The recent demonstrations of cascaded PDC (CPDC) and the hopeful prospects of realizing third-order PDC (TOPDC) for the generation of three-photon entangled states are paving the way for experimental studies on genuine three-photon interference. In this article, we formulate three-photon interference in terms of ``each three-photon interfering only with itself.'' We show that although a generalized two-alternative three-photon interference setup based on CPDC or TOPDC involves eight different length parameters, the interference can be fully characterized in terms of only three independent parameters. The first parameter is the three-photon path-length difference, which has a direct analog in the one-photon and two-photon cases, and the other two parameters quantify the path-asymmetry length. Unlike two-photon interference, which requires only one parameter to quantify path-asymmetry, two independent parameters are needed in three-photon interference. This results in a broader class of nonclassical three-photon effects, including three-photon HOM-type effects. Our work provides the theoretical basis for existing and future three-photon interference experiments exploring the rich and complex quantum correlations associated with three-particle entanglement and potentially enabling the development of novel protocols for harnessing those correlations.
The recent demonstrations of cascaded PDC (CPDC) and the hopeful prospects of realizing third-order PDC (TOPDC) for the generation of three-photon entangled states are paving the way for experimental studies on genuine three-photon interference. In this article, we formulate three-photon interference in terms of ``each three-photon interfering only with itself.'' We show that although a generalized two-alternative three-photon interference setup based on CPDC or TOPDC involves eight different length parameters, the interference can be fully characterized in terms of only three independent parameters. The first parameter is the three-photon path-length difference, which has a direct analog in the one-photon and two-photon cases, and the other two parameters quantify the path-asymmetry length. Unlike two-photon interference, which requires only one parameter to quantify path-asymmetry, two independent parameters are needed in three-photon interference. This results in a broader class of nonclassical three-photon effects, including three-photon HOM-type effects. Our work provides the theoretical basis for existing and future three-photon interference experiments exploring the rich and complex quantum correlations associated with three-particle entanglement and potentially enabling the development of novel protocols for harnessing those correlations.
Earth, Moon and Sun unite when they star together in the three-body problem, whose intricate plot still baffles us today. For some reason, the factorization of the two-body problem into two one-body problems does not, in general, cross the N=2 border. Is computational irreducibility responsible for this emergence of complexity, as Stephen Wolfram likes to think? We don't know. The introduction to this thesis in Chapter 1, however, makes it clear that the history of science is marked by intermittent encounters of sudden complexities when the number 2 is left behind. In Chapter 2, I present an experiment that is quite similar in spirit, for my colleagues and I observe three-photon interference without two-photon and single-photon interference. We had to overcome significant experimental challenges that are typical for most quantum interference experiments involving more than two photons. Next in line is the three-slit interference experiment. Again a deceptively simple extension of the famous double-slit experiment, we are faced with questions that are difficult to access experimentally: the existence of genuine three-slit interference was first denied and then affirmed, though no experiment has decided yet. My contribution to the study of this problem is outlined in Chapter 3, where I use symmetry of measurement settings in such interference experiments to theoretically derive higher-order interference terms. In Chapter 4, I take a step back in one sense, for we study a two-photon phenomenon, but we also leap forward and discover entirely new interference landscapes. Theoretically and experimentally, I demonstrate how to use a polarization-modulated lasers to go beyond the standard Hong-Ou-Mandel (HOM) dip, and generate both triangular and square wave HOM interference patterns. Two-photon interference is also subject of Chapter 5, but with an interesting twist. While laser HOM interference relies on two independent photons, here we endow the pair with the strongest known correlations, namely entanglement. More specifically, we entangle a polarization and a time-bin qubit and use this hybrid to assess the viability of a rather special interferometer for quantum communication purposes.
We show that temporal two-photon interference effects involving the signal and idler photons created by parametric down-conversion can be fully characterized in terms of the variations of two length parameters---called the biphoton path-length difference and the biphoton path-asymmetry-length difference---which we construct using the six different length parameters that a general two-photon interference experiment involves. We perform an experiment in which the effects of the variations of these two parameters can be independently controlled and studied. In our experimental setup, which does not involve mixing of signal and idler photons at a beam splitter, we further report observations of Hong-Ou-Mandel- (HOM-)like effects both in coincidence and in one-photon count rates. As an important consequence, we argue that the HOM and the HOM-like effects are best described as observations of how two-photon coherence changes as a function of the biphoton path-asymmetry-length difference.
In this work I demonstrate the interference of three photons, a generalisation of the famous Hong Ou Mandel (HOM) interference. I show that three-photon interference is governed by four parameters and measure three-photon interference independent of two-photon interference. I demonstrate that even when the states of the photons are highly distinguishable they can still exhibit strong quantum interference, challenging our intuition formed by the double slit and HOM interference. This is followed by a demonstration of four-photon interference, where surprisingly we can still observe a "fringe" when the involved particles are pairwise orthogonal. To explain these effects, I present a new framework to describe multi-photon interference in terms of a graph-theoretical approach, which illustrates the origin of different orders of multi-photon interference. My work leads to a more general definition of what we regard as an interference fringe in multi-photon scattering. This study of multi-photon interference is followed by an interdisciplinary work between photonics and solid state physics in the newly developing field of topological photonics. I realise a simulation of the Jackiw-Rossi model as a localised topological mode in a photonic-crystal analogue of the 2D graphene lattice. I succeed in the experimental demonstration of a single such excitation and I am able to study the detailed mode structure for the first time. The mode is a result of a topological defect and is, as such, protected against errors that do not change the topology of the system.
Quantum interference of two independent particles in pure quantum states is fully described by the particles' distinguishability: the closer the particles are to being identical, the higher the degree of quantum interference. When more than two particles are involved, the situation becomes more complex and interference capability extends beyond pairwise distinguishability, taking on a surprisingly rich character. Here, we study many-particle interference using three photons. We show that the distinguishability between pairs of photons is not sufficient to fully describe the photons' behavior in a scattering process, but that a collective phase, the triad phase, plays a role. We are able to explore the full parameter space of three-photon interference by generating heralded single photons and interfering them in a fiber tritter. Using multiple degrees of freedom-temporal delays and polarization-we isolate three-photon interference from two-photon interference. Our experiment disproves the view that pairwise two-photon distinguishability uniquely determines the degree of nonclassical many-particle interference.
Quantum interference of two independent photons in pure quantum states is fully described by the particles' distinguishability: the closer the particles are to being identical, the higher the degree of quantum interference. When more than two particles are involved, the situation becomes more complex and interference capability extends beyond pairwise distinguishability. Here, we study many-particle interference using three photons. We show that the three distinct distinguishabilities between pairs of photons are not sufficient to fully describe the photons' behaviour in a scattering process, but that additionally a fourth parameter, a collective phase, governs the scattering process. We use heralded single photons and a fibre-optic tritter to explore this full parameter space for the first time and thereby demonstrate genuine three-photon interference. Further, our work challenges the view that using time delays between identical photons alone suffices to fully study multi-photon interference.
A number of recent interference experiments involving multiple photons are reviewed. These experiments include generalized photon bunching effects, generalized Hong-Ou-Mandel interference effects and multi-photon interferometry for demonstrations of multi-photon de Broglie wavelength. The multi-photon states used in these experiments are from two pairs of photons in parametric down-conversion. We find that the size of the interference effect in these experiments, characterized by the visibility of the interference pattern, is governed by the degree of distinguishability among different pairs of photons. Based on this discovery, we generalize the concept of multi-photon temporal distinguishability and relate it to a number of multi-photon interference effects. Finally, we make an attempt to interpret the coherence theory by multi-photon interference via the concept of temporal distinguishability of photons.