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arXiv:2603.28421 · Physical Review Applied

Learning unified control of intrinsic nonlinear spin dynamics in atomic qudits for magnetometry

C. Z. Cao, J. Z. Han, M. Xiong, M. Deng, L. Wang, Q. Liu, X. Lv, M. Xue

quant-phcs.AISubmitted Mar 30, 2026• Announced Mar 31, 2026• 0 citations• Revised Oct 28, 2026 (v3)
v1 · Mar 30, 2026v2 · Apr 28, 2026v3 · Oct 28, 2026
arXivHTMLPDF

Abstract

Generating and preserving metrologically useful quantum states is a central challenge in quantum-enhanced metrology. In low-field atomic magnetometry with multilevel atoms, the nonlinear Zeeman (NLZ) effect is both a resource and a limitation. It can generate internal spin squeezing within a single atomic qudit, but under fixed readout it also rotates and distorts the measurement-relevant quadrature, limiting the usable metrological gain. The problem is further complicated by the time dependence of both the squeezing axis and the nonlinear evolution itself. Here we show that reinforcement learning can transform NLZ dynamics from a source of readout degradation into a sustained metrological resource. Using only experimentally accessible low-order spin moments, a trained agent identifies a unified control policy for this class of intrinsically nonlinear sensing dynamics. We illustrate the approach in the \(f=21/2\) manifold of \(^{161}\mathrm{Dy}\), where the learned policy rapidly prepares strongly squeezed internal states and stabilizes more than \(4\,\mathrm{dB}\) of fixed-axis spin squeezing under continuous NLZ evolution. Including state-preparation overhead, the learned protocol yields a single-atom magnetic-field sensitivity of \(13.9\,\mathrm{pT}/\sqrt{\mathrm{Hz}}\), approximately \(3\,\mathrm{dB}\) beyond the standard quantum limit. Our results establish learning-based control as an experimentally feasible route for converting unavoidable intrinsic nonlinear dynamics in multilevel atomic sensors into operational metrological advantage.

DOI
10.1103/j8yl-nn8x
Comments
(6.5+3.5+4) pages, (4+4) figures

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Generating and preserving metrologically useful quantum states is a central challenge in quantum-enhanced metrology. In low-field atomic magnetometry with multilevel atoms, the nonlinear Zeeman (NLZ) effect is both a resource and a limitation. It can generate internal spin squeezing within a single atomic qudit, but under fixed readout it also rotates and distorts the measurement-relevant quadrature, limiting the usable metrological gain. The problem is further complicated by the time dependence of both the squeezing axis and the nonlinear evolution itself. Here we show that reinforcement learning can transform NLZ dynamics from a source of readout degradation into a sustained metrological resource. Using only experimentally accessible low-order spin moments, a trained agent identifies a unified control policy for this class of intrinsically nonlinear sensing dynamics. We illustrate the approach in the (f=21/2) manifold of (^{161}\mathrm{Dy}), where the learned policy rapidly prepares strongly squeezed internal states and stabilizes more than (4,\mathrm{dB}) of fixed-axis spin squeezing under continuous NLZ evolution. Including state-preparation overhead, the learned protocol yields a single-atom magnetic-field sensitivity of (13.9,\mathrm{pT}/\sqrt{\mathrm{Hz}}), approximately (3,\mathrm{dB}) beyond the standard quantum limit. Our results establish learning-based control as an experimentally feasible route for converting unavoidable intrinsic nonlinear dynamics in multilevel atomic sensors into operational metrological advantage.
In the Earth-field range, the nonlinear Zeeman (NLZ) effect has been a bottleneck limiting the sensitivity and accuracy of atomic magnetometry from physical mechanism. To break this bottleneck, various techniques are introduced to suppress the NLZ effect. Here we revisit the spin dynamics in the Earth-field-range magnetometry with the NLZ effect and identify the existence of the intrinsic spin squeezed state (SSS), generated from the coupling between nuclear and electron spins of each individual atom, with the oscillating squeezing degree and squeezing axis. Such oscillating features of the SSS prevent its direct observation and as well, accessibility to magnetic sensing. To exploit quantum advantage of the intrinsic SSS in the Earth-field-range magnetometry, it’s essential to lock the oscillating SSS to a persistent one. Hence we develop a quantum locking technique to achieve a persistent SSS, benefiting from which the sensitivity of the Earth-field-range magnetometer is quantum-enhanced. This work presents an innovative way turning the drawback of NLZ effect into the quantum advantage and opens a new access to quantum-enhanced magnetometry in the Earth-field range.
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Abstract Quantum metrology exploits quantum resources and strategies to improve measurement precision of unknown parameters. One crucial issue is how to prepare a quantum entangled state suitable for high-precision measurement beyond the standard quantum limit. Here, we propose a scheme to optimize the state preparation pulse sequence to accelerate the one-axis twisting dynamics for entanglement generation with the aid of deep reinforcement learning (DRL). We consider the pulse train as a sequence of π /2 pulses along one axis or two orthogonal axes, and the operation is determined by maximizing the quantum Fisher information using DRL. Within a limited evolution time, the ultimate precision bounds of the prepared entangled states follow the Heisenberg-limited scalings. These states can also be used as the input states for Ramsey interferometry and the final measurement precisions still follow the Heisenberg-limited scalings. While the pulse train along only one axis is more simple and efficient, the scheme using pulse sequence along two orthogonal axes show better robustness against atom number difference between simulation and experiment. Our protocol with DRL is efficient and easy to be implemented in state-of-the-art experiments.