The LaAlO$_3$/SrTiO$_3$ (LAO/STO) interface hosts a gate-tunable superconducting two-dimensional electron gas (2DEG) which can be programmed to create quantum devices such as ballistic electron waveguides and quantum dots. To fully exploit this platform for quantum transport, a key requirement is the ability to shuttle single electrons, electron pairs, and other exotic states between spatially separated devices with precision. Surface acoustic waves (SAWs), which travel along the surface of a solid, offer a powerful route to achieve this through their moving electrical potential that captures and transfers electrons. %acoustoelectric coupling. In particular, SAWs in the GHz regime enable fast, controlled transport of individual quantum particles. Although this approach is well-explored in GaAs-based 2DEG, SAW generation in STO remains largely unexplored due to the lack of intrinsic piezoelectricity at room temperature. Here, we investigate room-temperature SAWs in LAO/STO and observe SAW modes up to 2.2 GHz with very low propagation loss of the order $10^{-3}$ dB per wavelength. To directly visualize these modes, we employ Atomic Acoustic Force Microscopy (AAFM), achieving sub-micron resolution imaging of the SAW wave forms, providing insight into the electrostriction-induced SAW generation mechanism. Our measurements indicate a shear horizontal-type mode, which provides the ability to couple to in-plane degrees of freedom for future acoustoelectric and quantum device applications. This work studies the fundamentals of SAW excitation and propagation on STO, a widely used and commercially available substrate, enabling straightforward coupling of SAWs to a broad range of materials that can be grown or transferred onto STO.
Imaging GHz surface acoustic wave modes in electrostricted LaAlO3/SrTiO3 heterostructures
The LaAlO3/SrTiO3 (LAO/STO) interface hosts a gate-tunable superconducting two-dimensional electron gas (2DEG) which can be programmed to create quantum devices such as ballistic electron waveguides and quantum dots. To fully exploit this platform for quantum transport, a key requirement is the ability to shuttle single electrons, electron pairs, and other exotic states between spatially separated devices with precision. Surface acoustic waves (SAWs), which travel along the surface of a solid, offer a powerful route to achieve this through their moving electrical potential that captures and transfers electrons. %acoustoelectric coupling. In particular, SAWs in the GHz regime enable fast, controlled transport of individual quantum particles. Although this approach is well-explored in GaAs-based 2DEG, SAW generation in STO remains largely unexplored due to the lack of intrinsic piezoelectricity at room temperature. Here, we investigate room-temperature SAWs in LAO/STO and observe SAW modes up to 2.2 GHz with very low propagation loss of the order 10−3 dB per wavelength. To directly visualize these modes, we employ Atomic Acoustic Force Microscopy (AAFM), achieving sub-micron resolution imaging of the SAW wave forms, providing insight into the electrostriction-induced SAW generation mechanism. Our measurements indicate a shear horizontal-type mode, which provides the ability to couple to in-plane degrees of freedom for future acoustoelectric and quantum device applications. This work studies the fundamentals of SAW excitation and propagation on STO, a widely used and commercially available substrate, enabling straightforward coupling of SAWs to a broad range of materials that can be grown or transferred onto STO.
Gallium arsenide is piezoelectric, so it is possible to generate coupled mechanical and electrical surface acoustic waves (SAWs) by applying a high-frequency voltage to a transducer on the surface of GaAs. By combining SAWs with existing low-dimensional nanostructures one can create a series of dynamic quantum dots corresponding to the minima of the travelling electric wave, and each dot carries a single electron at the SAW velocity (∼ 2800 m/s). These devices may be of use in developing future quantum information processors, and also offer an ideal environment for probing the quantum mechanical behaviour of single electrons. This thesis describes a numerical and theoretical study of the dynamics of an electron in a range of geometries. The numerical techniques for solving the time-dependent Schr ̈dinger equation with an arbitrary time-dependent potential will be described in Chapter 2, and then applied in Chapter 3 to calculate the transmission of an electron through an Aharonov-Bohm (AB) ring. It will be seen that an important property of the techniques used in this thesis is that they can be easily adapted to study realistic geometries, and we will see features in the AB oscillations which do not arise in simplified analytic descriptions. In Chapter 4, we will then study a device consisting of two parallel SAW channels separated by a controllable tunnelling barrier. We will use numerical simulations to investigate the effect of electric and magnetic fields upon the electron dynamics, and develop an analytic model to explain the simulation results. From the model, it will be apparent that it is possible to use this device to rotate the state of the electron to an arbitrary superposition of the first two eigenstates. We then introduce coherent and squeezed states in Chapter 5, which are ex- cited states of the quantum harmonic oscillator. Coherent and squeezed electronic states may be of use in quantum information processing, and could also arise due to unwanted perturbations in a SAW device. We will discuss how these states can be controllably generated in a SAW device, and also discuss how they could then be detected. In Chapter 6 we describe how to use the motion of a SAW to create a rapidly- changing potential in the frame of the electron, leading to a nonadiabatic excita- tion. The nonadiabatically-excited state oscillates from side to side within a 1D channel on a few-picosecond timescale, and this motion can be probed by placing a tunnelling barrier at one side of the channel. Numerical simulations will be performed to show how this motion can be controlled, and the simulation results will be seen to be in good agreement with recent experimental work performed by colleagues. Finally, we will show that this device can be used to measure the initial state of an electron which is an arbitrary superposition of the first two eigenstates.
We present systematic measurements of the quality factors of surface acoustic wave (SAW) resonators on ST-X quartz in the gigahertz range at a temperature of 10mK. We demonstrate an internal quality factor Qi approaching 0.5 million at 0.5GHz and show that ${Q}_{\mathrm{i}}\ensuremath{\ge}4.0\ifmmode\times\else\texttimes\fi{}{10}^{4}$ is achievable up to 4.4GHz. We show evidence for a polynomial dependence of propagation loss on frequency, as well as a weak drive power dependence of Qi that saturates at low power, the latter being consistent with coupling to a bath of two-level systems. Our results indicate that SAW resonators are promising devices for integration with superconducting quantum circuits.
The past 20 years has seen rapid developments in circuit quantum electrodynamics, where superconducting qubits and resonators are used to control and study quantum light-matter interaction at a fundamental level. The development of this field is strongly influenced by quantum information science and the prospect of realizing quantum computation, but also opens up opportunities for combinations of different physical systems and research areas. Superconducting circuits in the microwave domain offer a versatile platform for interfacing with other quantum systems thanks to strong nonlinearities and zero-point fluctuations, as well as flexibility in design and fabrication. Hybrid quantum systems based on circuit quantum electrodynamics could enable novel functionalities by exploiting the strengths of the individual components.This thesis covers experiments coupling superconducting circuits to surface acoustic waves (SAWs), mechanical waves propagating along the surface of a solid. Strong coupling can be engineered using the piezoelectric properties of GaAs substrates, and our experiments exploit this to investigate phenomena in quantum field-matter interaction. A key property of surface acoustic waves is the slow propagation speed, typically five orders of magnitude slower than light in vacuum, and the associated short wavelength. This enables the giant atom regime where the artificial atom in the form of a superconducting circuit is large compared to the wavelength of interacting SAW radiation, a condition which is difficult to realize in other systems. Experiments described in this thesis use these properties to demonstrate electromagnetically induced transparency for a mechanical mode, as well as non-Markovian interactions between an artificial giant atom and the SAW field. When the SAW field is confined to a resonant cavity, the short wavelength allows multimode spectra suitable for interacting with a frequency comb. We use a multimode SAW resonator to characterize the ensemble of microscopic two-level system defects with a two-tone spectroscopy approach. Finally, we introduce a hybrid superconducting-SAW resonator with applications in quantum information processing in mind. Experiments with this device demonstrate entanglement of SAW modes, and show promising results on the way to engineer cluster states for quantum computation in continuous variables.
One of the most fundamental phenomena occurring in nature is the interaction between single atoms and electromagnetic fields. This is studied in quantum optics to probe the quantum nature of the system. In appended Paper I, we demonstrated that an artificial atom can couple to propagating sound, which is the acoustic analogue of quantum optics. This thesis covers experiments where surface acoustic waves (SAWs) are used in superconducting circuits at gigahertz frequencies with the aim for quantum applications.Since SAWs are mechanical vibrations that propagate on the surface of solids and dissipate little power, they can propagate freely over long distances before and after they interact with the artificial atom. Their five order of magnitude slower speed and smaller wavelength than light at gigahertz frequencies, open up for exploring new regimes of quantum physics. In addition, the coupling between the artificial atom and the SAWs is promising for reaching ultrastrong coupling limits, which is hard in other types of systems. Many of the future applications are discussed in appended Paper II, together with a more detailed description of the theory and fabrication of the devices.Although the possibilities are many, a variety of potential experiments would benefit from higher conversion efficiency between electric signals and SAWs. Therefore, improvements of this conversion are studied in appended Paper III, making use of the many advances in classical SAW devices. More specifically, the conversion of unidirectional transducers (UDTs) on lithium niobate is studied and compared to symmetric interdigital transducers (IDTs). The results show that 99.4 % of the acoustic power can be focused in the desired direction and that the conversion between electric signals and SAWs is greatly improved by using UDTs, eliminating the largest contribution to loss of the IDTs. However, there is a trade-off between conversion efficiency and bandwidth. This knowledge allows us to better tailor potential quantum experiments based on SAWs, possibly towards measuring quantum sound.
Surface acoustic waves (SAWs) are mechanical vibrations that propagate on the surface of solids while dissipating little power, consequently enabling them to propagate freely over long distances. The speed and wavelength of SAWs are reduced a five order of magnitude compared to when light is used as a carrier at gigahertz frequencies. The unique properties of SAWs combined with the possibility to let them interact with artificial atoms, discovered and shown for the very first time in appended Paper I of this thesis, open up for exploration of new regimes of quantum physics. The appended Paper II is a book chapter providing an overview of many of the new areas of research, as well as going into depth of the method and significance of the results ofthe appended Paper I.The essential interaction between artificial atoms and SAWs was further investigated by using Autler-Townes splitting to achieve fast control of the interactions. The appended Paper IV, shows a transmitted field extinction of 80 %, and provides proof of concept for a SAW router in the quantum regime. In addition, due to the artificial atom's highly frequency dependent coupling to SAWs, electromagnetically induced transparency (EIT) could be observed in the appended Paper V. Furthermore, the EIT region was distinguished from the Autler-Townes splitting region by a threshold in the applied power. The results produce parallel findings to quantum optics, but are perhaps best described as part of a different field, quantum acoustics.Among the many possible areas of research emerging as an outcome of this work, a variety of potential quantum experiments would benefit greatly from a higher conversion efficiency between electric signals and SAWs. Due to this, focus was put on improving this conversion efficiency by studying superconducting unidirectional transducers (UDTs), making use of advances in classical SAW devices. The appended Paper III shows that 99.4~\\% of the acoustic power can be focused in a desired direction and that the conversion between electric signals and SAWs is greatly improved by using UDTs, thereby eliminating the largest source of loss of symmetric inter-digital transducers. There is, however, a trade-off between conversion efficiency and bandwidth. This finding allows tailoring of quantum experiments based on SAWs that may pave the way towards measuring quantum sound.
Ferroelectric materials, with their strong nonlinearities, underpin key technologies across radio-frequency (RF) signal processing, optical communications, and emerging quantum systems. Barium titanate (BTO) is a notable example, combining strong piezoelectric and electro-optic responses. While bulk BTO has been studied for decades, the piezoelectric properties of its recently available thin films, and their behavior at the millikelvin temperatures relevant to quantum hardware, remain largely unexplored. Here, we fabricate and characterize surface acoustic wave (SAW) resonators on thin-film BTO. The measured devices exhibit high electromechanical coupling (k2eff 0.14 at 5.2 GHz) and operate up to 7.8 GHz. From these measurements, combined with finite-element modeling of the multi-domain microstructure, we extract an effective piezoelectric coefficient d33eff of 53 pC/N, comparable to bulk BTO. Exploiting the intrinsic ferroelectricity, we further demonstrate low-voltage switching with a fast (100 ns) response, attractive for reconfigurable RF front-ends and parametric amplifiers. Extending these measurements to millikelvin temperatures, we find that the piezoelectric response persists, with d33eff 19 pC/N, pointing to the potential of BTO for piezoelectric coupling in superconducting quantum circuits. These results position thin-film BTO as a promising piezoelectric platform for both classical and quantum information technologies.