We investigate high frequency motional states of trapped atomic ions. Trapped ions in rf traps are confined by an approximate harmonic potential and exhibit quantum motional states that mediate essential techniques in quantum computing, simulation, networking, and precision measurement. However, motional state decoherence mechanisms, heating and dephasing, are broadly limiting: reduced two-qubit gate fidelities; lower fidelity and lifetime of highly nonclassical bosonic states; long laser cooling times; and large recoil heating rates. These also challenge the scalability of increasingly sophisticated protocols. We propose high motional frequency ion trapping as an operating regime that addresses these challenges and reshapes the design landscape for quantum information experiments and quantum control techniques. We report an experimentally motivated investigation of realizing this high-frequency regime and discuss the consequences for laser cooling, motional state coherence, fidelity and lifetime of nonclassical bosonic states, and scalability of experimental runtimes. We report clear design trajectories for ion traps to reach high motional frequency, a new limiting mechanism for laser cooling at these high frequencies, and more than an order-of-magnitude speedup in experimental duty cycles with larger speed ups possible for quantum error correction protocols. Taken together, high motional frequency ion trapping has broad implications for the future of quantum information experiments.
We investigate high frequency motional states of trapped atomic ions. Trapped ions in rf traps are confined by an approximate harmonic potential and exhibit quantum motional states that mediate essential techniques in quantum computing, simulation, networking, and precision measurement. However, motional state decoherence mechanisms, heating and dephasing, are broadly limiting: reduced two-qubit gate fidelities; lower fidelity and lifetime of highly nonclassical bosonic states; long laser cooling times; and large recoil heating rates. These also challenge the scalability of increasingly sophisticated protocols. We propose high motional frequency ion trapping as an operating regime that addresses these challenges and reshapes the design landscape for quantum information experiments and quantum control techniques. We report an experimentally motivated investigation of realizing this high-frequency regime and discuss the consequences for laser cooling, motional state coherence, fidelity and lifetime of nonclassical bosonic states, and scalability of experimental runtimes. We report clear design trajectories for ion traps to reach high motional frequency, a new limiting mechanism for laser cooling at these high frequencies, and more than an order-of-magnitude speedup in experimental duty cycles with larger speed ups possible for quantum error correction protocols. Taken together, high motional frequency ion trapping has broad implications for the future of quantum information experiments.
Since the dawn of quantum information science, laser-cooled trapped atomic ions have been one of the most compelling systems for the physical realization of a quantum computer. By applying qubit state dependent forces to the ions, their collective motional modes can be used as a bus to realize entangling quantum gates. Ultrafast state-dependent kicks [1] can provide a universal set of quantum logic operations, in conjunction with ultrafast single qubit rotations [2], which uses only ultrafast laser pulses. This may present a clearer route to scaling a trapped ion processor [3]. In addition to the role that spin-dependent kicks (SDKs) play in quantum computation, their utility in fundamental quantum mechanics research is also apparent. In this thesis, we present a set of experiments which demonstrate some of the principle properties of SDKs including ion motion independence (we demonstrate single ion thermometry from the ground state to near room temperature and the largest Schrodinger cat state ever created in an oscillator), high speed operations (compared with conventional atom-laser interactions), and multi-qubit entanglement operations with speed that is not fundamentally limited by the trap oscillation frequency. We also present a method to provide higher stability in the radial mode ion oscillation frequencies of a linear radiofrequency (rf) Paul trap--a crucial factor when performing operations on the rf-sensitive modes. Finally, we present the highest atomic position sensitivity measurement of an isolated atom to date of ~0.5 nm Hz^(-1/2) with a minimum uncertainty of 1.7 nm using a 0.6 numerical aperature (NA) lens system, along with a method to correct aberrations and a direct position measurement of ion micromotion (the inherent oscillations of an ion trapped in an oscillating rf field). This development could be used to directly image atom motion in the quantum regime, along with sensing forces at the yoctonewton [10^(-24) N)] scale for gravity sensing, and 3D imaging of atoms from static to higher frequency motion. These ultrafast atomic qubit manipulation tools demonstrate inherent advantages over conventional techniques, offering a fundamentally distinct regime of control and speed not previously achievable.
A trapped-ion harmonic oscillator represents a rich and well-controlled platform for tests of quantum physics, with applications to quantum simulations, quantum sensing, and quantum information processing. Owing to its net charge, the ion's motion is affected by changes in the electric potential. Consequently, electric field and potential curvature noise will limit the coherence of the ion's harmonic oscillation. While in some respects, this serves as a limitation in the performance of the trapped ion system (for example, in the fidelity of two-qubit gates or quantum simulations with motional quanta), it also opens an opportunity to use the ion as a precise field sensor and to use engineered quantum states of motion to enhance the sensitivity to these fields beyond the standard quantum limit (SQL). This thesis describes the implementation of such applications on a single beryllium ion confined in a Paul trap. In the thesis, I present the theory of an ideal harmonic oscillator and the implementation of this system using the motion of a single trapped ion, including producing special quantum states of motion; these states include the energy eigenstates of the harmonic oscillator, called number states, up to n=100, superpositions of number states of the form (1/√2)(|0> + |n>), with n up to 18, and coherently displaced number states with an average occupation up to approximately 300. I describe how we use these quantum states of motion for precise sensing of fluctuations of the harmonic oscillator frequency. The sensitivity of the (1/√2)(|0> + |n>) state ideally follows the 1/n Heisenberg scaling for frequency sensitivity. Additionally, I describe investigations of the spectrum of motional frequency noise using a series of coherent displacements of the motion of the ion, with features similar to Ramsey and dynamical decoupling sequences for two-level systems. While these displaced states don't improve sensitivity over the SQL, they can be simply and rapidly implemented with trapped ions. I discuss extensions to all of these experiments, including to multiple ions in a new trap designed to confine 3 or 4 ions in individually tunable potential wells.
Laser-cooled trapped ions are one of the main systems used in experiments in the fields of quantum optics and quantum information. There are two commonly-used types of ion trap, the radiofrequency trap and the Penning trap. In general, the RF trap has been more widely used in quantum information experiments, meaning that the set of experimental tools for conducting these types of experiments in a Penning trap is currently less complete. The aim of the work presented in this thesis is to increase this array of tools. Our experiment uses 40Ca+ ions in a Penning trap alongside lasers. Spectroscopy has been performed on single Doppler cooled ions, and on ions that have been prepared close to their ground state of motion using a multiple-stage sideband cooling technique resulting in an average phonon occupation number of $\nzbar = 0.029\pm 0.011$ from an initial $\nzbar \approx 24$. This corresponds to a quantum ground state population of 97%, which is close to the sideband cooling limit in our system. An axial heating rate measurement of $\dot{\bar{n}}_z=\SI{0.56\pm0.52}{\per\second}$ has also been obtained, which is the lowest recorded to date, due in part to the large dimensions of our trap. Additionally improved control of the Penning trap radial motion has been demonstrated and the average phonon occupation number of the modified cyclotron motion has been reduced from $\ncbar\approx150$ after Doppler cooling to $\ncbar=0.6$ after sideband cooling. Some preliminary single-ion coherent operations have also been performed. In the future we hope that this system of ground state cooled ions in a Penning trap can be used to generate highly-entangled states in two or more ions, with a view to performing simple quantum error-correcting codes and eventually an analogue quantum simulation of spin systems.
From subatomic particles to macromolecules, quantum mechanics has a deep impact in understanding the interactions and nature of such constituents of matter. The paradoxical observations of entanglement in quantum systems is used in quantum computations. Ion traps are among the leading platforms which provide clean and highly controllable quantum systems. This thesis presents the study of quantum coherence aiming to devise and test coherent control with trapped ions in a Penning trap. Our apparatus contains one or more calcium ions that are confined in space using DC electric and magnetic fields. Doppler cooling and resolved sideband cooling of trapped ions are carried out to perform high fidelity quantum control. The ions are prepared in their motional ground state via a multi-stage resolved sideband cooling technique. The cooling methods are first verified through simulations. The axial mean phonon numbers for a single ion are measured to be 0.03 ± 0.01 and 0.012 ± 0.009 at 187 kHz and 420 kHz axial frequencies, respectively. The heating rate is measured to be 2.5 ± 0.5 phonons/s, which is consistent with the previous measurements in our system. Similarly, the radial motional modes of a single ion are cooled to 〈n_+ 〉<0.4 and 〈n_- 〉<0.6 from mean phonon numbers corresponding to each mode of around 100. Preliminary studies are carried out of the axial motional modes of a 1D chain and 2D planar crystals, extending sideband cooling to small ICC's in a Penning trap. Coherent control is examined in our system and the optical coherence time and motional coherence time are estimated to be approximately 1 ms and 0.5 s, respectively. Furthermore, a single ion is prepared outside the Lamb-Dicke regime via a sideband heating technique and coherent studies are performed in such a regime via a laser beam.
Trapped ions are currently one of the most promising architectures for realising the quantum information processor. The long lived internal states are ideal for representing qubit states and, through controlled interactions with electromagnetic radiation, ions can be manipulated to execute coherent logic operations. In this thesis an experiment capable of trapping Yb+ ions, including 171Yb+, is presented. Since ion energy can limit the coherence of qubit manipulations, characterisation of an ion trap heating rate is vital. Using a trapped 174Yb+ ion a heating rate consistent with previous measurements of other ion species in similar ion traps is obtained. This result shows abnormal heating of Yb+ does not occur, further solidifying the suitability of this species for quantum information processing. Efficient creation, and cooling of trapped ions requires exact wavelengths for the ionising, cooling and repump transitions. A simple technique to measure the 1S0 ? 1P1 transition wavelengths, required for isotope selective photoionisation of neutral Yb, is developed. Using the technique new wavelengths, accurate to 60 MHz, are obtained and differ from previously published results by 660 MHz. Through a simple modification the technique can also predict Doppler shifted transition frequencies, which may be required in non-perpendicular atom-laser interactions. Using trapped ions, the 2S1=2 ? 2P1/2 Doppler cooling and 2D3/2 ? 2D[3/2]1/2 repump transitions are also measured to a greater accuracy than previously reported. Many experiments require wavelengths which can only be obtained using complex expensive laser systems. To remedy this a simple cost effective laser is developed to enable laser diodes to be operated at sub zero temperatures, extending the range of obtainable wavelengths. Additional diode modulation capabilities allow for the manipulation of atoms and ions with hyperfine structures. The laser is shown to be suitable for manipulating Yb+ ions by cooling a diode from 372 nm to 369 nm and simultaneously generating 2.1 GHz frequency sidebands. Coherent manipulation such as arbitrary qubit rotations, motional coupling and ground state cooling, are required for trapped ion quantum computing. Two photon stimulated Raman transitions are identified as a suitable technique to implement all of these requirements and an investigation into implementing this technique with 171Yb+ is conducted. The possibility of exciting a Raman transition via either a dipole or quadrupole transitions in 171Yb+ is analysed, with dipole transitions preferred because quadrupole transitions are found to be too demanding experimentally. An inexpensive setup, utilising a dipole transition, is designed and tested. Although currently limited the setup shows potential to be an inexpensive, high fidelity method of exciting a Raman transition.
While quantum information processing offers a tantalizing possibility of a significant speedup in execution of certain algorithms, as well as enabling previously unmanageable simulations of large quantum systems, it remains extremely difficult to realize experimentally. Recently, fundamental building blocks of a quantum computer, including one and two qubit gates, teleportation and error correction, were demonstrated using trapped atomic ions. Scaling to a larger number of qubits requires miniaturization of the ion traps, currently limited by the sharply increasing motional state decoherence at sub-100 μm ion-electrode distances. This thesis explores the source and suppression of this decoherence at cryogenic temperatures, and demonstrates fundamental logic gates in a surface electrode ion trap.
Construction of the apparatus requires the development of a number of experimental techniques. Design, numerical simulation and implementation of a surface electrode ion trap is presented. Cryogenic cooling of the trap to near 4 K is accomplished by contact with a bath cryostat. Ions are loaded by ablation or photoionization, both of which are characterized in terms of generated stray fields and heat load.
The bulk of new experimental results deals with measurements of electric field noise at the ion's position. Upon cooling to 6 K, the measured rates are suppressed by up to 7 orders of magnitude, more than two orders of magnitude below previously published data for similarly sized traps operated at room temperature. The observed noise depends strongly on fabrication process, which suggests further improvements are possible. The measured dependence of the electric field noise on temperature is inconsistent with published models, and can be explained using a continuous spectrum of activated fluctuators.
The fabricated surface electrode traps are used to demonstrate coherent operations and the classical control required for trapped ion quantum computation. The necessary spectral properties of coherent light sources are achieved with a novel design using optical feedback to a triangular, medium finesse, cavity, followed by electronic feedback to an ultra-high finesse reference cavity. Single and two qubit operations on a single ion are demonstrated with classical fidelity in excess of 95%. Magnetic field gradient coils built into the trap allow for individual addressing of ions, a prerequisite to scaling to multiple qubits. (Copies available exclusively from MIT Libraries, Rm. 14-0551, Cambridge, MA 02139-4307. Ph. 617-253-5668; Fax 617-253-1690.)