeezed state by using linear optics. We generated the optical spin-squeezed state using one photon subtraction from a down converted photon source. To implement the sub-shot noise measurement, we used multiplexed photon number resolving detectors so that we can reconstruct the photon number statistics of the state. In the talk, we will analyse the generated state in terms of both squeezing and phase sensitivity by using Fisher information.
Nowadays there is a considerable progress in optical magnetometry and spin noise spectroscopy, which use magnetically-sensitive atomic ensembles and optical read-out, approaching the limits set by quantum mechanics. In recent years optical magnetometers have become the most sensitive instruments for measuring low-frequency magnetic fields, achieving sub-femtotesla sensitivity and surpassing the competitive superconducting quantum interference devices (SQUIDs), and have found applications in biomedicine, geophysics, space science as well as in tests of fundamental physics. Another emerging technique is spin noise spectroscopy (SNS), which allows one to determine physical properties of an unperturbed spin system from its power noise spectrum. 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The new experimental system is combined with an existing source of polarization squeezed light based on spontaneous parametric down conversion (SPDC) in a nonlinear crystal, which is the active medium of an optical parametric oscillator. Secondly, we report the first experimental demonstration of quantum-enhanced spin noise spectroscopy of natural abundance Rb via polarization squeezing of the probe beam. We found that input squeezing of 3.0 dB improves the signal-to-noise ratio by 1.5 dB to 2.6 dB over the combined (power¿number density) ranges (0.5 mW to 4.0 mW) ¿ (1.5 ׿10¿^12 ¿cm¿^(-3) to 1.3 ׿10¿^13 ¿cm¿^(-3)), covering the ranges used in optimized spin noise spectroscopy experiments. We also show that squeezing improves the trade-off between statistical sensitivity and broadening effects. Next, we introduce a novel theoretical model by defining a standard quantum limit (SQL) for optically-detected noise spectroscopy, identified as a bound to the covariance of the parameters estimated by fitting power noise spectra. We test the model for spin noise spectroscopy of natural abundance Rb and we demonstrate experimental performance of SNS at the SQL for a coherent probe and below the SQL for a polarization squeezed probe. Finally, we report an optical magnetometer based on amplitude modulated optical rotation (AMOR), using a 85Rb vapor cell, that achieves room temperature sensitivity of 70 fT/vHz at 7.6 µT and we demonstrate its photon shot-noise-limited (SNL) behaviour from 5 µT to 75 µT. 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For many years the "shot-noise limit" has been considered as the fundamental limitation on measurements made with light beams. Shot noise is due to the quantum nature of light: the number of photons detected in a given time from a "stable" light beam (for instance, a laser beam) is an intrinsically random number which has fluctuations of order N1/2 if the average result is N. So if the number of photons, N, is limited by time or power considerations, shot noise places a fundamental limitation on the precision to which intensity, and changes in intensity, can be measured. This is particularly critical for "one-shot" ultra-sensitive experiments, such as the detection of a gravitational burst using large-scale interferometers.
We investigate the properties of angular-momentum states which yield high sensitivity to rotation. We discuss the application of these ``squeezed-spin'' or correlated-particle states to spectroscopy. Transitions in an ensemble of N two-level (or, equivalently, spin-1/2) particles are assumed to be detected by observing changes in the state populations of the particles (population spectroscopy). When the particles' states are detected with 100% efficiency, the fundamental limiting noise is projection noise, the noise associated with the quantum fluctuations in the measured populations. If the particles are first prepared in particular quantum-mechanically correlated states, we find that the signal-to-noise ratio can be improved over the case of initially uncorrelated particles. We have investigated spectroscopy for a particular case of Ramsey's separated oscillatory method where the radiation pulse lengths are short compared to the time between pulses. We introduce a squeezing parameter ${\ensuremath{\xi}}_{\mathit{R}}$ which is the ratio of the statistical uncertainty in the determination of the resonance frequency when using correlated states vs that when using uncorrelated states. More generally, this squeezing parameter quantifies the sensitivity of an angular-momentum state to rotation. Other squeezing parameters which are relevant for use in other contexts can be defined. We discuss certain states which exhibit squeezing parameters ${\ensuremath{\xi}}_{\mathit{R}}$\ensuremath{\simeq}${\mathit{N}}^{\mathrm{\ensuremath{-}}1/2}$. We investigate possible experimental schemes for generation of squeezed-spin states which might be applied to the spectroscopy of trapped atomic ions. We find that applying a Jaynes-Cummings--type coupling between the ensemble of two-level systems and a suitably prepared harmonic oscillator results in correlated states with ${\ensuremath{\xi}}_{\mathit{R}}$1.