Measurements with quantum limited resolution have important applications in metrology and sensing, including atomic clocks, atom interferometry, and magnetometry. We perform a quantum-non-demolition measurement on a collective angular momentum of a million spin-4 Cs atoms with high optical depth in our work. Quantum mechanics limits the measurement's resolution to what is known as the standard quantum limit (SQL) when there is no entanglement between the individual atoms. We can generate entanglement between atoms to create spin squeezed states through quantum backaction, improving the measurement sensitivity by 5.5 dB relative to the SQL. We have recently rebuilt the entire experiment inside a state-of-the-art magnetic shield of mu-metal and aluminum. This upgrade has drastically mitigated classical control errors in the spin squeezing experiment. Furthermore, the ensemble's sensitivity to magnetic fields allows us to make precise measurements of the magnetic field environment. Using closed-loop feedback, we use our atomic magnetometer to measure magnetic fields 4.3 dB below the SQL. The shielded environment will allow us to optimize the magnetometer and sets the stage for future experiments to use the closed-loop control to explore more complicated quantum dynamics.
Measurements with quantum limited resolution have important applications in metrology and sensing, including atomic clocks, atom interferometry, and magnetometry. We perform a quantum-non-demolition measurement on a collective angular momentum of a million spin-4 Cs atoms with high optical depth in our work. Quantum mechanics limits the measurement's resolution to what is known as the standard quantum limit (SQL) when there is no entanglement between the individual atoms. We can generate entanglement between atoms to create spin squeezed states through quantum backaction, improving the measurement sensitivity by 5.5 dB relative to the SQL. We have recently rebuilt the entire experiment inside a state-of-the-art magnetic shield of mu-metal and aluminum. This upgrade has drastically mitigated classical control errors in the spin squeezing experiment. Furthermore, the ensemble's sensitivity to magnetic fields allows us to make precise measurements of the magnetic field environment. Using closed-loop feedback, we use our atomic magnetometer to measure magnetic fields 4.3 dB below the SQL. The shielded environment will allow us to optimize the magnetometer and sets the stage for future experiments to use the closed-loop control to explore more complicated quantum dynamics.
Squeezing of collective atomic spins has been shown to improve the sensitivity of atomic clocks and magnetometers to levels significantly below the standard quantum limit. In most cases the requisite atom-atom entanglement has been generated by dispersive interaction with a quantized probe field or by state-dependent collisions in a quantum gas. Such experiments typically use complex multilevel atoms like Rb or Cs, with the relevant interactions designed so that atoms behave like pseudospin-21 particles. We demonstrate the viability of spin squeezing for collective spins composed of the physical angular momenta of 106 Cs atoms, each in an internal spin-4 hyperfine state. A peak metrological squeezing of at least 5dB is generated by quantum backaction from a dispersive quantum nondemolition (QND) measurement, implemented using a two-color optical probe that minimizes tensor light shifts without sacrificing measurement strength. Other significant developments include the successful application of composite pulse techniques for accurate dynamical control of the collective spin, enabled by broadband suppression of background magnetic fields inside a state-of-the-art magnetic shield. The absence of classical noise allows us to compare the observed quantum projection noise and squeezing to a theoretical model that properly accounts for both the relevant atomic physics and the spatial mode of the collective spin, finding good quantitative agreement and thereby validating its use in other contexts. Our work sets the stage for experiments on quantum feedback, deterministic squeezing, and closed-loop magnetometry. The implementation of real-time feedback may also create an opportunity for new types of quantum simulation, wherein the evolution of a quantum system is conditioned on the outcome of a time-continuous QND measurement. Such a scheme has the potential to access new regimes near the quantum-classical boundary, with opportunities to study long-standing issues related to quantum-classical correspondence in chaotic systems.
Quantum control of many body atomic spins is often pursued in the context of an atom-light quantum interface, where a quantized light field acts as a "quantum bus" that can be used to entangle distant atoms. One key challenge is to improve the coherence of the atom-light interface and the amount of atom-light entanglement it can generate, given the constraints of working with multilevel atoms and optical fields in a 3D geometry. We have explored new ways to achieve this, through rigorous optimization of the spatial geometry, and through control of the internal atomic state. Our basic setup consists of a quantized probe beam passing through an atom cloud held in a dipole trap, first generating spin-probe entanglement through the Faraday interaction, and then using backaction from a measurement of the probe polarization to squeeze the collective atomic spin. The relevant figure of merit is the metrologically useful spin squeezing determined by the enhancement in the resolution of rotations of the collective spin, relative to the commonly used spin coherent state. With an optimized free-space geometry, and by using a 2-color probe scheme to suppress tensor light shifts, we achieve 3(2) dB of metrologically useful spin squeezing. We can further increase atom-light coupling by implementing internal state control to prepare spin states with larger initial projection noise relative to the spin coherent state. Under the right conditions this increase in projection noise can lead to stronger measurement backaction and increased atom-atom entanglement. With further internal state control the increased atom-atom entanglement can then be mapped to a basis where it corresponds to improved squeezing of, e.g., the physical spin-angular momentum or the collective atomic clock pseudospin. In practice, controlling the collective spin of N ~ 10⁶ atoms in this fashion is an extraordinarily difficult challenge because errors in the control of individual atoms tend to be highly correlated. By employing precise internal state control, we have prepared and detected projection noise limited "cat" states (which have initial projection noise that is larger by a factor of 2f = 8 for Cs relative to the spin coherent state) and estimate that we can generate up to 6.0(5) dB of metrologically useful spin squeezing, demonstrating the advantage of using the internal atomic structure as a resource for ensemble control.
Atomic sensors are among the best devices for precision measurements of time, electric and magnetic fields, and inertial forces. However, all atomic sensors that utilise uncorrelated particles are ultimately limited by quantum projection noise, as is already the case for state-of-the-art atomic clocks. This so-called standard quantum limit (SQL) can be overcome by employing entanglement, a prime example being the spin-squeezed states. Spin squeezing can be produced in a quantum non-demolition (QND) measurement of the collective spin, particularly with cavity quantum electrodynamical (cQED) interactions. In this thesis, I present the second-generation trapped-atom clock on a chip (TACC) experiment, where we combine a metrology-grade compact clock with a miniature cQED platform to test quantum metrology protocols at a metrologically-relevant precision level. In a standard Ramsey spectroscopy, the stability of the apparatus is confirmed by a fractional frequency Allan deviation of 6E-13 at 1 s. We demonstrate spin squeezing by QND measurement, reaching 8(1) dB for 1.7E4 atoms, currently limited by decoherence due to technical noise. Cold collisions between atoms play an important role at this level of precision, leading to rich spin dynamics. Here we find that the interplay between cavity measurements and collisional spin dynamics manifests itself in a quantum amplification effect of the cavity measurement. A simple model is proposed, and is confirmed by initial measurements. New experiments in this direction may shed light on the surprising many-body physics in this sytem of interacting cold atoms.
Large ensembles of uncorrelated atoms are extensively used as precise sensors of time, rotation, and gravity, and for tests of fundamental physics. The quantum nature of the sensors imposes a limit on their ultimate precision. Larger ensembles of N atoms can be used to average the quantum noise as 1/√N, a scaling known as the standard quantum limit. However, the ensemble size may be limited by technical constraints and/or atom-atom collisions -- a fundamental distinction from photon-based sensors. Learning to prepare entangled states of large ensembles with noise properties below the standard quantum limit will be key to extending both the precision and/or bandwidth of atomic sensors. More broadly, the generation and application of entanglement to solve problems is a core goal of quantum information science being pursued in both atomic and solid state systems.\nIn this thesis, we utilize the tools of cavity-QED to prepare entangled spin-squeezed states with 3.4(6) dB improvement in spectroscopic sensitivity over the standard quantum limit. The collective atomic spin is composed of the two-level clock states of 87Rb confined in a medium finesse F = 710 optical cavity. We employ cavity-aided quantum non-demolition measurements of the vacuum Rabi splitting to measure and subtract out the quantum projection noise of the collective spin state, preparing states with collective atomic spin projection noise 4.9(6) dB below the projection noise level. The conditionally reduced spin noise combined with the measured 1.5(3) dB reduction in the mean spin length implies a net 3.4(6) dB spectroscopic enhancement or conditional squeezing as defined by the Wineland criterion. Our method does not require single particle addressability and is applied to a spectroscopically large ensemble of N = 7 x 105 atoms using two collective population measurements, with the whole squeezing operation taking ~ 150 μs. The gain in sensitivity is spectroscopically equivalent to the enhancement obtained had we created > 105 pairs of maximally entangled qubits, demonstrating the power of a top-down approach for entangling large ensembles. The nondemolition probing of atomic populations via the vacuum Rabi splitting is also of broad interest for non-destructively reading out a wide variety of both atomic and solid state qubits.
We demonstrate spin squeezing and entanglement in a large-spin system via quantum non-demolition measurement. We make non-destructive, projection-noise-limited collective spin measurements on an ensemble of up to in 8.4 × 105 laser-cooled 87Rb atoms in the f = 1 hyperfine ground state. A dynamically-decoupled probing scheme [Phys. Rev. Lett. 105, 093602 (2010)] prevents probe-induced decoherence. Repeated measurements show correlations beyond the standard quantum limit, indicating generation of a spin-squeezed state with up to −3.6 dB of noise reduction and −2.6 dB of metrologically-relevant squeezing.
Quantum metrology uses quantum features such as entanglement and squeezing to improve the sensitivity of quantum-limited measurements. Long established as a valuable technique in optical measurements such as gravitational-wave detection, quantum metrology is increasingly being applied to atomic instruments such as matter-wave interferometers, atomic clocks, and atomic magnetometers. Several of these new applications involve dual optical/atomic quantum systems, presenting both new challenges and new opportunities. Here we describe an optical magnetometry system that achieves both shot-noise-limited and projection-noise-limited performance, allowing study of optical magnetometry in a fully-quantum regime [1]. By near-resonant Faraday rotation probing, we demonstrate measurement-based spin squeezing in a magnetically-sensitive atomic ensemble [2-4]. The versatility of this system allows us also to design metrologically-relevant optical nonlinearities, and to perform quantum-noise-limited measurements with interacting photons. As a first interaction-based measurement [5], we implement a non-linear metrology scheme proposed by Boixo et al. with the surprising feature of precision scaling better than the 1/N “Heisenberg limit” [6].