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arXiv:2511.08105 · APL Photonics

Enhanced quantum correlations from joint pump and photon pair scattering

Mamoon Safadi, Nir Kuchuk, Ohad Lib, Yaron Bromberg, Arthur Goetschy

quant-phphysics.opticsSubmitted Nov 11, 2025• Announced Nov 12, 2025• 0 citations
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Abstract

Scattering of non-classical light is enabling new ways to study and control photon transport. However, advances in this field often rely on simplifying assumptions regarding the quantum light's generation and its source. In this work, we relax some of these assumptions and probe the behavior of entangled photon pairs passing through a disordered layer after being generated by a randomly scattered pump via spontaneous parametric down conversion. We experimentally demonstrate that, even when both the pump and the down-converted photons propagate through a dynamic scattering medium, the pairs maintain a sharp peak in their correlations. A comprehensive theoretical and numerical analysis shows that these correlations persist regardless of when the pairs are generated, whether immediately after the pump is scattered or under other conditions. More specifically, we detail how the shape of the angular correlation depends on the pump's scattering and how it varies with the distance between the pair-generation region and the entrance of the disordered medium. These findings represent a crucial step toward understanding quantum light generation in complex media, and potentially exploiting it for quantum technologies.

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•Jan 1, 2002•1 citation
Scattering of non-classical light is enabling new ways to study and control photon transport. However, advances in this field often rely on simplifying assumptions regarding the quantum light's generation and its source. In this work, we relax some of these assumptions and probe the behavior of entangled photon pairs passing through a disordered layer after being generated by a randomly scattered pump via spontaneous parametric down conversion. We experimentally demonstrate that, even when both the pump and the down-converted photons propagate through a dynamic scattering medium, the pairs maintain a sharp peak in their correlations. A comprehensive theoretical and numerical analysis shows that these correlations persist regardless of when the pairs are generated, whether immediately after the pump is scattered or under other conditions. More specifically, we detail how the shape of the angular correlation depends on the pump's scattering and how it varies with the distance between the pair-generation region and the entrance of the disordered medium. These findings represent a crucial step toward understanding quantum light generation in complex media, and potentially exploiting it for quantum technologies.
Photon-pair correlations in spontaneous parametric down conversion (SPDC) processes are ubiquitous in quantum photonics. In this work, we engineer these correlations by imaging arbitrarily chosen objects in the second order correlations of spatially-entangled photon pairs produced by type-I SPDC in a non-linear crystal. Our approach is effective with both amplitude and phase objects, even when the beam intensity is spatially shaped. Additionally, we show that it is resistant to scattering by applying wavefront shaping techniques. We also find that certain phase patterns can refocus through the scattering medium exclusively with photon pairs, and not with classical coherent light. Consequently, the transmission of an image through the scattering medium is only possible if it is correlation encoded; coherent light alone cannot reconstruct the image. Our approach enables the transmission of complex, high-dimensional information using quantum correlations of photons, offering significant potential for advancing quantum communication and imaging protocols.
Spontaneous parametric down-conversion (SPDC) is one of the most important sources of entangled photons in quantum optics and underpins a wide range of applications in quantum communication, quantum imaging, quantum sensing, and photonic quantum information processing. In this nonlinear optical process, a pump photon is converted into a pair of lower-energy photons that exhibit strong correlations in multiple degrees of freedom. While the generation of photon pairs is governed by energy and momentum conservation, the resulting biphoton state possesses a rich spatial structure whose properties are determined by the interplay among the pump field, the nonlinear medium, and subsequent propagation. This thesis investigates the spatial properties of entangled photon pairs generated through SPDC, focusing on the evolution of their correlations in the near field and on the behavior of orbital-angular-momentum (OAM) entangled states under tight focusing conditions. A common theme throughout this work is the examination of physical effects that emerge when the full biphoton wavefunction is retained rather than reduced through the simplifying approximations often employed in theoretical treatments. The principal contribution of this thesis concerns the near-field propagation of SPDC photon pairs. The spatial correlations of SPDC-generated photons are commonly analyzed within the thin-crystal approximation, where the biphoton wavefunction is assumed to factorize into independent functions of the sum and difference coordinates. We demonstrate that birefringence-induced transverse walk-off breaks this factorization and introduces an intrinsic coupling between these coordinates. More importantly, this coupling survives free-space propagation and remains observable even for crystals that nominally satisfy the thin-crystal condition. As a result, the joint spatial correlations develop a characteristic tapering near the crystal image plane that cannot be captured by conventional factorized models. Numerical simulations and experimental measurements are found to be in excellent agreement, revealing a previously overlooked feature of SPDC and providing a more complete description of photon-pair generation and propagation in birefringent nonlinear media. The second part of the thesis explores the propagation of OAM-entangled photon pairs beyond the paraxial regime. While OAM correlations are typically studied under weak-focusing conditions, many emerging quantum technologies require structured quantum states to be manipulated in highly confined optical systems. We show that tight focusing modifies the OAM correlation spectrum, leading to a broadening of the accessible mode distribution. This broadening exhibits distinct transverse and longitudinal characteristics and arises from the emergence of nonparaxial field components absent in conventional scalar descriptions. These results provide new insight into the behavior of structured quantum light in strongly focused optical fields and establish a framework for understanding OAM entanglement beyond the paraxial approximation. Together, the results presented in this thesis reveal previously unexplored aspects of the structure and propagation of entangled photon pairs. By moving beyond widely used approximations, this work uncovers physical effects that influence the generation, evolution, and measurement of spatially entangled states, with implications for quantum imaging, high-dimensional quantum communication, and the broader development of structured-light-based quantum technologies.
We image with cameras entangled photon light transmitted through a random medium. Near-field and far-field spatial quantum correlations show that entangled photon pairs (bi-photons) generated by spontaneous optical parametric down-conversion exhibit speckle pattern. In contrast, no information from the random medium can be extracted using incoherent light issued from one photon of the pair. Although these measurements require several hours to record thousands of image pairs, our method is instantaneous for the recording of one pair of twin images and involve all the photons of the images.
Efficient Generation of Entangled Photon-Pairs The first experiments with correlated photons have been performed in the context of EPR-Bell experiments on the realistic and local properties of quantum mechanics. The source used there produced pairs of polarization entangled photons from a 2-photon decay of Calcium atoms. The technical requirements of these experiments were high (vacuum systems, stronge dye-lasers, etc.) whereas the efficiency of the source was quite low. An important step forward was the introduction of spontaneous parametric down conversion (SPDC), which has become the most common source in quantum optics for generating correlated or entangled photon pairs. In this process photons of an intense pump laser convert to photon pairs in an optical nonlinear crystal. Conservation of energy and momentum leads to strong correlations between the generated photons. With this kind of two-photon source it was possible to realize or improve many experiments on the foundations of quantum mechanics addressing the EPR-Paradoxon and in the new field of quantum information. But again, more advanced experiments and applications suffer from the limited ef- ficiency of the fluorescence process. Many photon pairs are lost by spatial and spectral filtering, which is necessary to achieve polarization entanglement and long coherence times. Different techniques have been implemented to increase the number of photon pairs using two-crystal arrangements, focusing techniques or periodically poled crystals. Most of these methods have the disadvantage that no entangled photons have been observed. It is the aim of this work to increase the yield and to improve the mode definition of entangled photon pairs generated by resonant enhancement of the pump mode and the fluorescence modes. As a first step a linear cavity for the pump mode was realized. Since the conversion probability is proportional to the pump power it was possible to increase the photon pair count rate by factor of 7 over the previous source. Besides the possibility of further improvement on already established pair correlation experiments, such an enhancement allows to build a compact source for photon pairs, in which an expensive argon-ion laser is replaced by a cheap diode laser. Among other applications such sources are of strong interest for quantum cryptography. 3 In many quantum information experiments optical fibers are use to carry the photons over long distance. Therefore, light from the parametric down-conversion source has to be efficiently coupled into fibers. In the second part we report on a new method to optimize collection efficiency by matching the angular distribution of the parametric fluorescence to the spatial mode of an optical fiber. By using this technique, we detected 366500 polarization-entangled photon pairs per second in the near-infrared region in single-mode optical fibers for 465 mW pump power (at 351.1 nm) with a 2 mm BBOcrystal. The entanglement of the photon pairs was verified by measuring polarization correlations of more than 96% in a HV-basis and in a ±45◦-basis. To our knowledge, such enormous count rates of highly entangled photon pairs have not been reached yet with any other technique. In the third part of this thesis we investigated the process of parametric downconversion in a cavity which is resonant to certain longitudinal down-conversion modes only. The idea of placing the parametric down-conversion source inside a cavity is not new. Such a device is usually referred to as a single or double resonant optical parametric oscillator (OPO) and is mainly used to generate squeezed quantum states. In that kind of application the system is operating close to but still under the threshold of oscillation. In our application the situation is quite different. The system is operating far below threshold so that mainly spontaneous emission occurs. In that mode correlations between single photons can still be observed. But bouncing the light back and forth inside the cavity increases the interaction length and hence enhances the signal levels of the down-conversion fields. Further, by resonating two certain modes only, the bandwidth is reduced by orders of magnitude and the coherence time is found to be inverse proportional to the bandwidth. A similar experiment has already been realized with a type-I parametric down-converter in the resonator. We have tried to realize a compact double resonant OPO far below threshold with a type-II parametric down-converter in a high-finesse cavity to realize a bright source of entangled photon pairs with extremely narrow bandwidth.