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arXiv:2512.24539

TLS-induced thermal nonlinearity in a micro-mechanical resonator

Cyril Metzger, Alec L. Emser, Brendon C. Rose, Konrad W. Lehnert

quant-phcond-mat.mes-hallSubmitted Dec 31, 2025• Announced Jan 1, 2026
arXivHTMLPDF

Abstract

We present experimental evidence of a thermally-driven amplitude-frequency nonlinearity in a thin-film quartz phononic crystal resonator at millikelvin temperatures. The nonlinear response arises from the coupling of the mechanical mode to an ensemble of microscopic two-level system defects driven out of equilibrium by a microwave drive. In contrast to the conventional Duffing oscillator, the observed nonlinearity exhibits a mixed reactive-dissipative character. Notably, the reactive effect can manifest as either a softening or hardening of the mechanical resonance, depending on the ratio of thermal to phonon energy. By combining the standard TLS theory with a thermal conductance model, the measured power-dependent response is quantitatively reproduced and readout-enhanced relaxation damping from off-resonant TLSs is identified as the primary mechanism limiting mechanical coherence. Within this framework, we delineate the conditions under which similar systems will realize this nonlinearity.

DOI
10.1103/q9g9-xbh2
Comments
45 pages, 16 figures, main paper followed by appendices and supplemental materials

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We present experimental evidence of a thermally-driven amplitude-frequency nonlinearity in a thin-film quartz phononic crystal resonator at millikelvin temperatures. The nonlinear response arises from the coupling of the mechanical mode to an ensemble of microscopic two-level system defects driven out of equilibrium by a microwave drive. In contrast to the conventional Duffing oscillator, the observed nonlinearity exhibits a mixed reactive-dissipative character. Notably, the reactive effect can manifest as either a softening or hardening of the mechanical resonance, depending on the ratio of thermal to phonon energy. By combining the standard TLS theory with a thermal conductance model, the measured power-dependent response is quantitatively reproduced and readout-enhanced relaxation damping from off-resonant TLSs is identified as the primary mechanism limiting mechanical coherence. Within this framework, we delineate the conditions under which similar systems will realize this nonlinearity.
Phonon modes within pristine crystalline resonators now routinely reach the quantum ground state. Such systems are attractive for quantum information science applications, as advanced fabrication and processing can enable relatively long quantum coherence times, and precision control can be realized through optical, electrical, or qubit coupling. In many state-of-the-art systems, the phonon lifetime is limited by disorder. In particular, native oxides or damaged `dead layers' at surfaces can host two-level tunneling states that lead to a particularly problematic form of dissipation that increases at lower temperatures. As mechanical losses are driven down in systems such as micro-fabricated bulk acoustic wave resonators, tunneling states are expected to emerge as the dominant mechanism for phonon decoherence. A quantitative description of these mesoscopic systems therefore requires a framework that captures interactions between a selected phonon mode and a large ensemble of TLS. Here, we derive a quantum master equation for this coupled system, permitting the phonon decoherence produced by two-level tunneling states to be calculated. As an example, we estimate the lifetime of a variety of quantum states within quartz micro-resonators hosting a thin surface layer of tunneling states. We find that the phonon coherence time is maximized at low temperatures, in spite of increased mechanical dissipation, and that phonon-TLS coupling can be reduced for modes with strain nodes at the surfaces.
Recent experiments on a range of engineered quantum systems have highlighted the important role of interacting two-level systems (TLSs) in modifying device properties and generating fluctuations. Focusing on the case of an oscillator coupled to a single near-resonant TLS, we explore how interactions between the TLS and lower-frequency thermally activated two-level fluctuators (TLFs) degrade the oscillator's coherence. Depending on the strength of the couplings, a single TLF can give rise to coherence oscillations that appear alongside, or supplant, Rabi oscillations of the oscillator-TLS system. Bath-driven transitions in the TLF cause irreversible coherence decay at a rate that is highly sensitive to both the couplings and the transition rate. For an ensemble of TLFs, we identify and characterise the different regimes of non-exponential phase-averaging-driven coherence decay that the oscillator can display. Using numerical calculations, we examine the extent to which systems with just a few TLFs differ from the limit of a large (continuum) TLF ensemble. Our work provides a theoretical framework for understanding the interplay of coherent TLS interactions and TLF-induced dephasing in quantum devices such as superconducting and phononic resonators.
Abstract Nanomechanical oscillators offer numerous advantages for quantum technologies. Their integration with superconducting qubits shows promise for hardware-efficient quantum error-correction protocols involving superpositions of mechanical coherent states. Limitations of this approach include mechanical decoherence processes, particularly two-level system (TLS) defects, which have been widely studied using classical fields and detectors. In this manuscript, we use a superconducting qubit as a quantum sensor to perform phonon number-resolved measurements on a piezoelectrically coupled phononic crystal cavity. This enables a high-resolution study of mechanical dissipation and dephasing in coherent states of variable size ( nˉ≃1−10\bar{n}\simeq 1-10nˉ≃1−10 n ¯ ≃ 1 − 10 phonons). We observe nonexponential relaxation and state size-dependent reduction of the dephasing rate, which we attribute to TLS. Using a numerical model, we reproduce the dissipation signatures (and to a lesser extent, the dephasing signatures) via emission into a small ensemble ( N = 5) of rapidly dephasing TLS. Our findings comprise a detailed examination of TLS-induced phonon decoherence in the quantum regime.
We show that the two-level systems (TLS) in lithographic superconducting circuits act as a power-dependent dielectric leading to non-linear responses in a parametrically coupled electromechanical system. Driven TLS shift the microwave resonance frequency and modulate the mechanical resonance through the optical spring effect. By pumping with two tones in a back-action evading measurement, these effects produce a mechanical parametric instability which limits single quadrature imprecision to 1.4 xzp. The microwave resonator noise is also consistent to a TLS-noise model. These observations suggest design strategies for minimizing TLS effects to improve ground-state cooling and quantum non-demolition measurements of motion.
We report the microwave response of coplanar-waveguide (CPW) resonators fabricated from YBa2Cu3O7−δ\mathrm{YBa_2Cu_3O_{7-δ}}YBa2​Cu3​O7−δ​ (YBCO) thin films over temperatures from approximately 70 mK70~\mathrm{mK}70 mK to 40 K40~\mathrm{K}40 K. The resonators exhibit internal quality factors QiQ_\mathrm{i}Qi​ in the range of 4×1034\times10^34×103 to 10410^4104 at 70 mK, which increase to a maximum of approximately 8×1038\times10^38×103 to 1.2×1041.2\times10^41.2×104 near 6 K6~\mathrm{K}6 K. At low temperatures, both QiQ_\mathrm{i}Qi​ and the fractional shift of the resonance frequency Δfr/frΔf_\mathrm{r}/f_\mathrm{r}Δfr​/fr​ increases with temperature, qualitatively resembling behavior commonly associated with two-level-system (TLS) defects. However, neither response saturates on the temperature scale set by the resonator frequency, and the loss exhibits no observable microwave-power dependence. We show that low-temperature frequency upturn may be better described by an additional paramagnetic response associated with defect-induced local moments or Andreev bound states, while the low-temperature loss follows an approximately logarithmic temperature dependence whose microscopic origin remains unresolved. These measurements establish the millikelvin performance of patterned YBCO resonators and show that their low-temperature response cannot be understood within the conventional TLS framework alone.
A quartz Bulk Acoustic Wave resonator is designed to coherently trap phonons in such a way that they are well confined and immune to suspension losses so they exhibit extremely high acoustic Q-factors at low temperature, with Q × f products of order 10¹⁸ Hz. In this work we couple such a resonator to a Superconducting Quantum Interference Device (SQUID) amplifier and investigate effects in the strong signal regime. Both parallel and series connection topologies of the system are investigated. The study reveals significant non-Duffing response that is associated with the nonlinear characteristics of Josephson junctions. The nonlinearity provides quasi-periodic structure of the spectrum in both incident power and frequency. The result gives an insight into the open loop behaviour of a future Cryogenic Quartz Oscillator in the strong signal regime.