High-harmonic generation is one of the most fundamental processes in strong laser-field physics that has led to countless achievements in atomic physics and beyond. However, a rigorous quantum electrodynamical picture of the process has never been reported. Here, we prove rigorously and demonstrate experimentally that the quantum state of the driving laser field, as well as that of harmonics, is coherent. Projecting this state on its part corresponding to harmonic generation, it becomes a superposition of a state, amplitude-shifted due to the quantum nature of light, and the initial state of the laser. This superposition interpolates between a Schrodinger kitten, and a genuine Schrodinger cat state. This work opens new paths for ground-breaking investigations in strong laser-field physics and quantum technology. We dedicate the work to the memory of Roy J. Glauber, the inventor of coherent states.
High-harmonic generation is one of the most fundamental processes in strong laser-field physics that has led to countless achievements in atomic physics and beyond. However, a rigorous quantum electrodynamical picture of the process has never been reported. Here, we prove rigorously and demonstrate experimentally that the quantum state of the driving laser field, as well as that of harmonics, is coherent. Projecting this state on its part corresponding to harmonic generation, it becomes a superposition of a state, amplitude-shifted due to the quantum nature of light, and the initial state of the laser. This superposition interpolates between a Schrodinger kitten, and a genuine Schrodinger cat state. This work opens new paths for ground-breaking investigations in strong laser-field physics and quantum technology. We dedicate the work to the memory of Roy J. Glauber, the inventor of coherent states.
Recently we have demonstrated the quantum nature of light in strongly laser driven atoms, and we have shown how the process of high harmonic generation can be used for the creation of highly non-classical light states, in particular superpositions of two coherent states, i.e., optical Schr\{o}dinger states [M. Lewenstein et al., Generation of optical Schr\odinger cat states in intense laser-matter interactions, Nat. Phys., 17 1104-1108 (2021)]. Here, we investigate the quantum optical description of the interaction, incorporating many atoms and the back-action of the high harmonic generation or above threshold ionization processes on the coherent state of the driving laser field. We show how the conditioning on high harmonic generation and above threshold ionization can lead to non-classical light states, and we discuss the key parameters that can be used for controlling and characterizing the non-classical states obtained after high harmonic generation. The theoretical results have been experimentally confirmed by demonstrating how the obtained coherent state superposition changes from an optical to kitten state by changing the number of atoms participating in the high harmonic generation process. Additionally, we experimentally verify the applicability of the approach for generating high photon number non-classical light states. This is shown by demonstrating the generation of a 9--photon optical state which, to our knowledge, is the highest photon number optical state experimentally reported. Our findings anticipate the development of new methods that naturally lead to the creation of high photon number controllable coherent state superpositions, advancing investigations in quantum technology.
Strong laser-atom interactions can produce highly non-classical states of light by using the process of high-harmonic generation in atoms. When the high-harmonic generation is present, the quantum state of the fundamental mode following the interaction is known as the Schrödinger cat state, which is a superposition of the laser’s initial coherent state and the coherent state with a smaller amplitude that results from its interaction with atoms. Here, we demonstrate that new light states with significantly different Wigner function distributions can be produced by combining two separate Schrödinger cat states. Through the engineering of Schrödinger cat states’ parameters, we are able to produce Wigner functions that exhibit high sensitivity in relation to the system parameter. Our research paves the way for the creation of non-classical light by superposing Schrödinger cat states with application in such as quantum sensing.
Strong laser-atom interactions can produce highly non-classical states of light by using the process of high-harmonic generation in atoms. When the high-harmonic generation is present, the quantum state of the fundamental mode following the interaction is known as the Schrödinger cat state, which is a superposition of the laser's initial coherent state and the coherent state with a smaller amplitude that results from its interaction with atoms. Here, we demonstrate that new light states with significantly different Wigner function distributions can be produced by combining two separate Schrödinger cat states. Through the engineering of Schrödinger cat states' parameters, we are able to produce Wigner functions that exhibit high sensitivity in relation to the system parameter. Our research paves the way for the creation of non-classical light by superposing Schrödinger cat states with application in such as quantum sensing.
Strong laser-atom interactions can produce highly non-classical states of light by using the process of high-harmonic generation in atoms. When the high-harmonic generation is present, the quantum state of the fundamental mode following the interaction is known as the Schrödinger cat state, which is a superposition of the laser’s initial coherent state and the coherent state with a smaller amplitude that results from its interaction with atoms. Here, we demonstrate that new light states with significantly different Wigner function distributions can be produced by combining two separate Schrödinger cat states. Through the engineering of Schrödinger cat states’ parameters, we are able to produce Wigner functions that exhibit high sensitivity in relation to the system parameter. Our research paves the way for the creation of non-classical light by superposing Schrödinger cat states with application in such as quantum sensing.
High-harmonic generation is a light up-conversion process occurring in a strong laser field, leading to coherent bursts of extreme ultrashort broadband radiation [Lewenstein , Phys. Rev. A , 2117 (1994)]. As a new perspective, we propose that ultrafast strong-field electronic or photonic processes such as high-harmonic generation can potentially generate nonclassical states of light well before the decoherence of the system occurs [Gorlach , Nat. Commun. , 4598 (2020); Stammer ., Phys. Rev. Lett. , 123603 (2022)]. This could address fundamental challenges in quantum technology such as scalability, decoherence, or the generation of massively entangled states [Lewenstein , Luca Argenti Michael Chini, 27 (2024)]. Here, we report experimental evidence of the nonclassical nature of the harmonic emission in several semiconductors excited by a femtosecond infrared laser. By investigating single- and double-beam intensity cross-correlation [Loudon, Rep. Prog. Phys. , 913 (1980)], we measure characteristic nonclassical features in the single-photon statistics. We observe two-mode squeezing in the generated harmonic radiation, which depends on the laser intensity that governs the transition from super-Poissonian to Poissonian photon statistics. The measured violation of the Cauchy-Schwarz inequality realizes a direct test of multipartite entanglement in high-harmonic generation [Wasak, Phys. Rev. A , 033616 (2014)]. This result is supported by the theory of multimodal detection and the Hamiltonian from which the effective squeezing modes of the harmonics can be derived [Gonoskov , Phys. Rev. B , 125110 (2024); Christ New J. Phys. , 033027 (2011)]. With this work, we show experimentally that high-harmonic generation is a new quantum bosonic platform that intrinsically produces nonclassical states of light with unique features such as multipartite broadband entanglement or multimode squeezing. The source operates at room temperature, using standard semiconductors and a standard commercial fiber laser, opening up new routes for the quantum industry, such as optical quantum computing, communication, and imaging. Published by the American Physical Society 2024
High-harmonic generation (HHG) provides a powerful platform for exploring the interaction between intense laser fields and matter on ultrafast timescales. Beyond its conventional description in terms of emitted radiation and electron dynamics, a fully quantum treatment of HHG reveals that the nonlinear light-matter interaction can modify the quantum state of the driving field itself, establishing correlations between the fundamental and harmonic modes. This perspective opens new possibilities for using HHG as a tool to engineer and control nonclassical states of light. In this work, we investigate the geometric properties of optical Schroedinger cat states generated in HHG via conditioning and post-selection. By analyzing the coherent-state displacements induced by different structured driving fields, we characterize the resulting phase-space evolution and the associated geometric phases of the generated quantum states. Particular emphasis is placed on how the polarization and spatial-mode structure of the driving light influence the geometry and evolution of displaced coherent states. Our results demonstrate that structured light offers a versatile means of controlling the geometric dynamics of HHG-generated cat states across the parameter space. Furthermore, we discuss the prospects for realizing genuinely topological optical cat states by exploiting more complex structured light configurations.