Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:2504.04959 · Applied Physics Letters

All optical broadband tunable quantum frequency shifter

Li Chen, Jia-Ning Guo, Di-Yuan Zheng, M. Gao, Zhao-Qi-Zhi Han, Wu‐Zhen Li, Yue-Wei Song, Ren-Hui Chen, Chun Hua Zhou, Wan-Su Bao, Zhiyuan Zhou, Bao‐Sen Shi

Published Jul 20, 2026• 1 citation
arXivHTMLPDF

Abstract

A frequency shifter of the photon is a key component for frequency-multiplexed high-capacity quantum communications and frequency-encoded quantum computation. Existed methods for shifting the frequency of a photon based on electro-optical or acousto-optical effect, however, suffer the limited frequency shift up to a few hundreds of GHz; furthermore, high-quality micro-wave electronics are required. The frequency of a photon can also be shifted with the frequency difference equal to the frequency of pump laser by using an all optical-wave-mixing approach, which is usually about tens of THz. So, there is a big frequency shifting gap between these methods. Here, we propose a new scheme of a quantum frequency shifter based on an all-optical-wave-mixing process, which can theoretically achieve a frequency shift ranging from GHz to a few THz, therefore bridging the gap. As a principle of poof, by using two pump beams in a three-wave mixing cascading process, a heralded single photon is frequency-shifted more than ±400 GHz, and the shift can be tuned continuously over broadband by changing the frequency difference between two pump lasers. In addition, high coincidence to accidence ratio between the shifted photons and the heralded photon indicates the preserve of quantum properties. The present quantum frequency shifter is in analog to an electro-optical based shifter, but with much broader tuning ability. Our all-optical quantum frequency shifter will become a fundamental building block for high-speed quantum communication networks and frequency-domain photonic quantum computation.

DOI
10.1063/5.0342689

Related papers

Electro-optic bandwidth manipulation of quantum light (Conference Presentation)

Michał Karpiński, Michał Jachura, Laura J. Wright +1 more

Spectral-temporal manipulation of optical pulses has enabled numerous developments within a broad range of research topics, ranging from fundamental science to practical applications. Within quantum optics spectral-temporal degree of freedom of light offers a promising platform for integrated photonic quantum information processing. An important challenge in experimentally realizing spectral-temporal manipulation of quantum states of light is the need for highly efficient manipulation tools. In this context the intrinsically deterministic electro-optic methods show great promise for quantum applications. We experimentally demonstrate application of electro-optic platform for spectral-temporal manipulation of ultrashort pulsed quantum light. Using techniques analogous to serrodyne frequency shifting we show active spectral translation of few-picosecond single photon pulses by up to 0.5 THz. By employing an approach based on an electro-optic time lens we demonstrate up to 6-fold spectral compression of heralded single photon pulses with efficiency that enables us to significantly increase single photon flux through a narrow bandpass filter. We realize the required temporal phase manipulation by driving a lithium niobate waveguided electrooptic modulator with 33 dBm sinusoidal RF field at the frequency of either 10 GHz or 40 GHz. We use a phase lock loop to temporally lock the RF field to the 80 MHz repetition rate of approximately 1 ps long optical pulses. Heralded single photon wavepackets are generated by means of spontaneous parametric down-conversion in potassium dihydrogen phosphate (KDP) crystal, which enables preparation of spectrally pure single photon wavepackets without the need for spectral filtering. Spectral shifting is achieved by locking single-photon pulses to the linear slope of sinusoidal 40 GHz RF phase modulation. We verify the spectral shift by performing spectrally resolved heralded single photon counting, using frequency-to-time conversion by means of a highly dispersive chirped fiber Bragg grating. We verify the non-classicality of spectrally shifted single photons by measuring high-visibility Hong-Ou-Mandel interference using a reference single photon pulse. Spectral compression is based on the time lens principle, which requires locking optical pulses to approximately quadratic region of sinusoidal phase modulation. We utilize both 10 GHz and 40 GHz RF driving frequencies. Bandwidth compression is achieved by chirping the single photon pulse using an appropriate length of single-mode fibre and subsequently subjecting it to the action of the time lens. We verify spectral compression directly using the aforementioned spectrally-resolved heralded single photon counting method. We achieve 3-fold spectral compression of 2 nm bandwidth single photon pulses using 40 GHZ modulation frequency, and 6-fold spectral compression of 0.9 nm bandwidth single photon pulses using 10 GHz modulation frequency. Overall transmission of our set-up exceeding 30% enables practical usability of our spectral compression method which we demonstrate experimentally by showing an increased photon flux through a narrowband filter. Our results present an important contribution towards implementing quantum information processing in the spectral-temporal degree of freedom of a photon. In the context of quantum networks they present an enabling tool towards efficient photonic interfacing of different quantum information processing platforms.

•Aug 3, 2016•0 citations

Broadband Spectral Manipulation of Single Photons Using Cross-Phase Modulation

Kate L. Fenwick, Frédéric Bouchard, Guillaume Thekkadath +3 more

Manipulating the frequency and bandwidth of light is crucial in classical and quantum applications including communication, spectroscopy, imaging, and signal processing. Such capabilities also offer potential for interfacing disparate quantum systems in quantum networking and for quantum information processing. We experimentally demonstrate deterministic, broadband frequency control of heralded telecom-band single photons via cross-phase modulation in a short length of single-mode fiber. An intense, ultrafast pump pulse imposes a transient, intensity-dependent refractive-index gradient which imparts a tunable phase shift on the single photons. We present absolute frequency shifts of up to +6.42±0.06 THz and -5.82±0.02 THz, and bandwidth manipulation ranging from a factor of 0.76±0.03 to 7.1±0.4 times that of the input. Spectral measurements are acquired with a time-of-flight spectrometer and superconducting nanowire detectors. Our scheme offers a compact and scalable route to spectral routing and bandwidth engineering for ultrafast quantum networking and quantum information processing.

arXiv:2508.15886•Physical Review Letters•Jan 7, 2026•3 citations

Single-photon frequency shifting with a quadrature phase-shift keying modulator

Changchen Chen, Jane E. Heyes, Jeffrey H. Shapiro +1 more

Deterministic frequency manipulation of single photons is an essential tool for quantum communications and quantum networks. We demonstrate a 15.65 GHz frequency shift for classical and nonclassical light using a commercially available quadrature phase-shift keying modulator. The measured spectrum of frequency-shifted single photons indicates a high carrier-to-sideband ratio of 30 dB. We illustrate our frequency shifter's utility in quantum photonics by performing Hong-Ou-Mandel quantum interference between two photons whose initial frequency spectra overlap only partially, and showing visibility improvement from 62.7 to 89.1% after one of the photons undergoes a corrective frequency shift.

Scientific Reports•Jan 11, 2021•14 citations

Efficient quantum frequency translation of broadband single photons by Bragg-scattering four-wave mixing

Ramy Tannous, Philip J. Bustard, Duncan G. England +3 more

We experimentally demonstrate frequency translation of a non-classical optical field by Bragg-scattering four-wave mixing, driven by orthogonally polarized pump pulses in a birefringent optical fiber. Heralded single photons are up- and down-translated by 6.8 THz between bands at 688.1 nm and 678.2 nm, each with efficiency > 97%. The input and output spectral shape and bandwidth show negligible modulation. Second-order auto-correlation measurements of the 678.2 nm and 688.1 nm fields at maximum conversion yield values of 0.0302 ± 0.0005 and 0.028 ± 0.001, respectively, compared with the input second-order correlation of 0.026 ± 0.001; this indicates that the frequency translation process preserves the non-classical nature of the field. The high efficiency, broad bandwidth, and low noise render this scheme useful for quantum networks and sources.

Optica Quantum•Mar 12, 2025•3 citations

Wideband and low-spurious optical waveform generator for optically addressable quantum systems manipulation and control

Sacha Welinski, Eduardo Beattie, Lothaire Ulrich +4 more

Optical manipulation of quantum systems requires stable laser sources able to produce complex waveforms over a large frequency range. In the visible region, such waveforms can be generated using an acousto-optic modulator driven by an arbitrary waveform generator, but these suffer from a limited tuning range typically of a few tens of MHz. Visible-range electro-optic modulators are an alternative option offering a larger modulation bandwidth, however they have limited output power which drastically restricts the scalability of quantum applications. There is currently no architecture able to perform phase-stabilized waveforms over several GHz in the visible or near infrared region while providing sufficient optical power for quantum applications. Here we propose and develop a modulation and frequency conversion set-up able to deliver optical waveforms over a large frequency range, with a high spurious extinction ratio, scalable to the entire visible/near infrared region with high optical power. The optical waveforms are first generated at telecom wavelength and then converted to the emitter wavelength through a sum frequency generation process. By adapting the pump laser frequency, the optical waveforms can be tuned to interact with a broad range of optical quantum emitters or qubits such as alkali atoms, trapped ions, rare earth ions, or fluorescent defects in solid-state matrices. Using this architecture, we were able to detect and study a single erbium ion in a nanoparticle. We also generated high bandwidth signals at 606 nm, which would enable frequency multiplexing of on-demand read-out Pr3+:Y2SiO5 quantum memories.

Optics Express•May 13, 2024•1 citation

1 × N DWDM channel selective quantum frequency conversion

Tomoaki Arizono, Toshiki Kobayashi, Shigehito Miki +5 more

Dense wavelength division multiplexing (DWDM) is a key technology for realizing high-capacity and flexible quantum communication networks. To enable the emerging quantum internet, quantum frequency conversion is also essential for bridging different quantum systems over optical fiber networks. In this work, aiming at a frequency-multiplexed quantum internet, we present a channel-selective quantum frequency conversion (CS-QFC) based on difference frequency generation in a PPLN waveguide, which has been widely used in conventional QFC experiments. The CS-QFC converts a frequency of a photon at a single frequency to any frequency in the DWDM channels by dynamically selecting one of the pump lights. In the experiment, we demonstrated the CS-QFC from 780 nm to around 1540 nm employing one of the pump lights around 1580 nm detuned with a spacing of 25 GHz. From the experiment using the laser light, we showed that the output-frequency tunability of our CS-QFC reaches 2.5 THz, which corresponds to the ability to establish a 100-ch DWDM dynamic link from a single quantum system. Using photon pairs, we performed an experiment in which photons were routed into seven of the DWDM channels. As a result, photons were converted to the channels corresponding to the pump frequencies, while keeping the nonclassical cross-correlation functions, and no crosstalk to the other channels was observed.

arXiv:2409.08025•Optics Express•Dec 19, 2025•3 citations
A frequency shifter of the photon is a key component for frequency-multiplexed high-capacity quantum communications and frequency-encoded quantum computation. Existed methods for shifting the frequency of a photon based on electro-optical or acousto-optical effect, however, suffer the limited frequency shift up to a few hundreds of GHz; furthermore, high-quality micro-wave electronics are required. The frequency of a photon can also be shifted with the frequency difference equal to the frequency of pump laser by using an all optical-wave-mixing approach, which is usually about tens of THz. So, there is a big frequency shifting gap between these methods. Here, we propose a new scheme of a quantum frequency shifter based on an all-optical-wave-mixing process, which can theoretically achieve a frequency shift ranging from GHz to a few THz, therefore bridging the gap. As a principle of poof, by using two pump beams in a three-wave mixing cascading process, a heralded single photon is frequency-shifted more than ±400 GHz, and the shift can be tuned continuously over broadband by changing the frequency difference between two pump lasers. In addition, high coincidence to accidence ratio between the shifted photons and the heralded photon indicates the preserve of quantum properties. The present quantum frequency shifter is in analog to an electro-optical based shifter, but with much broader tuning ability. Our all-optical quantum frequency shifter will become a fundamental building block for high-speed quantum communication networks and frequency-domain photonic quantum computation.
Spectral-temporal manipulation of optical pulses has enabled numerous developments within a broad range of research topics, ranging from fundamental science to practical applications. Within quantum optics spectral-temporal degree of freedom of light offers a promising platform for integrated photonic quantum information processing. An important challenge in experimentally realizing spectral-temporal manipulation of quantum states of light is the need for highly efficient manipulation tools. In this context the intrinsically deterministic electro-optic methods show great promise for quantum applications. We experimentally demonstrate application of electro-optic platform for spectral-temporal manipulation of ultrashort pulsed quantum light. Using techniques analogous to serrodyne frequency shifting we show active spectral translation of few-picosecond single photon pulses by up to 0.5 THz. By employing an approach based on an electro-optic time lens we demonstrate up to 6-fold spectral compression of heralded single photon pulses with efficiency that enables us to significantly increase single photon flux through a narrow bandpass filter. We realize the required temporal phase manipulation by driving a lithium niobate waveguided electrooptic modulator with 33 dBm sinusoidal RF field at the frequency of either 10 GHz or 40 GHz. We use a phase lock loop to temporally lock the RF field to the 80 MHz repetition rate of approximately 1 ps long optical pulses. Heralded single photon wavepackets are generated by means of spontaneous parametric down-conversion in potassium dihydrogen phosphate (KDP) crystal, which enables preparation of spectrally pure single photon wavepackets without the need for spectral filtering. Spectral shifting is achieved by locking single-photon pulses to the linear slope of sinusoidal 40 GHz RF phase modulation. We verify the spectral shift by performing spectrally resolved heralded single photon counting, using frequency-to-time conversion by means of a highly dispersive chirped fiber Bragg grating. We verify the non-classicality of spectrally shifted single photons by measuring high-visibility Hong-Ou-Mandel interference using a reference single photon pulse. Spectral compression is based on the time lens principle, which requires locking optical pulses to approximately quadratic region of sinusoidal phase modulation. We utilize both 10 GHz and 40 GHz RF driving frequencies. Bandwidth compression is achieved by chirping the single photon pulse using an appropriate length of single-mode fibre and subsequently subjecting it to the action of the time lens. We verify spectral compression directly using the aforementioned spectrally-resolved heralded single photon counting method. We achieve 3-fold spectral compression of 2 nm bandwidth single photon pulses using 40 GHZ modulation frequency, and 6-fold spectral compression of 0.9 nm bandwidth single photon pulses using 10 GHz modulation frequency. Overall transmission of our set-up exceeding 30% enables practical usability of our spectral compression method which we demonstrate experimentally by showing an increased photon flux through a narrowband filter. Our results present an important contribution towards implementing quantum information processing in the spectral-temporal degree of freedom of a photon. In the context of quantum networks they present an enabling tool towards efficient photonic interfacing of different quantum information processing platforms.
Manipulating the frequency and bandwidth of light is crucial in classical and quantum applications including communication, spectroscopy, imaging, and signal processing. Such capabilities also offer potential for interfacing disparate quantum systems in quantum networking and for quantum information processing. We experimentally demonstrate deterministic, broadband frequency control of heralded telecom-band single photons via cross-phase modulation in a short length of single-mode fiber. An intense, ultrafast pump pulse imposes a transient, intensity-dependent refractive-index gradient which imparts a tunable phase shift on the single photons. We present absolute frequency shifts of up to +6.42±0.06 THz and -5.82±0.02 THz, and bandwidth manipulation ranging from a factor of 0.76±0.03 to 7.1±0.4 times that of the input. Spectral measurements are acquired with a time-of-flight spectrometer and superconducting nanowire detectors. Our scheme offers a compact and scalable route to spectral routing and bandwidth engineering for ultrafast quantum networking and quantum information processing.
Deterministic frequency manipulation of single photons is an essential tool for quantum communications and quantum networks. We demonstrate a 15.65 GHz frequency shift for classical and nonclassical light using a commercially available quadrature phase-shift keying modulator. The measured spectrum of frequency-shifted single photons indicates a high carrier-to-sideband ratio of 30 dB. We illustrate our frequency shifter's utility in quantum photonics by performing Hong-Ou-Mandel quantum interference between two photons whose initial frequency spectra overlap only partially, and showing visibility improvement from 62.7 to 89.1% after one of the photons undergoes a corrective frequency shift.
We experimentally demonstrate frequency translation of a non-classical optical field by Bragg-scattering four-wave mixing, driven by orthogonally polarized pump pulses in a birefringent optical fiber. Heralded single photons are up- and down-translated by 6.8 THz between bands at 688.1 nm and 678.2 nm, each with efficiency > 97%. The input and output spectral shape and bandwidth show negligible modulation. Second-order auto-correlation measurements of the 678.2 nm and 688.1 nm fields at maximum conversion yield values of 0.0302 ± 0.0005 and 0.028 ± 0.001, respectively, compared with the input second-order correlation of 0.026 ± 0.001; this indicates that the frequency translation process preserves the non-classical nature of the field. The high efficiency, broad bandwidth, and low noise render this scheme useful for quantum networks and sources.
Optical manipulation of quantum systems requires stable laser sources able to produce complex waveforms over a large frequency range. In the visible region, such waveforms can be generated using an acousto-optic modulator driven by an arbitrary waveform generator, but these suffer from a limited tuning range typically of a few tens of MHz. Visible-range electro-optic modulators are an alternative option offering a larger modulation bandwidth, however they have limited output power which drastically restricts the scalability of quantum applications. There is currently no architecture able to perform phase-stabilized waveforms over several GHz in the visible or near infrared region while providing sufficient optical power for quantum applications. Here we propose and develop a modulation and frequency conversion set-up able to deliver optical waveforms over a large frequency range, with a high spurious extinction ratio, scalable to the entire visible/near infrared region with high optical power. The optical waveforms are first generated at telecom wavelength and then converted to the emitter wavelength through a sum frequency generation process. By adapting the pump laser frequency, the optical waveforms can be tuned to interact with a broad range of optical quantum emitters or qubits such as alkali atoms, trapped ions, rare earth ions, or fluorescent defects in solid-state matrices. Using this architecture, we were able to detect and study a single erbium ion in a nanoparticle. We also generated high bandwidth signals at 606 nm, which would enable frequency multiplexing of on-demand read-out Pr3+:Y2SiO5 quantum memories.
Dense wavelength division multiplexing (DWDM) is a key technology for realizing high-capacity and flexible quantum communication networks. To enable the emerging quantum internet, quantum frequency conversion is also essential for bridging different quantum systems over optical fiber networks. In this work, aiming at a frequency-multiplexed quantum internet, we present a channel-selective quantum frequency conversion (CS-QFC) based on difference frequency generation in a PPLN waveguide, which has been widely used in conventional QFC experiments. The CS-QFC converts a frequency of a photon at a single frequency to any frequency in the DWDM channels by dynamically selecting one of the pump lights. In the experiment, we demonstrated the CS-QFC from 780 nm to around 1540 nm employing one of the pump lights around 1580 nm detuned with a spacing of 25 GHz. From the experiment using the laser light, we showed that the output-frequency tunability of our CS-QFC reaches 2.5 THz, which corresponds to the ability to establish a 100-ch DWDM dynamic link from a single quantum system. Using photon pairs, we performed an experiment in which photons were routed into seven of the DWDM channels. As a result, photons were converted to the channels corresponding to the pump frequencies, while keeping the nonclassical cross-correlation functions, and no crosstalk to the other channels was observed.