Planar germanium heterostructures hosting hole-spin qubits are among the leading platforms for scalable semiconductor-based quantum computing. Yet, device performance is hindered by significant quantum dot variability, which leads to uncertainty in qubit energy levels and random orientations of the spin quantization axis. Tailored control of the g-tensor offers a strategy to overcome these limitations and achieve more reliable qubit operations. Here, we introduce a flexible optimization framework for engineering g-tensor properties. As a benchmark, we numerically obtain the optimal reshaping of the out-of-plane potential in a SiGe-Ge-SiGe quantum well to suppress the in-plane g-tensor components and realize the recently proposed gapless single-spin qubit encoding. This reshaping is achieved through heterostructure engineering, specifically by adjusting the silicon concentration within the quantum well, though the framework remains readily adaptable to alternative design objectives. Our results provide practical design principles for improving the tunability of the spin response, paving the way towards large-scale germanium-based quantum computers.
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Code available at https://gitlab.com/QMAI/papers/germaniumoptimization 18 pages, 14 figures
Planar germanium heterostructures hosting hole-spin qubits are among the leading platforms for scalable semiconductor-based quantum computing. Yet, device performance is hindered by significant quantum dot variability, which leads to uncertainty in qubit energy levels and random orientations of the spin quantization axis. Tailored control of the g-tensor offers a strategy to overcome these limitations and achieve more reliable qubit operations. Here, we introduce a flexible optimization framework for engineering g-tensor properties. As a benchmark, we numerically obtain the optimal reshaping of the out-of-plane potential in a SiGe-Ge-SiGe quantum well to suppress the in-plane g-tensor components and realize the recently proposed gapless single-spin qubit encoding. This reshaping is achieved through heterostructure engineering, specifically by adjusting the silicon concentration within the quantum well, though the framework remains readily adaptable to alternative design objectives. Our results provide practical design principles for improving the tunability of the spin response, paving the way towards large-scale germanium-based quantum computers.
Hole spin qubits in planar germanium heterostructures are frontrunners for scalable semiconductor quantum computing. However, their current performance is mostly limited by large dot-to-dot variability that leads to uncontrolled qubit energies and random tilts in the spin quantization axis. Here, we propose a systematic and local method to engineer the spin qubit response by imprinting a controlled anisotropy in the quantum dot confinement, enabling on-demand electric g-tensor control. In particular, we find that both the quantum-dot size and asymmetry allow electrical tuning of the g-tensor and significantly suppress magnitude and angular variability of the spin response for selected magnetic field directions. We confirm this behavior by analyzing single-disorder realizations and statistical ensembles in state-of-the-art strained and unstrained germanium channels, showing that the latter provides an optimal path for g-tensor engineering. Our results provide practical design principles for on-demand control of the spin response and mitigating variability, paving the way towards large-scale germanium-based quantum computers.
Achieving valley splittings well in excess of the thermal energy of electrons and avoiding valley excitations is essential for the consistent initialization, operation and readout of gate-defined Si spin qubits. In this work, we present a device-level optimization strategy for pushing valley splittings to between 1 and 5 meV, well beyond values reported in nearly all previous theoretical studies. Using device-scale simulations that incorporate atomistic alloy disorder through a 1D tight-binding theory, we demonstrate that our proposed approach yields large valley splittings with a tight distribution across disorder realizations, a key requirement for reproducible qubit performance at scale. The approach rests on an unorthodox Si/SiGe heterostructure design combining a narrow quantum well, a small Ge spike, and a pure-Ge cap. We corroborate these predictions with targeted atomistic density functional theory calculations. These results offer a clear path forward for scalable Si/SiGe spin qubit devices and, if realized experimentally, effectively eliminate valley splitting as an existential problem for large scale SiGe-based quantum processors.
Spin qubits in semiconductor quantum dots constitute one of the leading platforms for quantum information processing, combining long coherence times, high-fidelity gate operations, and compatibility with semiconductor industry technologies. In particular, holes confined in planar Ge/SiGe heterostructures have recently emerged as promising qubit candidates owing to their low effective mass, high mobility, low percolation density, absence of valley states, and strong spin-orbit interaction, which enables fast all-electrical spin control. At the same time, spin-orbit interaction also gives rise to a highly anisotropic and electrically tunable gyromagnetic response. Understanding and controlling this response is therefore essential for high-fidelity single- and multi-qubit operations. The realization of scalable quantum processors also requires efficient qubit readout and long-range connectivity. Circuit quantum electrodynamics (cQED), based on the coupling between artificial atoms and microwave photons confined in superconducting resonators, provides a natural framework to address these challenges. However, the implementation of hybrid semiconductor-superconductor devices in planar Ge has so far been hindered by large microwave losses originating from the heterostructure. In this thesis, we demonstrate, for the first time in planar Ge, strong coupling between a hole charge qubit in a double quantum dot and a high-impedance microwave resonator, reaching a cooperativity of C â 100. In addition, we leverage the frequency tunability of the resonator to perform detailed spectroscopy of a multi-level energy spectrum of low-lying states arising from strong Coulomb-correlation effects. To further improve the quality of the hole-photon interface, we investigate the source of microwave losses in different Ge/SiGe heterostructures, identifying defects at the lattice-mismatched Si/Ge interface as the dominant source of resonator losses in reverse-graded heterostructures. To mitigate this limitation, a deep tapered-etching approach is introduced, enabling the fabrication of superconducting resonators directly on etched heterostructures. This method yields internal quality factors exceeding Qint > 10 000 for high-impedance Josephson junction array resonators and Qint > 100 000 for 50 â Nb resonators. Finally, this thesis explores the spin properties of multi-hole quantum dots beyond the conventional single-orbital picture. By reconstructing and electrically tuning the g tensors of holes confined in different orbital states, we show that confinement can substantially modify both their magnitude and orientation. These results open new opportunities for engineering qubit properties through orbital occupation. Furthermore, highly coherent singlet-triplet oscillations are demonstrated in the seven-hole regime, yielding a quality factor of approximately 330 at in-plane magnetic fields as low as 2.5 mT. Together, these results establish a foundation for high-fidelity hole-spin-qubit operation based on g-tensor engineering and for the integration of planar Ge quantum dots with superconducting quantum circuits.
Strained germanium (ε-Ge) quantum wells on metamorphic SiGe buffers have enabled advanced hole-based spin qubit devices. Alternatively, unstrained Ge with lattice-matched strained silicon-germanium (ε-SiGe) barriers eliminates the need for metamorphic buffers altogether. The ground state character of both these platforms is predominantly heavy-hole (HH) with a largely anisotropic spin response. We propose and study an alternative heterostructure, lattice-matched to Ge, in which both the SiGe quantum well and barriers are tensile strained, with their composition contrast providing the band offset for confinement and the tensile strain stabilizing a light-hole (LH) ground state. We show large spin-orbit coupling (SOC), both linear and cubic, along with a significantly more isotropic spin response compared to strained HH qubits. We also study the decoherence properties of the proposed device, showing an appreciable gain in the quality factor compared to their HH counterparts. Finally, we propose a bilayer heterostructure that allows for electrical switching between HH and LH ground state character.
Small and device-dependent valley splittings remain a key challenge for electron spin qubits in silicon (Si), directly limiting qubit fidelity, device uniformity, and the scalability of Si-based quantum processors. In silicon-germanium (SiGe) heterostructures, this problem can be addressed through engineering of the epitaxial layer stack. Several heuristic strategies have been proposed to enhance the energy gap between the two nearly degenerate valley states in strained Si/SiGe quantum wells (QWs), e.g., sharp Si/SiGe interfaces, Ge spikes, or oscillating Ge concentrations within the QW. Here, we develop a systematic variational optimization approach to compute optimal Ge concentration profiles that enhance selected properties of the intervalley coupling matrix element. Our free-shape optimization framework is augmented by realistic technological constraints to ensure feasibility of the resulting epitaxial profiles and is based on an effective-mass envelope-function theory accounting for strain and compositional alloy disorder. Previously proposed heterostructure designs are recovered as special cases of the constrained optimization problem. Our main result is a novel heterostructure design, which we refer to as the "modulated wiggle well", providing both a large deterministic enhancement of the valley splitting and a strong suppression of disorder-induced variability. In addition, this design enables wide electrical tunability of the valley splitting - from approximately 200μeV to above 1meV - offering new opportunities for engineering robust and switchable silicon qubits.
Hole spin qubits based on semiconductor quantum dots are promising for building future large-scale quantum computers owing to their all-electrical manipulation. However, abundant physical mechanisms of valence band holes lead to anisotropic qubit properties. There is an opportunity to prolong the coherence time and achieve high-fidelity qubit manipulations. Here, we report a single-hole spin qubit in a planar germanium quantum dot and investigate its anisotropic susceptibility to charge noise under an in-plane magnetic field. By correlating the longitudinal spin-electric susceptibility with qubit coherence and control performance, we identify an optimal operating point where the sensitivity to charge noise is minimized. We find that optimizing the magnetic-field orientation reduces the spin-electric susceptibility, resulting in a five-fold enhancement of the Hahn-echo coherence time and a nearly tenfold suppression of control infidelity. At the optimal operating point, gate set tomography demonstrates the maximum gate fidelity of 99.82 %. Our finding enhances the prospects of hole spin qubits for scalable quantum information processing.