Transparent conductive oxides (TCO) enable confinement of charge-sensitive ions and Rydberg atoms proximal to dielectric structures including waveguides and photon detectors. However, optical loss precludes the use of TCOs within high-finesse optical micro-resonators. Here we characterize a ZnO-based TCO that markedly reduces optical absorption. At 1650\text{ nm} we observe a 22,000 finesse in a Fabry-Pérot optical cavity coated with a 30\text{ nm} ZnO layer. This is a 5000 times reduction relative to indium tin oxide (ITO) at this wavelength. The same ZnO film exhibits 0.01\text{ \ensuremathΩ\ensuremath{\cdot}cm} surface resistivity at DC. We anticipate a step change in cavity-QED systems incorporating ultra-low loss TCOs like ZnO.
Transparent conductive oxides (TCO) enable confinement of charge-sensitive ions and Rydberg atoms proximal to dielectric structures including waveguides and photon detectors. However, optical loss precludes the use of TCOs within high-finesse optical micro-resonators. Here we characterize a ZnO-based TCO that markedly reduces optical absorption. At 1650\text{ nm} we observe a 22,000 finesse in a Fabry-Pérot optical cavity coated with a 30\text{ nm} ZnO layer. This is a 5000 times reduction relative to indium tin oxide (ITO) at this wavelength. The same ZnO film exhibits 0.01\text{ \ensuremathΩ\ensuremath{\cdot}cm} surface resistivity at DC. We anticipate a step change in cavity-QED systems incorporating ultra-low loss TCOs like ZnO.
Open Fabry-Perot microcavities represent a promising route for achieving a quantum electrodynamics (cavity-QED) platform with diamond-based emitters. In particular, they offer the opportunity to introduce high-purity, minimally fabricated material into a tunable, high quality factor optical resonator. Here, we demonstrate a fiber-based microcavity incorporating a thick ($>10\phantom{\rule{4pt}{0ex}}\ensuremath{\mu}\text{m}$) diamond membrane with a finesse of 17 000, corresponding to a quality factor $Q\ensuremath{\sim}{10}^{6}$. Such minimally fabricated thick samples can contain optically stable emitters similar to those found in bulk diamond. We observe modified microcavity spectra in the presence of the membrane, and we develop analytic and numerical models to describe the effect of the membrane on cavity modes, including loss and coupling to higher-order transverse modes. We estimate that a Purcell enhancement of approximately 20 should be possible for emitters within the diamond in this device, and we provide evidence that better diamond surface treatments and mirror coatings could increase this value to 200 in a realistic system.
Atomic, molecular and optical (AMO) visible light systems are the heart of precision applications including quantum, atomic clocks and precision metrology. As these systems scale in terms of number of lasers, wavelengths, and optical components, their reliability, space occupied, and power consumption will push the limits of using traditional laboratory-scale lasers and optics. Visible light photonic integration is critical to advancing AMO based sciences and applications, yet key performance aspects remain to be addressed, most notably waveguide losses and laser phase noise and stability. Additionally, a visible light integrated solution needs to be wafer-scale CMOS compatible and capable of supporting a wide array of photonic components. While the regime of ultra-low loss has been achieved at telecommunication wavelengths, progress at visible wavelengths has been limited. Here, we report the lowest waveguide losses and highest resonator Qs to date in the visible range, to the best of our knowledge. We report waveguide losses at wavelengths associated with strontium transitions in the 461 nm to 802 nm wavelength range, of 0.01 dB/cm to 0.09 dB/cm and associated intrinsic resonator Q of 60 Million to 9.5 Million, a decrease in loss by factors of 6x to 2x and increase in Q by factors of 10x to 1.5x over this visible wavelength range. Additionally, we measure an absorption limited loss and Q of 0.17 dB/m and 340 million at 674 nm. This level of performance is achieved in a wafer-scale foundry compatible Si 3 N 4 platform with a 20 nm thick core and TEOS-PECVD deposited upper cladding oxide, and enables waveguides for different wavelengths to be fabricated on the same wafer with mask-only changes per wavelength. These results represent a significant step forward in waveguide platforms that operate in the visible, opening up a wide range of integrated applications that utilize atoms, ions and molecules including sensing, navigation, metrology and clocks.
Contemporary experiments in cavity quantum electrodynamics (cavity QED) with gas-phase neutral atoms rely increasingly on laser cooling and optical, magneto-optical or magnetostatic trapping methods to provide atomic localization with sub-micron uncertainty. Difficult to achieve in free space, this goal is further frustrated by atom-surface interactions if the desired atomic placement approaches within several hundred nanometers of a solid surface, as can be the case in setups incorporating monolithic dielectric optical resonators such as microspheres, microtoroids, microdisks or photonic crystal defect cavities. Typically in such scenarios, the smallest atom-surface separation at which the van der Waals interaction can be neglected is taken to be the optimal localization point for associated trapping schemes, but this sort of conservative strategy generally compromises the achievable cavity QED coupling strength. Here we suggest a new approach to the design of optical dipole traps for atom confinement near surfaces that exploits strong surface interactions, rather than avoiding them, and present the results of a numerical study based on (39)K atoms and indium tin oxide (ITO). Our theoretical framework points to the possibility of utilizing nanopatterning methods to engineer novel modifications of atom-surface interactions.
Achieving efficient microwave–optical transduction is a critical challenge for quantum networks where information is shared optically across disparate microwave systems and for coherent optical detection and manipulation of microwave states. Resonant electro-optic systems are being pursued as a means of efficiently bridging these frequencies. Here, we present a platform that employs a bulk lithium niobate crystal whose large dielectric constant creates wavelength-scale confinement of microwave photons. By incorporating this crystal within a high-finesse Fabry–Pérot optical cavity, microwave photons couple to optical photons through the electro-optic effect. We demonstrate the ability to tune our system into triply resonant operation, where microwave photons, optical pump photons, and upconverted optical photons are simultaneously resonant with high quality factor electromagnetic modes of the system. The device achieves photon-number conversion efficiency at the percent level, comparable to that of state-of-the-art devices at room temperature—sufficient to resolve the thermal occupation of the microwave mode—by taking advantage of the high-power handling, low loss, and low noise of all-dielectric devices. These results establish our all-dielectric devices as a promising platform for high-precision sensing of optically detected microwave fields and as a viable route toward single-photon-level microwave–optical quantum transduction.
High-finesse optical cavities placed under vacuum are foundational platforms in quantum information science with photons and atoms. We study the vacuum-induced degradation of high-finesse optical cavities with mirror coatings composed of SiO₂-Ta₂O₅ dielectric stacks, and present methods to protect these coatings and to recover their initial low loss levels. For separate coatings with reflectivities centered at 370 nm and 422 nm, a vacuum-induced continuous increase in optical loss occurs if the surface-layer coating is made of Ta₂O₅, while it does not occur if it is made of SiO₂. The incurred optical loss can be reversed by filling the vacuum chamber with oxygen at atmospheric pressure, and the recovery rate can be strongly accelerated by continuous laser illumination at 422 nm. Both the degradation and the recovery processes depend strongly on temperature. We find that a 1 nm-thick layer of SiO₂ passivating the Ta₂O₅ surface layer is sufficient to reduce the degradation rate by more than a factor of 10, strongly supporting surface oxygen depletion as the primary degradation mechanism.