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arXiv:2507.23144 · Physical Review Letters

Geometric Phase in Anisotropic Kepler Problem: Perspective for Realization in Rydberg Atoms

Nikolai A. Sinitsyn, Fumika Suzuki

Published Nov 17, 2025• 0 citations
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Abstract

We predict a gyroscopic effect that can be demonstrated with Rydberg atoms following the dynamics of a Kepler Hamiltonian with an additional uniaxial anisotropy induced by optical ponderomotive force. This effect is analogous to the rotation of the Foucault pendulum in response to the Earth's rotation. We argue that in Rydberg states with a large principal quantum number a similar geometric angle can be generated by mechanical rotations of an atomic-optical setup on timescales between 1 μs and 1 ms.

DOI
10.1103/1jxx-smg7

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•Oct 6, 2023•0 citations
We predict a gyroscopic effect that can be demonstrated with Rydberg atoms following the dynamics of a Kepler Hamiltonian with an additional uniaxial anisotropy induced by optical ponderomotive force. This effect is analogous to the rotation of the Foucault pendulum in response to the Earth's rotation. We argue that in Rydberg states with a large principal quantum number a similar geometric angle can be generated by mechanical rotations of an atomic-optical setup on timescales between 1 μs and 1 ms.
Abstract Perspective methods of quantum metrology are highly suitable for designing new types of gyroscopes. Matter waves-based gyroscopic schemes have already been implemented in optical setups. In the nearing future, it might be possible to implement them with macroscopic coherent structures of atomic Bose-Einstein condensates (BECs). This work considers a ring-shaped BEC configuration interrupted by a localized potential “defect.” It is shown that variation of the shape of this “defect” generates atomic geometric phase. In a pair of such configurations opposite geometric phases may be obtained, with their difference equal to zero in absence of rotation. This difference can be revealed by observing interference of the atoms from different configurations. Calculation of resulting geometric phases is carried out for a model “defect” in a ring of 0.5 cm diameter detecting Earth’s diurnal rotation.
Stokes parameter formalism is applied to show the analogies between the motion of an asymmetric Foucault pendulum and several phenomena known from optics and atomic physics. Nonlinearity-induced precession of elliptical orbits of the pendulum is shown to correspond to twisting transformations used for spin squeezing of atomic systems. Transitions between regimes of predominant nonlinearity and regimes where the Coriolis force or the asymmetry of the pendulum are dominant correspond to quantum phase transitions in the Lipkin-Meshkov-Glick model. A Foucault pendulum with highly anisotropic damping can emulate an optical Zeno effect where a sequence of polarizing filters inhibits polarization rotation of light in an optically active medium.
The quantum theory of atoms is based on a Hamiltonian which is just that of the classical Kepler theory of planetary orbits. In spite of this common foundation, the predictions of quantum theory ordinarily do not much resemble those of classical theory. Even in the limit of large quantum numbers the energy eigenstates of quantum theory do not look at all like the classical elliptical orbits. Recently, Parker and Stroud1 have shown that it is possible to excite a Rydberg atom wave packet whose radial dependence resembles the classical ideal of a particle traveling in an elliptical orbit. In this paper we discuss the formation of a wave packet in the polar and azimuthal angles by the coherent excitation of Rydberg states with the same principal quantum, but with a distribution of the angular momentum quantum numbers. When this wave packet is formed of the Rydberg states of an alkali atom the connection with classical theory is again striking. The wave packet precesses due to the core polarization, just as the classical elliptical orbit precesses due to an added r–4 perturbing potential.
We discuss three proposed schemes of initializing circular-state Rydberg atoms via optical couplings provided by the ponderomotive effect in contrast to the current circularization methods that utilize electric-dipole interactions. In our first proposed method, a radial optical trap consisting of two Laguerre-Gaussian beams of opposite winding numbers transfers orbital angular momentum to the Rydberg atom, providing a first-order coherent coupling between an F state and a circular state. Additionally, we propose a one-dimensional ponderomotive optical lattice modulated at rf frequencies, providing quadrupolelike couplings in the hydrogenic manifold for rapid adiabatic passage through a series of intermediate Rydberg states into the circular state. For the third proposed scheme, a two-dimensional ponderomotive optical lattice with a time-orbiting trap center induces effectively the same coupling as a ${\ensuremath{\sigma}}^{+}$- or ${\ensuremath{\sigma}}^{\ensuremath{-}}$-polarized rf field of tunable purity for all-optical rapid adiabatic passage into the circular state.
Laser cooling and trapping of atomic matter waves in optical potentials has enabled rapid progress in quantum science, particularly when combined with Rydberg excitation of the atoms to induce long-range interactions. Here, we propose the local manipulation and spatiotemporal sculpting of the electronic matter wave of a Rydberg atom by a laser field focused so that its beam width is smaller than the Rydberg electron orbit. We compute the electronic eigenstates in the presence of a sharply focused Gaussian laser beam, and find strong Rydberg state mixing leading to large kilo-Debye dipole moments. These can be modulated with high bandwidth controlled by the local tweezer intensity. Oscillations in the position-dependent level shifts, analogous to the potential wells allowing ultralong-range Rydberg molecules to form, provide opportunities for eccentric radial trapping of the Rydberg electron via ponderomotive forces acting on suborbital length scales.
Circular Rydberg atoms, with their long lifetimes and adjustable strong dipolar interactions, are promising candidates for the implementation of quantum simulations in regimes that were previously out of reach. A new quantum simulator paradigm, based on qubits encoded in circular states, would implement an XXZ spin-1/2 Hamiltonian with dynamically adjustable parameters over a wide range of values. This thesis addresses the preliminary steps in constructing such a quantum simulator. First, we present the realization of two-dimensional arrays of optically-trapped circular Rydberg atoms with arbitrary geometries. For this purpose, we prepare arrays of ultra-cold rubidium atoms, individually trapped in optical tweezers. An additional beam with adjustable position allows us to rearrange the atoms within the array to implement the desired geometry in a deterministic manner. We then excite the atoms to the circular state with principal quantum number n=52, while trapping them in hollow beams using the ponderomotive force. These experimental capabilities allowed us to control and characterize, for the first time, the dipolar interactions between circular states, within pairs of individually trapped atoms. We showed the good agreement of these measurements with theoretical expectations and highlighted their dependence on the system's geometry. This experimental study is coupled to an investigation of the motion of the circular atoms within their traps.