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arXiv:2512.07589 · Applied Physics Letters

On-Demand Microwave Single-Photon Source Based on Tantalum Thin Film

Ying Hu, Sheng-Yong Li, En-Qi Chen, Jing Zhang, Yu-xi Liu, Jia-Gui Feng, Zhihui Peng

quant-phSubmitted Dec 8, 2025• Announced Dec 9, 2025• 2 citations
arXivHTMLPDF

Abstract

Single-photon sources are crucial for quantum information technologies. Here, we demonstrate a microwave single-photon source fabricated using a tantalum-based thin film, whose favorable material properties enable high-quality and stable photon emission. The antibunching behavior of the emitted radiation is revealed by second-order correlation measurements. Furthermore, traveling-wave parametric amplifiers are used as the pre-amplifier in the detection chains, we substantially improve the signal-to-noise ratio and thereby greatly reduce the acquisition time required for second-order correlation measurements. These results demonstrate the viability of tantalum-based superconducting devices as reliable platforms for microwave quantum photonics.

DOI
10.1063/5.0316437
Comments
9 pages, 5 figures

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Single-photon sources are crucial for quantum information technologies. Here, we demonstrate a microwave single-photon source fabricated using a tantalum-based thin film, whose favorable material properties enable high-quality and stable photon emission. The antibunching behavior of the emitted radiation is revealed by second-order correlation measurements. Furthermore, traveling-wave parametric amplifiers are used as the pre-amplifier in the detection chains, we substantially improve the signal-to-noise ratio and thereby greatly reduce the acquisition time required for second-order correlation measurements. These results demonstrate the viability of tantalum-based superconducting devices as reliable platforms for microwave quantum photonics.
Single-photon sources of high efficiency are of great interest because they are the key elements in many prospective quantum technologies and applications. Based on our previous work, here we demonstrate a high-quality tunable microwave single-photon source based on transmon qubit with intrinsic emission efficiency more than 99%. To further confirm the single-photon property of the source, we study the single-photon interference in a Hanbury-Brown-Twiss (HBT) type setup and measure the correlation functions of the emission field using linear detectors with GPU-enhanced signal processing technique. The antibunching in second-order correlation function is clearly observed. The theoretical calculations agree well with the experimental results. Such a high-quality single-photon source may be used as a building block for quantum communication, simulation and information processing in microwave regime.
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Single-photon generation is an important proof of the underlying quantum nature of a physical process and a ubiquitous tool for scientific exploration, with applications ranging from spectroscopy and metrology to quantum computing.In the microwave regime, emission of antibunched radiation has so far relied on coherent control of Josephson qubits requiring precisely calibrated microwave pulses.In this work, we experimentally demonstrate the operation of a bright on-demand source of quantum microwave radiation driven by a simple dc voltage bias across a Josephson junction.Our source is based on photon emission into a microwave resonator through inelastic Cooper pair tunneling regulated by a high-impedance RC circuit preventing simultaneous tunnel events.It is characterized by its normalized second-order correlation function of g ð2Þ ð0Þ ≈ 0.43 corresponding to antibunching in the single-photon regime.Our device can be triggered, and its in situ tunable emission rate exceeds those obtained with current microwave singlephoton sources by more than 1 order of magnitude.
Using modern micro and nano-fabrication techniques combined with superconducting materials we realize quantum electronic circuits in which we create, store, and manipulate individual microwave photons. The strong interaction of photons with superconducting quantum two-level systems allows us to probe fundamental quantum effects of microwave radiation and also to develop components for applications in quantum technology. Previously we have realized on-demand single photon sources which we have characterized using correlation function measurements [1] and full quantum state tomography [2]. For this purpose we have developed efficient methods to separate the quantum signals of interest from the noise added by the linear amplifiers used for quadrature amplitude detection [3]. We now regularly employ superconducting parametric amplifiers [4] to perform nearly quantum limited detection of propagating electromagnetic fields. These enable us to probe the entanglement which we generate on demand between stationary qubits and microwave photons freely propagating down a transmission line [5]. Using two independent microwave single photon sources, we have recently performed Hong-Ou-Mandel experiments at microwave frequencies [6] and have probed the coherence of two-mode multi-photon states at the out-put of a beam-splitter. The non-local nature of such states may prove to be useful for distributing entanglement in future small-scale quantum networks.
Efficient and stable microwave-optical transduction is a key enabling technology for distributed superconducting quantum computing and heterogeneous quantum networks. Electro-optic transducers based on thin-film lithium niobate (TFLN) have shown strong promise, but demonstrations to date have been limited by various factors such as low frequency bias drift, low efficiency, fabrication complexity, and scalability. Here we demonstrate the first integrated electro-optic microwave-optical transducers realized in thin-film lithium tantalate (TFLT), a material platform offering Pockels nonlinearity comparable to TFLN together with improved bias stability and high-power handling. We fabricate superconducting microwave resonators coupled to tunable photonic-molecule optical resonators using wafer-scale deep ultraviolet lithography, offering high-throughput production of hundreds of devices per wafer. Across six devices we observe coherent bidirectional conversion between C-band optical photons and 4.9-5.5 GHz microwave photons, with measured on-chip efficiencies and inferred single-photon coupling rates g_0/2π ~ 1 kHz consistent with theory. Continuous operation over multiple days is achieved using a static bias field with minimal feedback, demonstrating a major operational advantage. We further characterize optical loss statistics, microwave resonator performance, and optically induced added noise under pulsed pumping, finding less than one added photon for 100 microsecond pulses at the highest measured efficiencies. These results establish TFLT as a scalable and robust electro-optic platform for future quantum interconnects and modular quantum processors.
Abstract We demonstrate an on-demand source of microwave single photons with 71–99% intrinsic quantum efficiency. The source is narrowband (300 kHz) and tuneable over a 600 MHz range around 5.2 GHz. Such a device is an important element in numerous quantum technologies and applications. The device consists of a superconducting transmon qubit coupled to the open end of a transmission line. A π-pulse excites the qubit, which subsequently rapidly emits a single photon into the transmission line. A cancellation pulse then suppresses the reflected π-pulse by 33.5 dB, resulting in 0.005 photons leaking into the photon emission channel. We verify strong antibunching of the emitted photon field and determine its Wigner function. Non-radiative decay and 1/f flux noise both affect the quantum efficiency. We also study the device stability over time and identify uncorrelated discrete jumps of the pure dephasing rate at different qubit frequencies on a time scale of hours, which we attribute to independent two-level system defects in the device dielectrics, dispersively coupled to the qubit. Our single-photon source with only one input port is more compact and scalable compared to standard implementations.