Quantum interference of two independent particles in pure quantum states is fully described by the particles' distinguishability: the closer the particles are to being identical, the higher the degree of quantum interference. When more than two particles are involved, the situation becomes more complex and interference capability extends beyond pairwise distinguishability, taking on a surprisingly rich character. Here, we study many-particle interference using three photons. We show that the distinguishability between pairs of photons is not sufficient to fully describe the photons' behavior in a scattering process, but that a collective phase, the triad phase, plays a role. We are able to explore the full parameter space of three-photon interference by generating heralded single photons and interfering them in a fiber tritter. Using multiple degrees of freedom-temporal delays and polarization-we isolate three-photon interference from two-photon interference. Our experiment disproves the view that pairwise two-photon distinguishability uniquely determines the degree of nonclassical many-particle interference.
Quantum interference of two independent particles in pure quantum states is fully described by the particles' distinguishability: the closer the particles are to being identical, the higher the degree of quantum interference. When more than two particles are involved, the situation becomes more complex and interference capability extends beyond pairwise distinguishability, taking on a surprisingly rich character. Here, we study many-particle interference using three photons. We show that the distinguishability between pairs of photons is not sufficient to fully describe the photons' behavior in a scattering process, but that a collective phase, the triad phase, plays a role. We are able to explore the full parameter space of three-photon interference by generating heralded single photons and interfering them in a fiber tritter. Using multiple degrees of freedom-temporal delays and polarization-we isolate three-photon interference from two-photon interference. Our experiment disproves the view that pairwise two-photon distinguishability uniquely determines the degree of nonclassical many-particle interference.
Quantum interference of two independent photons in pure quantum states is fully described by the particles' distinguishability: the closer the particles are to being identical, the higher the degree of quantum interference. When more than two particles are involved, the situation becomes more complex and interference capability extends beyond pairwise distinguishability. Here, we study many-particle interference using three photons. We show that the three distinct distinguishabilities between pairs of photons are not sufficient to fully describe the photons' behaviour in a scattering process, but that additionally a fourth parameter, a collective phase, governs the scattering process. We use heralded single photons and a fibre-optic tritter to explore this full parameter space for the first time and thereby demonstrate genuine three-photon interference. Further, our work challenges the view that using time delays between identical photons alone suffices to fully study multi-photon interference.
Quantum interference constitutes one of the sharpest divides between our classical intuition and the weirdness of the quantum world. Whenever there are multiple paths leading to the same outcome, it is the interplay of associated probability amplitudes that determines measurement results. In the double slit experiment, wave-like interference governs the distribution of particles on a detection screen. Extending to multiple particles allows behaviour that cannot be described by a classical wave, such as the bunching of photon pairs in Hong-Ou-Mandel interference. In both these examples, the ability to distinguish the interfering paths leads to degradation of interference and a return to behaviour described by probabilities. Understanding how this transition evolves for larger multiparticle quantum systems is of fundamental interest and also vital for developing photonic quantum technologies that rely on many-photon interference. In this thesis we investigate the role of distinguishability in the interference of three and four independent photons by using polarisation and time delays. For three photons, a new type of collective distinguishing phase appears that goes beyond a pairwise description of the similarity of quantum states. We use nonlinear photon sources and a fibre interferometer to experimentally demonstrate the ability to tune and isolate this phase in interference statistics. Extending to four photons we show that, contrary to intuition from two-photon experiments, the interference of photons prepared in distinguishable states is possible due to a four-particle phase. This is confirmed experimentally using a bulk four-mode interferometer. We then extend our study to include the effects of state impurity in the interference of three photons. New properties of this interference enable diagnosis of realistic experimental imperfections and characterisation tasks impossible using only two photons. Finally, we link discussions of state distinguishability to the group representations underpinning the exchange symmetry of multiparticle wavefunctions.
To describe how distinguishability affects multiparticle interference of identical bosons (or fermions) is an important fundamental problem. We propose a solution based the weighted graph theory. We show, for instance, that quantum interference of N independent identical particles with no pair of them being in orthogonal internal states is governed by (N−1)(N−2)/2 independent triad phases, i.e., no genuine N-particle interference, beyond the three-particle interference recently observed, exists with N≥4 partially distinguished particles. Surprisingly, deterministic distinguishability, preventing quantum interference with two or three particles, can break this rule: setting each particle to be deterministically distinguishable from all others except two, one can switch off the R-particle interference for 3≤R≤N−1, whereas leaving switched on a novel (circle-dance) interference of N≥4 particles due to the Nth order quantum correlations. Our results can be useful in quantum computation, quantum information, and quantum metrology with single photons.
We study the impact of distinguishability and mixedness, two fundamental properties of quantum states, on quantum interference. We show that these can influence the interference of multiple particles in different ways, leading to effects that cannot be observed in the interference of two particles alone. This is demonstrated experimentally by interfering three independent photons in pure and mixed states and observing their different multiphoton interference, despite exhibiting the same two-photon Hong-Ou-Mandel interference. In addition to its fundamental relevance, our observation has important implications for quantum technologies relying on photon interference.
We introduce collective geometric phases of bosons and fermions interfering on a linear unitary multiport, where each phase depends on the internal states of identical particles (i.e., not affected by the multiport) and corresponds to a cycle of the symmetric group. We show that quantum interference of N particles in generic pure internal states, i.e., with no pair being orthogonal, is governed by $(N\ensuremath{-}1)(N\ensuremath{-}2)/2$ independent triad phases (each involving only three particles). The deterministic distinguishability, preventing quantum interference with two or three particles, allows for the genuine $(N\ensuremath{\ge}4)$-particle phase (interference) on a multiport: setting each particle to be deterministically distinguishable from all others except two by their internal states allows for a novel (circle-dance) interference of $N\ensuremath{\ge}4$ particles governed by a collective N-particle phase, while simultaneously preventing the R-particle interference for $3\ensuremath{\le}R\ensuremath{\le}N\ensuremath{-}1$. The genuine N-particle interference manifests the Nth-order quantum correlations between identical particles at a multiport output; it does not appear in the marginal probability for a subset of the particles, e.g., it cannot be detected if at least one of the particles is lost. This means that the collective phases are not detectable by the usual ``quantumness'' criteria based on the second-order quantum correlations. The results can be useful for quantum computation, quantum information, and other quantum technologies with single photons.
Abstract Quantum interference is known to become extinct with distinguishing information, as illustrated by the ubiquitous double-slit experiment or the two-photon Hong–Ou–Mandel effect. In the former case single particle interference is destroyed with which-path information while in the latter bunching interference tails-off as photons become distinguishable. It has been observed that when more than two particles are involved, these interference patterns are in general a non-monotonic function of the distinguishability. Here we perform a comprehensive characterization, both theoretically and experimentally, of four-photon interference by analyzing the corresponding correlation functions, contemplating several degrees of distinguishability across different parameters. This study provides all the necessary tools to quantify the impact of multi-photon interference on precision measurements of parameters such as phase, frequency, and time difference. We apply these insights to quantify the precision in the estimation of an interferometric phase in a two-port interferometer using a four-photon state. Our results reveal that, for certain phase values, partially distinguishable multi-photon states can achieve higher Fisher information values compared to the two-photon experiment. These findings highlight the potential of distinguishable multi-photon states for enhanced precision in quantum metrology and related applications.