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arXiv:1909.06612 · Physical Review A

Circularizing Rydberg atoms with time-dependent optical traps

Ryan Cardman, Georg A. Raithel

Published Jan 30, 2020• 24 citations
arXivHTMLPDF

Abstract

We discuss three proposed schemes of initializing circular-state Rydberg atoms via optical couplings provided by the ponderomotive effect in contrast to the current circularization methods that utilize electric-dipole interactions. In our first proposed method, a radial optical trap consisting of two Laguerre-Gaussian beams of opposite winding numbers transfers orbital angular momentum to the Rydberg atom, providing a first-order coherent coupling between an F state and a circular state. Additionally, we propose a one-dimensional ponderomotive optical lattice modulated at rf frequencies, providing quadrupolelike couplings in the hydrogenic manifold for rapid adiabatic passage through a series of intermediate Rydberg states into the circular state. For the third proposed scheme, a two-dimensional ponderomotive optical lattice with a time-orbiting trap center induces effectively the same coupling as a ${\ensuremath{\sigma}}^{+}$- or ${\ensuremath{\sigma}}^{\ensuremath{-}}$-polarized rf field of tunable purity for all-optical rapid adiabatic passage into the circular state.

DOI
10.1103/physreva.101.013434

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We discuss three proposed schemes of initializing circular-state Rydberg atoms via optical couplings provided by the ponderomotive effect in contrast to the current circularization methods that utilize electric-dipole interactions. In our first proposed method, a radial optical trap consisting of two Laguerre-Gaussian beams of opposite winding numbers transfers orbital angular momentum to the Rydberg atom, providing a first-order coherent coupling between an F state and a circular state. Additionally, we propose a one-dimensional ponderomotive optical lattice modulated at rf frequencies, providing quadrupolelike couplings in the hydrogenic manifold for rapid adiabatic passage through a series of intermediate Rydberg states into the circular state. For the third proposed scheme, a two-dimensional ponderomotive optical lattice with a time-orbiting trap center induces effectively the same coupling as a \ensuremathσ+{\ensuremath{\sigma}}^{+}\ensuremathσ+- or \ensuremathσ\ensuremath−{\ensuremath{\sigma}}^{\ensuremath{-}}\ensuremathσ\ensuremath−-polarized rf field of tunable purity for all-optical rapid adiabatic passage into the circular state.
Quantum simulation offers interesting perspectives for the understanding of complex systems that are out of reach for numerical approaches. In this line, a new quantum simulation platform has recently been proposed. A spin-1/2 XXZ hamiltonian is thus realized in which the parameters can be controlled over a large range. The spin states are encoded by circular Rydberg states coupled through dipole-dipole interaction. These states benefit from longer lifetimes compared to the low angular momentum states used for current quantum simulations. In addition, they can be laser-trapped through the ponderomotive effect, and their lifetime can be further enhanced by spontaneous emission inhibition. We present in this thesis the first step towards the implementation of the proposed quantum simulator. We first prepare an array of rubidium 87 atoms trapped individually in optical tweezers. These atoms are subsequently excited to the circular Rydberg state n = 52 and transferred to hollow bottle-beam traps. We thus demonstrate the ponderomotive trapping of these states over durations of several milliseconds. We take advantage of the optical detection of the states thus prepared with various experiments. We characterize the trapping potential by measuring its transverse frequency. We finally conclude with the coherent manipulation of these trapped circular states through Rabi oscillations and Ramsey interferometry to determine their coherence.
Circular Rydberg atoms, with their long lifetimes and adjustable strong dipolar interactions, are promising candidates for the implementation of quantum simulations in regimes that were previously out of reach. A new quantum simulator paradigm, based on qubits encoded in circular states, would implement an XXZ spin-1/2 Hamiltonian with dynamically adjustable parameters over a wide range of values. This thesis addresses the preliminary steps in constructing such a quantum simulator. First, we present the realization of two-dimensional arrays of optically-trapped circular Rydberg atoms with arbitrary geometries. For this purpose, we prepare arrays of ultra-cold rubidium atoms, individually trapped in optical tweezers. An additional beam with adjustable position allows us to rearrange the atoms within the array to implement the desired geometry in a deterministic manner. We then excite the atoms to the circular state with principal quantum number n=52, while trapping them in hollow beams using the ponderomotive force. These experimental capabilities allowed us to control and characterize, for the first time, the dipolar interactions between circular states, within pairs of individually trapped atoms. We showed the good agreement of these measurements with theoretical expectations and highlighted their dependence on the system's geometry. This experimental study is coupled to an investigation of the motion of the circular atoms within their traps.
Abstract We propose to trap circular Rydberg atoms (CRAs) via a ponderomotive potential well formed by a superimposed vortex light beam. We analytically calculate the ponderomotive potential energy for a Bessel vortex light beam. We work out a corrected version of the classical circular orbit approximation for a CRA which fits the exact result much better than the usual approximation. We reveal the three-dimensional characteristics of the potential well for some benchmark values of the CRA principal quantum number and beam parameters such as the frequency, the opening angle and topological charge of the vortex. We investigate how we can achieve similar trapping effects for different principal quantum numbers by varying beam parameters. The potential provides a lattice structure along the beam axis where one CRA could be trapped at each lattice site.
Circular Rydberg atoms (CRAs), i.e., Rydberg atoms with maximal orbital momentum, ideally combine long coherence times and strong interactions, a key property of quantum systems, in particular for the development of quantum technologies. However, the dipole-dipole interaction between CRAs has not been observed so far. We report the measurement and characterization of the resonant dipole-dipole interaction between two CRAs, individually trapped in optical tweezers, and find excellent agreement with theoretical predictions. We demonstrate a dynamic control over the strength of the interaction by tuning the orientation of an electric field. We use the interaction between the CRAs as a meter for the interatomic distance, and record the relative motion between two atoms in their traps. This motion, that we induce through the interaction between Rydberg levels with permanent electric dipoles, transiently populated during the preparation of the circular states, is a signature of spin-motion coupling.
Abstract We present a degenerate perturbation analysis in the spin–orbit coupled basis for Rydberg atoms in an optical trap. The perturbation matrix is found to be nearly the same for two states with the same total angular momentum j , and orbital angular momentum number l differing by 1, The same perturbation matrices result in the same state-mixing and energy shift. We also study the dependence of state mixing and energy shift on the periodicity and symmetry of the ponderomotive potentials induced by different optical traps. State mixing in a one-dimensional lattice formed with two counterpropagating Gaussian beams is studied and yields a state-dependent trap depth. We also calculate the state-mixing in an optical trap formed by four parallel, separated and highly focused Gaussian beams.
We calculate the adiabatic potentials and adiabatic wavefunctions of Rydberg atoms in a one-dimensional ponderomotive optical lattice. All lattice-induced couplings between the degenerate high-angular-momentum Rydberg states are taken into account. To obtain insight into the underlying physics, we analyze the numerical results in terms of effective electric and magnetic fields produced by the lattice. Near the inflection points of the lattice potential and for sufficiently low principal quantum numbers ( n ≲35 in the cases studied), the adiabatic level structure resembles that of the dc Stark effect, and an effective electric-field model can be used to model the lattice-induced perturbation. Near the nodes and anti-nodes of the lattice field, the adiabatic level structure exhibits a combination of adjacent rotational and vibrational energy level sequences. Here, an analogy between the ponderomotive optical lattice and the diamagnetic problem works well to interpret the lattice-induced perturbation in terms of an effective magnetic field.