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Evolution of Spatially Entangled Photons Beyond Standard Approximations

Christian Howard

Published Aug 24, 2026• 0 citations
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Abstract

Spontaneous parametric down-conversion (SPDC) is one of the most important sources of entangled photons in quantum optics and underpins a wide range of applications in quantum communication, quantum imaging, quantum sensing, and photonic quantum information processing. In this nonlinear optical process, a pump photon is converted into a pair of lower-energy photons that exhibit strong correlations in multiple degrees of freedom. While the generation of photon pairs is governed by energy and momentum conservation, the resulting biphoton state possesses a rich spatial structure whose properties are determined by the interplay among the pump field, the nonlinear medium, and subsequent propagation. This thesis investigates the spatial properties of entangled photon pairs generated through SPDC, focusing on the evolution of their correlations in the near field and on the behavior of orbital-angular-momentum (OAM) entangled states under tight focusing conditions. A common theme throughout this work is the examination of physical effects that emerge when the full biphoton wavefunction is retained rather than reduced through the simplifying approximations often employed in theoretical treatments. The principal contribution of this thesis concerns the near-field propagation of SPDC photon pairs. The spatial correlations of SPDC-generated photons are commonly analyzed within the thin-crystal approximation, where the biphoton wavefunction is assumed to factorize into independent functions of the sum and difference coordinates. We demonstrate that birefringence-induced transverse walk-off breaks this factorization and introduces an intrinsic coupling between these coordinates. More importantly, this coupling survives free-space propagation and remains observable even for crystals that nominally satisfy the thin-crystal condition. As a result, the joint spatial correlations develop a characteristic tapering near the crystal image plane that cannot be captured by conventional factorized models. Numerical simulations and experimental measurements are found to be in excellent agreement, revealing a previously overlooked feature of SPDC and providing a more complete description of photon-pair generation and propagation in birefringent nonlinear media. The second part of the thesis explores the propagation of OAM-entangled photon pairs beyond the paraxial regime. While OAM correlations are typically studied under weak-focusing conditions, many emerging quantum technologies require structured quantum states to be manipulated in highly confined optical systems. We show that tight focusing modifies the OAM correlation spectrum, leading to a broadening of the accessible mode distribution. This broadening exhibits distinct transverse and longitudinal characteristics and arises from the emergence of nonparaxial field components absent in conventional scalar descriptions. These results provide new insight into the behavior of structured quantum light in strongly focused optical fields and establish a framework for understanding OAM entanglement beyond the paraxial approximation. Together, the results presented in this thesis reveal previously unexplored aspects of the structure and propagation of entangled photon pairs. By moving beyond widely used approximations, this work uncovers physical effects that influence the generation, evolution, and measurement of spatially entangled states, with implications for quantum imaging, high-dimensional quantum communication, and the broader development of structured-light-based quantum technologies.

DOI
10.20381/ruor-32175

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Spontaneous parametric down-conversion (SPDC) is one of the most important sources of entangled photons in quantum optics and underpins a wide range of applications in quantum communication, quantum imaging, quantum sensing, and photonic quantum information processing. In this nonlinear optical process, a pump photon is converted into a pair of lower-energy photons that exhibit strong correlations in multiple degrees of freedom. While the generation of photon pairs is governed by energy and momentum conservation, the resulting biphoton state possesses a rich spatial structure whose properties are determined by the interplay among the pump field, the nonlinear medium, and subsequent propagation. This thesis investigates the spatial properties of entangled photon pairs generated through SPDC, focusing on the evolution of their correlations in the near field and on the behavior of orbital-angular-momentum (OAM) entangled states under tight focusing conditions. A common theme throughout this work is the examination of physical effects that emerge when the full biphoton wavefunction is retained rather than reduced through the simplifying approximations often employed in theoretical treatments. The principal contribution of this thesis concerns the near-field propagation of SPDC photon pairs. The spatial correlations of SPDC-generated photons are commonly analyzed within the thin-crystal approximation, where the biphoton wavefunction is assumed to factorize into independent functions of the sum and difference coordinates. We demonstrate that birefringence-induced transverse walk-off breaks this factorization and introduces an intrinsic coupling between these coordinates. More importantly, this coupling survives free-space propagation and remains observable even for crystals that nominally satisfy the thin-crystal condition. As a result, the joint spatial correlations develop a characteristic tapering near the crystal image plane that cannot be captured by conventional factorized models. Numerical simulations and experimental measurements are found to be in excellent agreement, revealing a previously overlooked feature of SPDC and providing a more complete description of photon-pair generation and propagation in birefringent nonlinear media. The second part of the thesis explores the propagation of OAM-entangled photon pairs beyond the paraxial regime. While OAM correlations are typically studied under weak-focusing conditions, many emerging quantum technologies require structured quantum states to be manipulated in highly confined optical systems. We show that tight focusing modifies the OAM correlation spectrum, leading to a broadening of the accessible mode distribution. This broadening exhibits distinct transverse and longitudinal characteristics and arises from the emergence of nonparaxial field components absent in conventional scalar descriptions. These results provide new insight into the behavior of structured quantum light in strongly focused optical fields and establish a framework for understanding OAM entanglement beyond the paraxial approximation. Together, the results presented in this thesis reveal previously unexplored aspects of the structure and propagation of entangled photon pairs. By moving beyond widely used approximations, this work uncovers physical effects that influence the generation, evolution, and measurement of spatially entangled states, with implications for quantum imaging, high-dimensional quantum communication, and the broader development of structured-light-based quantum technologies.
Spontaneous parametric down-conversion is the primary source of position-correlated and momentum-anti-correlated photon pairs that form the canonical Einstein-Podolsky-Rosen (EPR) state. Their transverse spatial correlations are usually analyzed within the thin-crystal approximation, where the two-photon wavefunction is assumed to factorize into independent functions of the sum and difference coordinates. In practice, however, birefringence-induced transverse walk-off breaks this factorization and couples these degrees of freedom. Here, we show that this coupling persists even for nominally thin crystals once the free-space propagation of the joint spatial intensity is taken into account. This sum-difference coordinate coupling leads to a distinctive tapering of the transverse correlations near the crystal image plane - an effect that standard factorized models cannot capture. Numerical simulations and experimental data clearly confirm this novel behavior. Our findings provide a more complete description of photon-pair generation in birefringent nonlinear media and clarify fundamental limits on spatially resolved quantum imaging and spatial-mode quantum information processing with EPR states.
Spontaneous parametric down-conversion is the primary source of position-correlated and momentum-anticorrelated photon pairs that form the canonical Einstein-Podolsky-Rosen (EPR) state. Their transverse spatial correlations are usually analyzed within the thin-crystal approximation, where the two-photon wavefunction is assumed to factorize into independent functions of the sum and difference coordinates. In practice, however, birefringence-induced transverse walk-off breaks this factorization and couples these degrees of freedom. Here, we show that this coupling persists even for nominally thin crystals once the free-space propagation of the joint spatial intensity is taken into account. This sum-difference coordinate coupling leads to a distinctive tapering of the transverse correlations near the crystal image plane-an effect that standard factorized models cannot capture. Numerical simulations and experimental data clearly confirm this novel behavior. Our findings provide a more complete description of photon-pair generation in birefringent nonlinear media and clarify fundamental limits on spatially resolved quantum imaging and spatial-mode quantum information processing with EPR states.
Abstract Spontaneous parametric down-conversion (SPDC) is the most widely used process for generating photon pairs entangled in various degrees of freedom such as polarization, time-energy, position-transverse momentum, and angle-orbital angular momentum (OAM). In SPDC, a pump photon interacts with a non-linear optical crystal and splits into two entangled photons called the signal and the idler photons. The SPDC process has been studied extensively in the last few decades for various pump and crystal configurations, and the entangled photon pairs produced by SPDC have been used in numerous experimental studies on quantum entanglement and entanglement-based real-world quantum-information applications. In this tutorial article, we present a thorough study of phase matching in BBO crystals for spontaneous parametric down-conversion and thereby also investigate the generation of entangled photons in such crystals. First, we present a theoretical derivation of two-photon wavefunction produced by SPDC in the frequency and transverse momentum bases. We then discuss in detail the effects due to various crystal and pump parameters including the length of the crystal, the angle between the optic axis and the pump propagation direction, the pump incidence angle on the crystal surface, the refraction at the crystal surfaces, and the pump propagation direction inside the crystal. These effects are extremely relevant in experimental situations. We then present our numerical and experimental results in order to illustrate how various experimental parameters affect the phase matching and thus the generation of entangled photons. Finally, using the two-photon wavefunction in the transverse wave-vector basis, we show how to derive the two-photon wavefunction in the OAM basis and thereby calculate the two-photon angular Schmidt spectrum. We expect this article to be useful for researchers working in various capacities with entangled photons generated by SPDC in BBO crystals.
Entanglement generated by Spontaneous Parametric Down Conversion (SPDC) involves multiple, often mutually correlated degrees of freedom. These degrees of freedom are often treated independently, overlooking the intrinsic correlation between them. We focus on the spatial spectral correlations that, if left uncontrolled, introduce distinguishability and reduce coherence, undermining applications such as high-dimensional OAM encoding. We analyze the spatio spectral structure of the biphoton and identify source configurations enabling a strong reduction of such correlations. We then quantify how spatial spectral coupling degrades OAM spatial purity, mapping high-purity regions as functions of OAM order, crystal length, and pump/collection waists. The resulting design parameters enable engineering bright, high purity OAM entangled sources, reducing the need for loss-introducing filtering and therefore supporting scalable high-dimensional photonic quantum technologies.
Spatial correlations of photon pairs from spontaneous parametric down-conversion (SPDC) underpin quantum imaging and entanglement certification. We present the first systematic study of spectral filter bandwidth effects on transverse spatial correlations in bulk Type-I BBO for degenerate and non-degenerate configurations. In the far field, the degenerate conditional momentum width is pump-limited and filter-invariant, while non-degenerate configurations exhibit monotonic growth in both marginal and conditional momentum widths -- with the walk-off axis ≈100\approx 100≈100 times more sensitive than the non-walk-off axis. In the near field, we identify a previously unreported flat-dip-rise profile: the conditional position width narrows by ≈10%\approx 10\%≈10% at an optimal bandwidth Δdip≈1.35 ΔλSPDCΔ_\mathrm{dip} \approx 1.35\,Δλ_\mathrm{SPDC}Δdip​≈1.35ΔλSPDC​ before rising due to geometric displacement. When the filter is placed on the idler arm, the dip shifts by the exact factor (λi/λs)2(λ_i/λ_s)^2(λi​/λs​)2. Both results are universal for any non-degenerate SPDC source, requiring only a finite crystal length, dθ/dλ≠0dθ/dλ\neq 0dθ/dλ=0, and incoherent spectral averaging. The Reid EPR uncertainty product is consistently smaller on the walk-off axis -- a structural advantage of bulk birefringent geometry absent in quasi-phase-matched sources. The optimal filter bandwidth ΔF=ΔdipΔ_F = Δ_\mathrm{dip}ΔF​=Δdip​ is determined entirely by the intrinsic phase-matching bandwidth of the crystal and is directly readable from the X-entanglement spectral width of the source.
Summary form only given. Spontaneous parametric down-conversion (SPDC), one of the most important nonlinear processes, is of paramount interest especially in the field of quantum optics due to its intrinsic capability in generating entangled photon pairs in different degree of freedoms (DoFs). The spatial distribution of the paired photons generated through SPDC process are highly influenced by different crystal parameters including birefringence and length, and the spatial structure of the pump beam [1]. Recent studies have shown the transfer of pump properties such as phase profile and doughnut intensity distribution [2] into the transverse amplitude of heralded single photon. Here we report, first time to best of our knowledge, the direct transfer of the non-separable state in OAM and polarization DoFs of classical pump beam to generate two photons state with hybrid entanglement in both OAM and polarization. Using same scheme one can produce macroscopic entanglement with very high quanta of OAM.