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arXiv:2602.05806

Assessing the Sensitivity of Niobium- and Tantalum-Based Superconducting Qubits to Infrared Radiation

Michael Kerschbaum, Felix Wagner, Uroš Ognjanović, Giovanni Vio, Kuno Knapp, Dante Colao Zanuz, Alexander Flasby, Mohsen Bahrami Panah, Andreas Wallraff, Jean-Claude Besse

quant-phSubmitted Feb 5, 2026• Announced Feb 6, 2026• 0 citations
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Abstract

The use of tantalum films for superconducting qubits has recently extended qubit coherence times significantly, primarily due to reduced dielectric losses at the metal-air interface. However, the choice of base material also influences the sensitivity to quasiparticle-induced decoherence. In this study, we investigate quasiparticle tunneling rates in niobium and tantalum-based offset-charge-sensitive qubits. Using a source of thermal radiation, we characterize the sensitivity of either material to infrared radiation and explore the impact of the infrared background through the targeted use of in-line filters in the wiring and ambient infrared absorbers. We identify both radiation channels as significant contributions to decoherence for tantalum but not for niobium qubits and achieve tunneling rates of 100 Hz and 300 Hz for niobium and tantalum respectively upon installation of infrared filters. Additionally, we find a time-dependence in the observed tunneling rates on the scale of days, which we interpret as evidence of slowly cooling, thermally radiating components in the experimental setup. Our findings indicate that continued improvements in coherence times may require renewed attention to radiative backgrounds and experimental setup design, especially when introducing new material platforms.

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14 pages, 4 main figures

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The use of tantalum films for superconducting qubits has recently extended qubit coherence times significantly, primarily due to reduced dielectric losses at the metal-air interface. However, the choice of base material also influences the sensitivity to quasiparticle-induced decoherence. In this study, we investigate quasiparticle tunneling rates in niobium and tantalum-based offset-charge-sensitive qubits. Using a source of thermal radiation, we characterize the sensitivity of either material to infrared radiation and explore the impact of the infrared background through the targeted use of in-line filters in the wiring and ambient infrared absorbers. We identify both radiation channels as significant contributions to decoherence for tantalum but not for niobium qubits and achieve tunneling rates of 100 Hz and 300 Hz for niobium and tantalum respectively upon installation of infrared filters. Additionally, we find a time-dependence in the observed tunneling rates on the scale of days, which we interpret as evidence of slowly cooling, thermally radiating components in the experimental setup. Our findings indicate that continued improvements in coherence times may require renewed attention to radiative backgrounds and experimental setup design, especially when introducing new material platforms.
One of the primary origins of the energy relaxation in superconducting qubits is the quasiparticle loss. The quasiparticles can be excited remarkably by infrared radiation. In order to minimize the density of quasiparticle and increase the qubit relaxation time, we design and fabricate the infrared filter and shield for superconducting qubits. In comparison with previous filters and shields, a nonmagnetic dielectric is used as the infrared absorbing material, greatly suppressing the background magnetic fluctuations. The filters can be made to impedance-match with other microwave devices. Using the as-fabricated infrared filter and shield, we increased the relaxation time of a transmon qubit from 519 ns to 1125 ns.
Over the past decades, superconducting qubits have emerged as one of the leading hardware platforms for realizing a quantum processor. Consequently, researchers have made significant effort to understand the loss channels that limit the coherence times of superconducting qubits. A major source of loss has been attributed to two level systems that are present at the material interfaces. It is recently shown that replacing the metal in the capacitor of a transmon with tantalum yields record relaxation and coherence times for superconducting qubits, motivating a detailed study of the tantalum surface. In this work, the chemical profile of the surface of tantalum films grown on c-plane sapphire using variable energy X-ray photoelectron spectroscopy (VEXPS) is studied. The different oxidation states of tantalum that are present in the native oxide resulting from exposure to air are identified, and their distribution through the depth of the film is measured. Furthermore, it is shown how the volume and depth distribution of these tantalum oxidation states can be altered by various chemical treatments. Correlating these measurements with detailed measurements of quantum devices may elucidate the underlying microscopic sources of loss.
Superconducting qubits can be sensitive to sudden energy deposits into the substrate from cosmic rays and ambient radioactivity. While previous studies have primarily focused on exploring correlated effects over time and distance due to cosmic rays, this study uniquely offers a direct comparison of a transmon qubit's response at Fermilab SQMS above-ground facilities and the deep-underground Gran Sasso Laboratory (INFN-LNGS, Italy). Despite the vastly different radiation environments, we observe a similar average qubit lifetime (T1) of approximately 80 microseconds at both sites. We then employ a fast decay detection protocol and investigate the time structure, sensitivity, and relative rates of triggered events due to radiation versus intrinsic noise. We compare the above and underground performance of several high-coherence qubits with similar designs. Our findings reveal no significant difference in events with radiation-like signatures between above-ground and underground conditions for these sapphire and niobium-based transmon qubits. This suggests that most such events are likely due to other noise sources, which predominantly contribute to single-qubit errors in contemporary transmon qubits. By exposing the qubits to gamma sources with varying activity levels, we further evaluate their response to radiation in a low-background environment. The results show that qubits can indeed detect particle impacts; however, this capability is only realized by substantially reducing other noise sources, which in turn affects detection efficiency [1].
times 2 to 5 times longer than baseline niobium qubit devices with native niobium oxides. When capping niobium with tantalum, we obtain median qubit lifetimes above 200 microseconds. Our comparative structural and chemical analysis suggests that amorphous niobium oxides may induce higher losses compared to other amorphous oxides. These results are in line with high-accuracy measurements of the niobium oxide loss tangent obtained with ultra-high Q superconducting radiofrequency (SRF) cavities. This new surface encapsulation strategy enables even further reduction of dielectric losses via passivation with ambient-stable materials, while preserving fabrication and scalable manufacturability thanks to the compatibility with silicon processes.
times 2 to 5 times longer than baseline niobium qubit devices with native niobium oxides. When capping niobium with tantalum, we obtain median qubit lifetimes above 200 microseconds. Our comparative structural and chemical analysis suggests that amorphous niobium oxides may induce higher losses compared to other amorphous oxides. These results are in line with high-accuracy measurements of the niobium oxide loss tangent obtained with ultra-high Q superconducting radiofrequency (SRF) cavities. This new surface encapsulation strategy enables even further reduction of dielectric losses via passivation with ambient-stable materials, while preserving fabrication and scalable manufacturability thanks to the compatibility with silicon processes.
The superconducting transmon qubit is a leading platform for quantum computing and quantum science. Building large, useful quantum systems based on transmon qubits will require significant improvements in qubit relaxation and coherence times, which are orders of magnitude shorter than limits imposed by bulk properties of the constituent materials. This indicates that relaxation likely originates from uncontrolled surfaces, interfaces, and contaminants. Previous efforts to improve qubit lifetimes have focused primarily on designs that minimize contributions from surfaces. However, significant improvements in the lifetime of two-dimensional transmon qubits have remained elusive for several years. Here, we fabricate two-dimensional transmon qubits that have both lifetimes and coherence times with dynamical decoupling exceeding 0.3 milliseconds by replacing niobium with tantalum in the device. We have observed increased lifetimes for seventeen devices, indicating that these material improvements are robust, paving the way for higher gate fidelities in multi-qubit processors.