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arXiv:2507.21849

Saturating interaction in coherently coupled two-component Bose-Einstein condensates

Eid, R, S. Tiengo, Lévy, M, Thomas Bourdel

Published Jul 29, 2025• 0 citations
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Abstract

Rabi-coupled spinor Bose-Einstein condensates, with competing intra-and interspecies interactions, enable independent control of two-and three-body interactions. We show that coupling can also drive the system into a strongly nonlinear regime of saturating interaction. More precisely, the equation of state interpolates between low-and high-density regimes described by two different two-body scattering lengths. Interestingly, the transition can be determined by the strength of the coupling. We experimentally demonstrate this saturation phenomenon by measurements of the interaction energy of a Bose-Einstein condensate as a function of the detuning and of the strength of the Rabi coupling in spin mixtures of potassium 39.

DOI
10.48550/arxiv.2507.21849

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Rabi-coupled spinor Bose-Einstein condensates, with competing intra-and interspecies interactions, enable independent control of two-and three-body interactions. We show that coupling can also drive the system into a strongly nonlinear regime of saturating interaction. More precisely, the equation of state interpolates between low-and high-density regimes described by two different two-body scattering lengths. Interestingly, the transition can be determined by the strength of the coupling. We experimentally demonstrate this saturation phenomenon by measurements of the interaction energy of a Bose-Einstein condensate as a function of the detuning and of the strength of the Rabi coupling in spin mixtures of potassium 39.
This thesis investigates the response of coherently coupled spin-mixture Bose-Einstein condensates across a broad range of nonlinear regimes, extending from the deep-Rabi regime to the strongly nonlinear regime. On the theoretical side, collision processes induced and enhanced by strong coherent coupling are analyzed within a perturbative framework. Interaction channels arising from both mean-field and beyond-mean-field processes are identified, providing a microscopic description of the mechanisms through which few-body interactions contribute to the energy of the many-body system. On the experimental side, precise control over the interaction landscape is achieved in a 39-K spin mixture through improved stabilization of the magnetic field near 57 G, the operating point of the system. A feedforward compensation circuit is implemented to suppress magnetic-field noise, and Ramsey spectroscopy measurements demonstrate a twelvefold reduction in field fluctuations, corresponding to a residual root-mean-square noise level of a few tens of μG. This enhanced stability enables controlled measurements of the density-dependent equation of state of the coherently driven two-component condensate. As the density is increased, the system exhibits distinct interaction regimes. At low densities, the equation of state is dominated by repulsive two-body interactions. At intermediate densities, three-body contributions emerge and become increasingly relevant. At higher densities, the interaction energy shows an unusual saturation-like behavior. This behaviour reflects the nontrivial interplay between coherent coupling and interactions.
We propose and demonstrate the appearance of an effective attractive three-body interaction in coherently driven two-component Bose-Einstein condensates. It originates from the spinor degree of freedom that is affected by a two-body mean-field shift of the driven transition frequency. Importantly, its strength can be controlled with the Rabi-coupling strength and it does not come with additional losses. In the experiment, the three-body interactions are adjusted to play a predominant role in the equation of state of a cigar-shaped trapped condensate. This is confirmed through two striking observations: a downshift of the radial breathing mode frequency and the radial collapses for positive values of the dressed-state scattering length.
We theoretically calculate and experimentally measure the beyond-mean-field (BMF) equation of state in a coherently coupled two-component Bose-Einstein condensate (BEC) in the regime where averaging of the interspecies and intraspecies coupling constants over the hyperfine composition of the single-particle dressed state predicts the exact cancellation of the two-body interaction. We show that with increasing the Rabi-coupling frequency ?, the BMF energy density crosses over from the nonanalytic Lee-Huang-Yang scaling ?n5/2 to an expansion in integer powers of density, where, in addition to a two-body BMF term ?n2?, there emerges a repulsive three-body contribution ?n3/?. We experimentally evidence these two contributions, thanks to their different scaling with ?, in the expansion of a Rabi-coupled two-component K39 condensate in a waveguide. By studying the expansion with and without Rabi coupling, we reveal an important feature relevant for observing BMF effects and associated phenomena in mixtures with spin-asymmetric losses: Rabi coupling helps preserve the spin composition and thus prevents the system from drifting away from the point of the vanishing mean field.
We theoretically calculate and experimentally measure the beyond-mean-field (BMF) equation of state in a coherently coupled two-component Bose-Einstein condensate (BEC) in the regime where averaging of the interspecies and intraspecies coupling constants over the hyperfine composition of the single-particle dressed state predicts the exact cancellation of the two-body interaction. We show that with increasing the Rabi-coupling frequency Ω, the BMF energy density crosses over from the nonanalytic Lee-Huang-Yang scaling ∝n^{5/2} to an expansion in integer powers of density, where, in addition to a two-body BMF term ∝n^{2}sqrt[Ω], there emerges a repulsive three-body contribution ∝n^{3}/sqrt[Ω]. We experimentally evidence these two contributions, thanks to their different scaling with Ω, in the expansion of a Rabi-coupled two-component ^{39}K condensate in a waveguide. By studying the expansion with and without Rabi coupling, we reveal an important feature relevant for observing BMF effects and associated phenomena in mixtures with spin-asymmetric losses: Rabi coupling helps preserve the spin composition and thus prevents the system from drifting away from the point of the vanishing mean field.
The dynamics of coherent Rabi oscillations in coupled atomic and molecular Bose-Einstein condensates is considered taking into account the atom-atom, atom-molecule, and molecule-molecule elastic interactions. The exact solution for the molecule formation probability is derived in terms of the elliptic functions. The two-dimensional space of the involved parameters intensity and detuning is analyzed and divided into two regions where the Rabi oscillations show different characteristics. A resonance curve is found, on which the molecular formation probability monotonically increases as a function of time. The maximum value of the final transition probability on this curve is 1∕21∕21∕2 (i.e., total transition to the molecular state) and it is achieved at high field intensities starting from a minimal threshold defined by the interspecies interaction scattering lights. The explicit form of the resonance curve is determined, and it is shown that the resonance frequency position reveals a nonlinear dependence on the Rabi frequency of the applied field. A singular point is found on the resonance curve, where a power-law time evolution of the system is observed.
We study a two-component Bose gas with a symmetric spin-orbit coupling, and find that two atoms can form a bound state with any intra- or inter-species scattering length. Consequently, in the dilute limit, the BCS-pairing state of bosons can be formed with weakly attractive interspecies and repulsive intraspecies interactions. The quasiparticle excitation energies are anisotropic due to spin-orbit coupling. This BCS-pairing state is energetically favored over Bose-Einstein condensation (BEC) of atoms at low densities. As the density increases, there is a first-order transition from the BCS to BEC states.