Lasers serve as the fundamental workhorses of photonic quantum technologies, with perfectly coherent light fields being essential for many protocols that generate nonclassical light, implement coherent control schemes, and initialize qubits. However, no laser is absolutely ideal and the implications of deviations from perfect coherence in quantum technological tasks remain unclear. In this study, we theoretically and experimentally explore the quantum coherence properties of lasers from a resource theory perspective, establishing a significant connection between photonics, quantum optics, and quantum information science. We demonstrate that the maximum achievable quantum coherence for laser light is constrained by spontaneous emission and the purity of the dephased laser field state. As a critical example application in quantum information protocols, we show that the quantum coherence of a laser field with a given mean photon number directly governs the maximum purity attainable when initializing a qubit in a superposition state through resonant driving. Our findings are highly relevant for bridging applied physics and engineering with integrated photonic quantum technologies and resource theories, paving the way for reliable benchmarking of various coherent light sources for applications in photonics and quantum protocols.
Lasers serve as the fundamental workhorses of photonic quantum technologies, with perfectly coherent light fields being essential for many protocols that generate nonclassical light, implement coherent control schemes, and initialize qubits. However, no laser is absolutely ideal and the implications of deviations from perfect coherence in quantum technological tasks remain unclear. In this study, we theoretically and experimentally explore the quantum coherence properties of lasers from a resource theory perspective, establishing a significant connection between photonics, quantum optics, and quantum information science. We demonstrate that the maximum achievable quantum coherence for laser light is constrained by spontaneous emission and the purity of the dephased laser field state. As a critical example application in quantum information protocols, we show that the quantum coherence of a laser field with a given mean photon number directly governs the maximum purity attainable when initializing a qubit in a superposition state through resonant driving. Our findings are highly relevant for bridging applied physics and engineering with integrated photonic quantum technologies and resource theories, paving the way for reliable benchmarking of various coherent light sources for applications in photonics and quantum protocols.
The goal of this work is to examine the coherence of classical light fields in order to assess their usefulness for quantum-informational tasks and to draw conclusions about the properties of the light source. To this end, we use and extend several optical homodyne tomography techniques employing four-port, eight-port, and sixteen-port detection schemes. To understand the role of coherence of a light field in solving a quantum informational task such as coherent qubit control, we begin by analyzing the qubit excitation process from a resource-theoretical perspective. By simulating the light-matter interactions, we demonstrate how the quantum coherence of the driving light field emerges as a key ingredient for coherent qubit control. At the same time, we show how the presence of thermal noise or dephasing significantly degrades the achievable quantum coherence of the light field. After studying the coherence properties of conventional lasers, we turn to non-conventional coherent light sources and investigate the emission of a non-resonantly excited exciton-polariton condensate. By employing long-lived polaritons and minimizing interactions with the reservoir, we optimize the condensation process and achieve a pronounced buildup of quantum superpositions in the condensate immediately above the condensation threshold. Finally, we shift our focus entirely to the matter system itself and use the coherence of the emitted light field to investigate its dynamics. For this purpose, we introduce a sixteen-port detection scheme that enables non-stationary and conditional analyses tailored to the requirements of semiconductor spectroscopy. Benchmarking the setup with a thermal light field, then demonstrate how we can resolve the stochastic fluctuations of the thermal state on the femtosecond level. Overall, our results establish connections between quantum optics, quantum information science, and semiconductor physics, providing insights relevant for quantum technologies and future hybrid quantum devices.
Strong-laser-field physics is a research direction that relies on the use of high-power lasers and has led to fascinating achievements ranging from relativistic particle acceleration to attosecond science. On the other hand, quantum optics has been built on the use of low photon number sources and has opened the way for groundbreaking discoveries in quantum technology, advancing investigations ranging from fundamental tests of quantum theory to quantum information processing. Despite the tremendous progress, until recently these directions have remained disconnected. This is because the majority of the interactions in the strong-field limit have been successfully described by semi-classical approximations treating the electromagnetic field classically, as there was no need to include the quantum properties of the field to explain the observations. The link between strong-laser-field physics, quantum optics, and quantum information science has been developed in the recent past. Studies based on fully quantized and conditioning approaches have shown that intense laser-matter interactions can be used for the generation of controllable entangled and non-classical light states. These achievements open the way for a vast number of investigations stemming from the symbiosis of strong-laser-field physics, quantum optics, and quantum information science. Here, after an introduction to the fundamentals of these research directions, we report on the recent progress in the fully quantized description of intense laser-matter interaction and the methods that have been developed for the generation of non-classical light states and entangled states. Also, we discuss the future directions of non-classical light engineering using strong laser fields, and the potential applications in ultrafast and quantum information science.
Nonclassical states of light and their correlations lie at the heart of quantum optics, serving as fundamental resources that underpin both the exploration of quantum phenomena and the realisation of quantum information protocols. These lecture notes provide an accessible yet rigorous introduction to the foundations of quantum optics, emphasising their relevance to quantum information science and technology. Starting from the quantisation of the electromagnetic field and the bosonic formalism of Fock space, the notes develop a unified framework for describing and analysing quantum states of light. Key families of states -- thermal, coherent, and squeezed -- are introduced as paradigmatic examples illustrating the transition from classical to nonclassical behaviour. The concepts of convexity, classicality, and quasiprobability representations are presented as complementary tools for characterising quantumness and defining operational notions such as P-nonclassicality. The discussion extends naturally to Gaussian states, composite systems, and continuous-variable entanglement, highlighting how nonclassicality serves as a resource for generating and quantifying quantum correlations. Theoretical developments are complemented by computational and experimental perspectives, including simulations of optical states using the Python library Strawberry Fields and data analysis from simulated data. Together, these notes aim to bridge the foundational concepts of quantum optics and modern quantum information, offering both conceptual insight and practical tools for students and researchers entering the field.
The resource theory of quantum coherence studies the off-diagonal elements of a density matrix in a distinguished basis, whereas the resource theory of purity studies all deviations from the maximally mixed state. We establish a direct connection between the two resource theories, by identifying purity as the maximal coherence which is achievable by unitary operations. The states that saturate this maximum identify a universal family of maximally coherent mixed states. These states are optimal resources under maximally incoherent operations, and thus independent of the way coherence is quantified. For all distance-based coherence quantifiers the maximal coherence can be evaluated exactly, and is shown to coincide with the corresponding distance-based purity quantifier. We further show that purity bounds the maximal amount of entanglement and discord that can be generated by unitary operations, thus demonstrating that purity is the most elementary resource for quantum information processing.
Intense laser-matter interactions are at the center of interest in research and technology since the development of high-power lasers.They have been widely used for fundamental studies in atomic, molecular, and optical physics, and they are at the core of attosecond physics and ultrafast optoelectronics.Although the majority of these studies have been successfully described using classical electromagnetic fields, recent investigations based on fully quantized approaches have shown that intense laser-atom interactions can be used for the generation of controllable high-photon-number entangled coherent states and coherent state superpositions.In this tutorial, we provide a comprehensive fully quantized description of intense laseratom interactions.We elaborate on the processes of high-harmonic generation, above-threshold ionization, and we discuss new phenomena that cannot be revealed within the context of semiclassical theories.We provide the description for conditioning the light field on different electronic processes, and their consequences for quantum state engineering of light.Finally, we discuss the extension of the approach to more complex materials, and the impact to quantum technologies for a new photonic platform composed of the symbiosis of attosecond physics and quantum information science.
High-harmonic generation is one of the most fundamental processes in strong laser-field physics that has led to countless achievements in atomic physics and beyond. However, a rigorous quantum electrodynamical picture of the process has never been reported. Here, we prove rigorously and demonstrate experimentally that the quantum state of the driving laser field, as well as that of harmonics, is coherent. Projecting this state on its part corresponding to harmonic generation, it becomes a superposition of a state, amplitude-shifted due to the quantum nature of light, and the initial state of the laser. This superposition interpolates between a Schrodinger kitten, and a genuine Schrodinger cat state. This work opens new paths for ground-breaking investigations in strong laser-field physics and quantum technology. We dedicate the work to the memory of Roy J. Glauber, the inventor of coherent states.