Combining decoherence protection with directional photon emission in a single waveguide quantum electrodynamics (QED) device remains an open challenge. Here we show that an artificial giant molecule -- strongly interacting artificial atoms coupled to a photonic waveguide at multiple spatially separated points -- achieves both: a fully operational decoherence-free (DF) qubit and state-dependent chiral single-photon emission, arising from the same photon-interference mechanism. Initialization reduces to a local excitation of a single atom, universal single-qubit gates are implemented by modulating a single atomic frequency, and readout exploits state-dependent chiral emission with directionality reaching 100% and low measurement error of 1.2%. The coexistence of decoherence protection and directional emission in a single device positions giant molecules as protected chiral nodes for modular quantum networks in waveguide QED.
Combining decoherence protection with directional photon emission in a single waveguide quantum electrodynamics (QED) device remains an open challenge. Here we show that an artificial giant molecule -- strongly interacting artificial atoms coupled to a photonic waveguide at multiple spatially separated points -- achieves both: a fully operational decoherence-free (DF) qubit and state-dependent chiral single-photon emission, arising from the same photon-interference mechanism. Initialization reduces to a local excitation of a single atom, universal single-qubit gates are implemented by modulating a single atomic frequency, and readout exploits state-dependent chiral emission with directionality reaching 100% and low measurement error of 1.2%. The coexistence of decoherence protection and directional emission in a single device positions giant molecules as protected chiral nodes for modular quantum networks in waveguide QED.
We study chiral and nonreciprocal single-photon scattering in a chiral-giant-molecule waveguide-QED system. Here, the giant molecule consists of two coupled giant atoms, which interact with two linear waveguides, forming a four-port quantum device. We obtain the exact analytical expressions of the four scattering amplitudes using a real-space method. Under the Markovian limit, we find that the single-photon scattering behavior is determined by the coupling strength between the giant atoms and the waveguides, the coupling strength between the two giant atoms, and the nondipole effect caused by the phase accumulation of photons traveling between the coupling points. It is also found that chiral and nonreciprocal single-photon scattering can be realized by introducing the chiral coupling to break the symmetry in the coupling configuration between the giant molecule and the waveguides. In addition, an ideal chiral emitter-waveguide coupling enables a directional single-photon routing. In the non-Markovian regime, the scattering spectra are characterized by more abundant structures with multiple peaks and dips. In particular, we demonstrate that the non-Markovian retarded effect can induce the nonreciprocal single-photon scattering. Our results have potential applications in the design of optical quantum devices involving giant atoms, which can provide an efficient platform for studying chiral quantum optics.
In this paper, we present an in-depth examination of single-photon routing in a multi-emitter waveguide quantum electrodynamics ladder with up to five giant atoms simultaneously coupled across two linear waveguides. Using a real-space approach, we analyze a non-chiral routing architecture and evaluate the impact of scaling the number of giant atoms in three topologically distinct configurations: fully separated, simply braided, and fully nested. Using numerical results, we show that increasing the number of giant atoms, in separate or braided configurations, greatly expands the operational parameter space for near-deterministic ($\sim$100%) photon routing into the target waveguide, achieving directionality through quantum interference alone. In contrast, the nested architecture is limited to a maximum routing efficiency of 25% due to rigid geometric symmetries, although this limitation could be mitigated by employing less symmetric coupling distances. Finally, we assess the system under direct interatomic interactions and environmental dissipation. Our results show that, while spontaneous emission reduces transport probabilities, the multi-atom-separated configuration maintains high routing efficiencies across broad operational windows of incoming photon frequency without requiring chiral coupling.
Radiative coupling between quantum emitters leads to a range of spectacular emission phenomena. Dicke studied the foundations of collectively enhanced and suppressed decay, commonly referred to as super- and subradiance. Collective effects can further result in directionality of the emission, thus offering a complimentary implementation of chiral quantum optics. Waveguide quantum electrodynamics (QED) allows coupling between spatially separated emitters, enabling selective driving. In this work, we control the emission direction for a pair of quantum dots embedded in a bidirectional photonic crystal waveguide offering independent electrical tuning. Notably the emitters are 13 \micro m apart, which corresponds to 26 effective wavelengths, but are nevertheless radiatively coupled. The directionality arises from a dispersive dipole-dipole interaction, which shifts the energy of the collective states, so that the emitter pair effectively forms an artificial molecule. We show that the emission direction can be switched from left- to rightwards by manipulating the relative driving phase while collectively exciting the emitters. In addition, we observe directional photon statistics under continuous driving, with, for example, single photons detected on one output port, and photon pairs on the other. With pulsed excitation, both emitters are fully inverted and correlated photon pairs are observed in time-resolved intensity correlation measurements. This work demonstrates a novel implementation of chiral quantum optics using quantum dots coupled via a non-chiral waveguide, and reports key steps for scaling up as a multi-emitter waveguide QED platform.
In quantum-optics experiments with both natural and artificial atoms, the atoms are usually small enough that they can be approximated as pointlike compared to the wavelength of the electromagnetic radiation with which they interact. However, superconducting qubits coupled to a meandering transmission line, or to surface acoustic waves, can realize "giant artificial atoms" that couple to a bosonic field at several points which are wavelengths apart. Here, we study setups with multiple giant atoms coupled at multiple points to a one-dimensional (1D) waveguide. We show that the giant atoms can be protected from decohering through the waveguide, but still have exchange interactions mediated by the waveguide. Unlike in decoherence-free subspaces, here the entire multiatom Hilbert space (2^{N} states for N atoms) is protected from decoherence. This is not possible with "small" atoms. We further show how this decoherence-free interaction can be designed in setups with multiple atoms to implement, e.g., a 1D chain of atoms with nearest-neighbor couplings or a collection of atoms with all-to-all connectivity. This may have important applications in quantum simulation and quantum computing.
Experiments utilizing quantum optics have progressed rapidly in last few decades, particularly in the context of quantum computation, simulation, and communication. Early work in this field focused on implementations of cavity quantum electrodynamics (QED), where atoms, either natural or artificial, are strongly coupled to the confined photonic modes of cavities. However, in recent years, achieving strong coupling between atoms and itinerant photons has also gained significant interest for its applications in quantum networking. To this end, many atomic platforms are attempting to realize the waveguide QED architecture: atoms that interact with the continua of propagating photonic modes within a waveguide. In this thesis, we realize the strong-coupling regime of a waveguide QED architecture by coupling superconducting artificial atoms, typically operated as qubits, to one-dimensional transmission lines. We first demonstrate that superconducting qubits in a waveguide QED system can be used as high-quality quantum emitters. We then leverage the quantum interference between the simultaneous emission from multiple qubits in order to generate non-classical, spatially entangled, and directional itinerant microwave photons. These types of photons are particularly useful for remote entanglement and quantum communication protocols. Finally, we demonstrate that superconducting qubits can be engineered to enter novel regimes of light-matter interactions that are difficult, or even impossible, to achieve in other atomic platforms. In particular, we realize the giant-atom regime of waveguide QED, where the atom can no longer be treated as a point-like object. We use our giant atoms to implement tunable atom-waveguide couplings, as well as decoherence-free waveguide-mediated interactions between multiple atoms.
We investigate single-photon scattering in a waveguide-QED setup, where a giant molecule composed of two frequency-detuned giant atoms is coupled to two parallel waveguides via multiple connection points. The competition between coherent atom--atom coupling and the effective decay rates dictates the splitting of a single resonance into a doublet in the transmission (reflection) spectra. By tailoring the asymmetry of the decay rates and the atomic detuning, one can engineer photon-path interference to optimize the transfer between waveguides; under chiral coupling conditions, this interference can be further harnessed to realize fully deterministic routing. In the non-Markovian regime, retardation effects can reshape the spectra and actively drive transitions between the weak- and strong-coupling regimes, converting an unsplit Markovian resonance into a clearly separated doublet, or conversely merging a split doublet back into a single resonance. For sufficiently long time delays, it further generates multiple resonances and avoided crossings, enriching the spectral response. Our results demonstrate how atomic detuning, decay-rate asymmetry, and non-Markovian retardation cooperate to provide versatile, interference-based control over single-photon routing in multi-port quantum networks.