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arXiv:2511.23301 · Nature Communications

Inhibited radiative decay enhances single-photon emitters

Florian Burger, Stephan Rinner, Andreas Gritsch, Kilian Sandholzer, Andreas Reiserer

quant-phcond-mat.otherSubmitted Nov 28, 2025• Announced Dec 1, 2025• 0 citations

v1 · Nov 28, 2025 v2 · Jun 17, 2026

Abstract

Quantum networks and the modular scaling of quantum computers require efficient spin-photon interfaces. This can be achieved with optical resonators that increase the local density of states, thereby enhancing the radiative decay of emitters on a specific transition. However, small mode volumes and high quality factors are required in this approach, which restricts the multiplexing capacity and necessitates precise tuning of the resonator frequency. Here, we demonstrate an alternative method that avoids these bottlenecks for up-scaling. Instead of strongly enhancing the emission on a selected transition, we suppress all other radiative decay channels by tailoring the photonic bandgap of a W1 silicon photonic crystal waveguide. In such a device, we can spectrally resolve and individually address tens of erbium dopants. We find that their emission is channeled to the desired transition, ensuring efficient collection. At the same time, their lifetimes are preserved or even extended compared to the bulk in a broad spectral range. Furthermore, the extended mode volume facilitates a low dopant concentration and thus a large spatial separation between the emitters, avoiding unwanted interactions that would limit their coherence. The demonstrated approach of inhibiting unwanted spontaneous emission can be combined with Purcell enhancement and applied to other leading spin-qubit platforms. It thus opens intriguing perspectives for photonic quantum technologies.

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Individual spins that are coupled to telecommunication photons offer unique promise for distributed quantum information processing once a coherent and efficient spin–photon interface can be fabricated at scale. We implement such an interface by integrating erbium dopants into a nanophotonic silicon resonator. We achieve spin-resolved excitation of individual emitters with <0.1GHz spectral diffusion linewidth. Upon resonant driving, we observe optical Rabi oscillations and single-photon emission with a 78-fold Purcell enhancement. Our results establish a promising platform for quantum networks.

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The unrivaled maturity of its nanofabrication makes silicon a promising hardware platform for quantum information processing. To this end, efficient single-photon sources and spin-photon interfaces have been implemented by integrating color centers or erbium dopants into nanophotonic resonators. However, the optical emission frequencies in this approach are subject to temporal fluctuations on both long and short timescales, which hinders the development of quantum applications. Here, we investigate this limitation and demonstrate that it can be alleviated by integrating the emitters into Fabry-Perot instead of nanophotonic resonators. Their larger optical mode volume enables both increasing the distance to crystal surfaces and operating at a lower dopant concentration, which reduces implantation-induced crystal damage and interactions between emitters. As a result, we observe a fivefold reduction of the spectral diffusion linewidth down to 4.0(2) MHz. Calculations and experimental investigations of isotopically purified 28-Si crystals suggest that the remaining spectral instability is caused by laser-induced electric-field fluctuations. In direct comparison with a nanophotonic device, the instability is significantly reduced at the same intracavity power, enabling a tenfold increase of the optical coherence time up to 20(1) microseconds. These findings represent a key step towards spectrally stable spin-photon interfaces in silicon and their potential applications in quantum networking and distributed quantum information processing.

Building quantum networks requires efficient coupling of solid-state quantum emitters to photonic devices. Tinvacancy center (SnV) has attracted much interest for having long spin coherence times at temperatures above 1 K. Employing SnV as an optically addressable qubit requires integration with photonic structures to both route the emitted photons and enhance the light-matter interaction. We present incorporation of high-quality SnV centers with narrow linewidths in suspended diamond waveguides. Furthermore, we fabricate photonic crystal cavities in diamond with embedded SnV centers. We observe strong intensity enhancement of the photon emission when the cavity is resonant with the color center. Time-resolved photoluminescence measurements confirm that this effect is due to radiative Purcell enhancement of the spontaneous emission. Finally, we demonstrate Stark tuning of transition frequency of SnV centers, essential for multiemitter applications. These results are a significant step toward color-center-based quantum information processing applications without the need for dilution refrigerators.

Solid-state spin-based quantum systems have emerged as popular platforms for quantum networking applications due to their optical interfaces, their long-lived quantum memories, and their natural compatibility with semiconductor manufacturing. Photonic crystal cavities are often used to enhance radiative emission; however, fabrication of the necessary subwavelength cavities is typically limited to small batch electron beam lithography. In this work, we demonstrate high quality factor, small mode volume nanobeam cavities fabricated on a scalable silicon photonic foundry platform. The foundry fabricated cavities are then interfaced with single erbium ions through backend deposition of TiO 2 thin films lightly doped with erbium. Single ion lifetime measurements indicate Purcell enhancement up to about 500, thereby demonstrating a route toward manufacturable deterministic single photon sources in the telecom C-band.

Telecom-band spin defects in silicon offer a compelling platform for integrated quantum networks by combining scalable silicon photonics with spin-based quantum memories and multiqubit registers. The T center and recently demonstrated Al1 center are particularly promising, but their limited coherent zero-phonon emission requires strong cavity enhancement for efficient spin-photon interfaces. Here, we inverse-design silicon nanobeam cavities for both centers using a unified adjoint-optimization framework targeting Purcell enhancement, resonance alignment, and photon extraction. For each emitter, symmetric cavities maximize Purcell enhancement, while asymmetric cavities provide directional coupling to an integrated waveguide. Three-dimensional finite-difference time-domain simulations yield loaded quality factors up to 3.25 x 10^6, Purcell factors up to 1.43 x 10^5, and cooperativities of approximately 280-5000, corresponding to cavity-coupled emission fractions exceeding 99.6%. The asymmetric cavities direct approximately 90% of emitted power into a single on-chip waveguide while maintaining cooperativity above 280. Under nanometer-scale fabrication perturbations, all four designs remain within the high-cooperativity regime, and high cooperativity persists when the cavity quality factor is constrained to a realistic absorption-limited value of 10^5. This unified, fabrication-compatible framework establishes a scalable cavity-design route for silicon telecom spin-photon interfaces and, to our knowledge, the first cavity designs for the Al1 center.