Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2603.04578

High Purity OAM Entangled Photons from SPDC with Reduced Spatial Spectral Correlations

F. Crislane V. de Brito, Sylwia Kolenderska, Piotr Kolenderski

quant-phphysics.opticsSubmitted Mar 4, 2026• Announced Mar 6, 2026• 0 citations
arXivHTMLPDF

Abstract

Entanglement generated by Spontaneous Parametric Down Conversion (SPDC) involves multiple, often mutually correlated degrees of freedom. These degrees of freedom are often treated independently, overlooking the intrinsic correlation between them. We focus on the spatial spectral correlations that, if left uncontrolled, introduce distinguishability and reduce coherence, undermining applications such as high-dimensional OAM encoding. We analyze the spatio spectral structure of the biphoton and identify source configurations enabling a strong reduction of such correlations. We then quantify how spatial spectral coupling degrades OAM spatial purity, mapping high-purity regions as functions of OAM order, crystal length, and pump/collection waists. The resulting design parameters enable engineering bright, high purity OAM entangled sources, reducing the need for loss-introducing filtering and therefore supporting scalable high-dimensional photonic quantum technologies.

Related papers

Enhancing the purity of single photons in parametric down-conversion through simultaneous pump-beam and crystal-domain engineering

Baghdasar Baghdasaryan, Fabian Steinlechner, S. Fritzsche

Spontaneous parametric down-conversion (SPDC) has shown great promise in the generation of pure and indistinguishable single photons. Photon pairs produced in bulk crystals are highly correlated in terms of transverse space and frequency. These correlations limit the indistinguishability of photons and result in inefficient photon sources. Domain-engineered crystals with a Gaussian nonlinear response have been explored to minimize spectral correlations. Here we study the impact of such domain engineering on spatial correlations of generated photons. We show that crystals with a Gaussian nonlinear response reduce the spatial correlations between photons. However, the Gaussian nonlinear response is not sufficient to fully eliminate the spatial correlations. Therefore, the development of a comprehensive method to minimize these correlations remains an open challenge. Our solution to this problem involves simultaneous engineering of the pump beam and crystal. We achieve purity of single-photon state up to 99% without any spatial filtering. Our findings provide valuable insights into the spatial waveform generated in structured SPDC crystals, with implications for applications such as boson sampling.

arXiv:2306.15569•Physical Review A•Aug 18, 2023•11 citations

Evolution of Spatially Entangled Photons Beyond Standard Approximations

Christian Howard

Spontaneous parametric down-conversion (SPDC) is one of the most important sources of entangled photons in quantum optics and underpins a wide range of applications in quantum communication, quantum imaging, quantum sensing, and photonic quantum information processing. In this nonlinear optical process, a pump photon is converted into a pair of lower-energy photons that exhibit strong correlations in multiple degrees of freedom. While the generation of photon pairs is governed by energy and momentum conservation, the resulting biphoton state possesses a rich spatial structure whose properties are determined by the interplay among the pump field, the nonlinear medium, and subsequent propagation. This thesis investigates the spatial properties of entangled photon pairs generated through SPDC, focusing on the evolution of their correlations in the near field and on the behavior of orbital-angular-momentum (OAM) entangled states under tight focusing conditions. A common theme throughout this work is the examination of physical effects that emerge when the full biphoton wavefunction is retained rather than reduced through the simplifying approximations often employed in theoretical treatments. The principal contribution of this thesis concerns the near-field propagation of SPDC photon pairs. The spatial correlations of SPDC-generated photons are commonly analyzed within the thin-crystal approximation, where the biphoton wavefunction is assumed to factorize into independent functions of the sum and difference coordinates. We demonstrate that birefringence-induced transverse walk-off breaks this factorization and introduces an intrinsic coupling between these coordinates. More importantly, this coupling survives free-space propagation and remains observable even for crystals that nominally satisfy the thin-crystal condition. As a result, the joint spatial correlations develop a characteristic tapering near the crystal image plane that cannot be captured by conventional factorized models. Numerical simulations and experimental measurements are found to be in excellent agreement, revealing a previously overlooked feature of SPDC and providing a more complete description of photon-pair generation and propagation in birefringent nonlinear media. The second part of the thesis explores the propagation of OAM-entangled photon pairs beyond the paraxial regime. While OAM correlations are typically studied under weak-focusing conditions, many emerging quantum technologies require structured quantum states to be manipulated in highly confined optical systems. We show that tight focusing modifies the OAM correlation spectrum, leading to a broadening of the accessible mode distribution. This broadening exhibits distinct transverse and longitudinal characteristics and arises from the emergence of nonparaxial field components absent in conventional scalar descriptions. These results provide new insight into the behavior of structured quantum light in strongly focused optical fields and establish a framework for understanding OAM entanglement beyond the paraxial approximation. Together, the results presented in this thesis reveal previously unexplored aspects of the structure and propagation of entangled photon pairs. By moving beyond widely used approximations, this work uncovers physical effects that influence the generation, evolution, and measurement of spatially entangled states, with implications for quantum imaging, high-dimensional quantum communication, and the broader development of structured-light-based quantum technologies.

•Aug 24, 2026•0 citations

Joint spectrum mapping of polarization entanglement in spontaneous parametric down-conversion

Hou Shun Poh, Chune Yang Lum, I. Marcikic +2 more

Polarization-entangled photon pairs can be efficiently prepared into pure Bell states with a high fidelity via type-II spontaneous parametric down-conversion (SPDC) of narrow-band pump light. However, the use of femtosecond pump pulses to generate multiphoton states with precise timing often requires spectral filtering to maintain a high quality of polarization entanglement. This typically reduces the efficiency of photon pair collection. We experimentally map the polarization correlations of photon pairs from such a source over a range of down-converted wavelengths with a high spectral resolution and find strong polarization correlations everywhere. A spectrally dependent imbalance between contributions from the two possible decay paths of SPDC is identified as the reason for a reduction in entanglement quality observed with femtosecond pump pulses. Our spectral measurements allow us to predict the polarization correlations for arbitrary filter profiles when the frequency degree of freedom of the photon pairs is ignored.

arXiv:quant-ph/0608009•Physical Review A•Apr 26, 2007•47 citations

Bright photon pair source with high spectral and spatial purity

J. Schaake, Ryan S. Bennink, Philip G. Evans +2 more

Spontaneous parametric down-conversion (SPDC) is a reliable and robust source of photons for quantum information applications. For applications that involve operations such as entanglement swapping or single-photon heralding, two-photon states are required to be factorable (uncorrelated) in their spectral and spatial degrees of freedom. We report the design and experimental characterization of an SPDC source that has been optimized for high spectral and spatial purity. The source is pumped by the 776 nm output of a mode-locked Ti:Sapphire laser and consists of a periodically-poled Potassium Titanyl Phosphate (PPKTP) crystal phase-matched for collinear type-II SPDC. The dispersive properties of PPKTP at these wavelengths is such that it is possible to minimize the spectral entanglement by matching the widths of the pump to the spectral phase-matching function. The spatial entanglement is minimized through careful control of the pump focus, yielding nearly single-mode emission. An advantage of this approach is that the emission rate into the collection modes is very high, resulting in a very bright SPDC source. We also report a scheme that employs the output of collinear sources such as these to produce polarization-entangled photon pairs. The scheme, which requires only simple polarization elements, can be scaled to N-photon GHZ states.

Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE•May 13, 2011•1 citation

Gaussian mode coupling of spectrally broadband photons from bulk spontaneous parametric down-conversion: A spatial-spectral mode analysis of fiber coupling

Carlos Sevilla-Gutiérrez, Varun Raj Kaipalath, Fabian Steinlechner

Photon sources based on spontaneous parametric down-conversion (SPDC) are central to experimental quantum optics and quantum technologies. Their performance is commonly quantified by three metrics: pair-collection probability, heralding efficiency, and spectral purity. In bulk-crystal SPDC, these metrics are known to be mutually constrained, yet the physical origin of the resulting trade-offs is often obscured. We show that these trade-offs originate from the frequency-dependent population of discrete spatial modes in the SPDC emission. By performing a Laguerre-Gauss mode decomposition at each frequency component, we show how spectral-spatial non-separability impacts collection probability, heralding efficiency, and purity. We apply this framework to two widely used quasi-phase-matching configurations: collinear degenerate type-0 and type-II SPDC in periodically poled bulk crystals, and quantify how different phase-matching functions shape the spectral-spatial mode structure. In particular, for type-II SPDC we compare standard periodically poled and aperiodically poled Gaussian phase matching. We experimentally validate some of our theoretical results using spatial- and spectral-projection measurements. This spectral-spatial mode analysis provides a quantitative and predictive framework for understanding and engineering bulk-crystal photon sources, enabling systematic multi-parameter optimization beyond qualitative design guidelines.

quant-pharXiv:2602.23238•Physical Review A•Feb 27, 2026•1 citation

Design of bright, fiber-coupled and fully factorable photon pair sources

Luis Edgar Vicent, Alfred B. U’Ren, Radhika Rangarajan +4 more

From quantum computation to quantum key distribution, many quantum-enhanced applications rely on the ability to generate pure single photons. Even though the process of spontaneous parametric downconversion (SPDC) is widely used as the basis for photon-pair sources, the conditions for pure heralded single-photon generation, taking into account both spectral and spatial degrees of freedom, have not been fully described. We present an analysis of the spatio-temporal correlations present in photon pairs produced by type-I, non-collinear SPDC. We derive a set of conditions for full factorability in all degrees of freedom—required for the heralding of pure single photons—between the signal and idler modes. In this paper, we consider several possible approaches for the design of bright, fiber-coupled and factorable photon-pair sources. We show through numerical simulations of the exact equations that sources based on: (i) the suppression of spatio-temporal entanglement according to our derived conditions and (ii) a tightly focused pump beam together with optimized fiber-collection modes and spectral filtering of the signal and idler photon pairs, lead to a source brightness of the same order of magnitude. Likewise, we find that both of these sources lead to a drastically higher factorable photon-pair flux, compared to an unengineered source.

New Journal of Physics•Sep 15, 2010•46 citations
Entanglement generated by Spontaneous Parametric Down Conversion (SPDC) involves multiple, often mutually correlated degrees of freedom. These degrees of freedom are often treated independently, overlooking the intrinsic correlation between them. We focus on the spatial spectral correlations that, if left uncontrolled, introduce distinguishability and reduce coherence, undermining applications such as high-dimensional OAM encoding. We analyze the spatio spectral structure of the biphoton and identify source configurations enabling a strong reduction of such correlations. We then quantify how spatial spectral coupling degrades OAM spatial purity, mapping high-purity regions as functions of OAM order, crystal length, and pump/collection waists. The resulting design parameters enable engineering bright, high purity OAM entangled sources, reducing the need for loss-introducing filtering and therefore supporting scalable high-dimensional photonic quantum technologies.
Spontaneous parametric down-conversion (SPDC) has shown great promise in the generation of pure and indistinguishable single photons. Photon pairs produced in bulk crystals are highly correlated in terms of transverse space and frequency. These correlations limit the indistinguishability of photons and result in inefficient photon sources. Domain-engineered crystals with a Gaussian nonlinear response have been explored to minimize spectral correlations. Here we study the impact of such domain engineering on spatial correlations of generated photons. We show that crystals with a Gaussian nonlinear response reduce the spatial correlations between photons. However, the Gaussian nonlinear response is not sufficient to fully eliminate the spatial correlations. Therefore, the development of a comprehensive method to minimize these correlations remains an open challenge. Our solution to this problem involves simultaneous engineering of the pump beam and crystal. We achieve purity of single-photon state up to 99% without any spatial filtering. Our findings provide valuable insights into the spatial waveform generated in structured SPDC crystals, with implications for applications such as boson sampling.
Spontaneous parametric down-conversion (SPDC) is one of the most important sources of entangled photons in quantum optics and underpins a wide range of applications in quantum communication, quantum imaging, quantum sensing, and photonic quantum information processing. In this nonlinear optical process, a pump photon is converted into a pair of lower-energy photons that exhibit strong correlations in multiple degrees of freedom. While the generation of photon pairs is governed by energy and momentum conservation, the resulting biphoton state possesses a rich spatial structure whose properties are determined by the interplay among the pump field, the nonlinear medium, and subsequent propagation. This thesis investigates the spatial properties of entangled photon pairs generated through SPDC, focusing on the evolution of their correlations in the near field and on the behavior of orbital-angular-momentum (OAM) entangled states under tight focusing conditions. A common theme throughout this work is the examination of physical effects that emerge when the full biphoton wavefunction is retained rather than reduced through the simplifying approximations often employed in theoretical treatments. The principal contribution of this thesis concerns the near-field propagation of SPDC photon pairs. The spatial correlations of SPDC-generated photons are commonly analyzed within the thin-crystal approximation, where the biphoton wavefunction is assumed to factorize into independent functions of the sum and difference coordinates. We demonstrate that birefringence-induced transverse walk-off breaks this factorization and introduces an intrinsic coupling between these coordinates. More importantly, this coupling survives free-space propagation and remains observable even for crystals that nominally satisfy the thin-crystal condition. As a result, the joint spatial correlations develop a characteristic tapering near the crystal image plane that cannot be captured by conventional factorized models. Numerical simulations and experimental measurements are found to be in excellent agreement, revealing a previously overlooked feature of SPDC and providing a more complete description of photon-pair generation and propagation in birefringent nonlinear media. The second part of the thesis explores the propagation of OAM-entangled photon pairs beyond the paraxial regime. While OAM correlations are typically studied under weak-focusing conditions, many emerging quantum technologies require structured quantum states to be manipulated in highly confined optical systems. We show that tight focusing modifies the OAM correlation spectrum, leading to a broadening of the accessible mode distribution. This broadening exhibits distinct transverse and longitudinal characteristics and arises from the emergence of nonparaxial field components absent in conventional scalar descriptions. These results provide new insight into the behavior of structured quantum light in strongly focused optical fields and establish a framework for understanding OAM entanglement beyond the paraxial approximation. Together, the results presented in this thesis reveal previously unexplored aspects of the structure and propagation of entangled photon pairs. By moving beyond widely used approximations, this work uncovers physical effects that influence the generation, evolution, and measurement of spatially entangled states, with implications for quantum imaging, high-dimensional quantum communication, and the broader development of structured-light-based quantum technologies.
Polarization-entangled photon pairs can be efficiently prepared into pure Bell states with a high fidelity via type-II spontaneous parametric down-conversion (SPDC) of narrow-band pump light. However, the use of femtosecond pump pulses to generate multiphoton states with precise timing often requires spectral filtering to maintain a high quality of polarization entanglement. This typically reduces the efficiency of photon pair collection. We experimentally map the polarization correlations of photon pairs from such a source over a range of down-converted wavelengths with a high spectral resolution and find strong polarization correlations everywhere. A spectrally dependent imbalance between contributions from the two possible decay paths of SPDC is identified as the reason for a reduction in entanglement quality observed with femtosecond pump pulses. Our spectral measurements allow us to predict the polarization correlations for arbitrary filter profiles when the frequency degree of freedom of the photon pairs is ignored.
Spontaneous parametric down-conversion (SPDC) is a reliable and robust source of photons for quantum information applications. For applications that involve operations such as entanglement swapping or single-photon heralding, two-photon states are required to be factorable (uncorrelated) in their spectral and spatial degrees of freedom. We report the design and experimental characterization of an SPDC source that has been optimized for high spectral and spatial purity. The source is pumped by the 776 nm output of a mode-locked Ti:Sapphire laser and consists of a periodically-poled Potassium Titanyl Phosphate (PPKTP) crystal phase-matched for collinear type-II SPDC. The dispersive properties of PPKTP at these wavelengths is such that it is possible to minimize the spectral entanglement by matching the widths of the pump to the spectral phase-matching function. The spatial entanglement is minimized through careful control of the pump focus, yielding nearly single-mode emission. An advantage of this approach is that the emission rate into the collection modes is very high, resulting in a very bright SPDC source. We also report a scheme that employs the output of collinear sources such as these to produce polarization-entangled photon pairs. The scheme, which requires only simple polarization elements, can be scaled to N-photon GHZ states.
Photon sources based on spontaneous parametric down-conversion (SPDC) are central to experimental quantum optics and quantum technologies. Their performance is commonly quantified by three metrics: pair-collection probability, heralding efficiency, and spectral purity. In bulk-crystal SPDC, these metrics are known to be mutually constrained, yet the physical origin of the resulting trade-offs is often obscured. We show that these trade-offs originate from the frequency-dependent population of discrete spatial modes in the SPDC emission. By performing a Laguerre-Gauss mode decomposition at each frequency component, we show how spectral-spatial non-separability impacts collection probability, heralding efficiency, and purity. We apply this framework to two widely used quasi-phase-matching configurations: collinear degenerate type-0 and type-II SPDC in periodically poled bulk crystals, and quantify how different phase-matching functions shape the spectral-spatial mode structure. In particular, for type-II SPDC we compare standard periodically poled and aperiodically poled Gaussian phase matching. We experimentally validate some of our theoretical results using spatial- and spectral-projection measurements. This spectral-spatial mode analysis provides a quantitative and predictive framework for understanding and engineering bulk-crystal photon sources, enabling systematic multi-parameter optimization beyond qualitative design guidelines.
From quantum computation to quantum key distribution, many quantum-enhanced applications rely on the ability to generate pure single photons. Even though the process of spontaneous parametric downconversion (SPDC) is widely used as the basis for photon-pair sources, the conditions for pure heralded single-photon generation, taking into account both spectral and spatial degrees of freedom, have not been fully described. We present an analysis of the spatio-temporal correlations present in photon pairs produced by type-I, non-collinear SPDC. We derive a set of conditions for full factorability in all degrees of freedom—required for the heralding of pure single photons—between the signal and idler modes. In this paper, we consider several possible approaches for the design of bright, fiber-coupled and factorable photon-pair sources. We show through numerical simulations of the exact equations that sources based on: (i) the suppression of spatio-temporal entanglement according to our derived conditions and (ii) a tightly focused pump beam together with optimized fiber-collection modes and spectral filtering of the signal and idler photon pairs, lead to a source brightness of the same order of magnitude. Likewise, we find that both of these sources lead to a drastically higher factorable photon-pair flux, compared to an unengineered source.