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Scientific Reports

Single-photon frequency shifting with a quadrature phase-shift keying modulator

Changchen Chen, Jane E. Heyes, Jeffrey H. Shapiro, Franco N. C. Wong

Published Jan 11, 2021• 14 citations
Publisher

Abstract

Deterministic frequency manipulation of single photons is an essential tool for quantum communications and quantum networks. We demonstrate a 15.65 GHz frequency shift for classical and nonclassical light using a commercially available quadrature phase-shift keying modulator. The measured spectrum of frequency-shifted single photons indicates a high carrier-to-sideband ratio of 30 dB. We illustrate our frequency shifter's utility in quantum photonics by performing Hong-Ou-Mandel quantum interference between two photons whose initial frequency spectra overlap only partially, and showing visibility improvement from 62.7 to 89.1% after one of the photons undergoes a corrective frequency shift.

DOI
10.1038/s41598-020-79511-8

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SPIE Conference on Quantum and Nonlinear Optics•Nov 14, 2018•0 citations
Deterministic frequency manipulation of single photons is an essential tool for quantum communications and quantum networks. We demonstrate a 15.65 GHz frequency shift for classical and nonclassical light using a commercially available quadrature phase-shift keying modulator. The measured spectrum of frequency-shifted single photons indicates a high carrier-to-sideband ratio of 30 dB. We illustrate our frequency shifter's utility in quantum photonics by performing Hong-Ou-Mandel quantum interference between two photons whose initial frequency spectra overlap only partially, and showing visibility improvement from 62.7 to 89.1% after one of the photons undergoes a corrective frequency shift.
Frequency translation of single photons while preserving their quantum characteristics is an important technology for flexible networking of photonic quantum communication systems. Here we demonstrate a flexible scheme to interface different-color photons using an optical single sideband (OSSB) modulator. By changing the radio-frequency signal that drives the modulators, we can easily shift and precisely tune the frequency of single photons. Using the OSSB modulator, we successfully erased the frequency distinguishability of non-degenerated photon pairs to obtain the Hong-Ou-Mandel interference with a visibility exceeding 90%. We also demonstrated that the level of distinguishability can be precisely controlled by the OSSB modulator. We expect that the OSSB modulator will provide a simple and flexible photonic interface for realizing advanced quantum information systems.
We introduce our recent photonic quantum information processing experiments using the high-speed electro-optic modulator (EOM) based on a lithium niobate waveguides. First, we demonstrated the frequency shifter for single photons by using an optical single sideband (OSSB) modulator, which is based on the nested configuration of four phase modulators (PMs). By properly setting the RF modulation signal and the bias voltage to each PM, we can suppress unwanted sidebands to realize a frequency shifter that can tune the frequency of single photons with accuracy of an RF synthesizer. Using the OSSB modulator, we eliminated the frequency distinguishability between two single photons whose frequencies were different by 25 GHz, and as a result observed a Hong-Ou- Mandel interference with a visibility exceeding 90%. We also proposed and demonstrated a two-qubit controlled logic gate for time-bin qubits using a two-input, two-output optical switch. The switch enables us to individually perform different functions for two temporal bases as a time-dependent beam splitter, so that we can realize controlled-phase (C-Phase) gate for a time-bin qubit. We showed that the states of two separable single photons were entangled as a result of the C-Phase gate operation. We performed the quantum state tomography to obtain density matrices of the output states from the C-Phase gate for some specific input states, and confirmed that the averaged state fidelity to the pure states was 85%. These results indicate that the EOMs will be a useful tool for realizing advanced photonic quantum communication systems.
Spectral-temporal manipulation of optical pulses has enabled numerous developments within a broad range of research topics, ranging from fundamental science to practical applications. Within quantum optics spectral-temporal degree of freedom of light offers a promising platform for integrated photonic quantum information processing. An important challenge in experimentally realizing spectral-temporal manipulation of quantum states of light is the need for highly efficient manipulation tools. In this context the intrinsically deterministic electro-optic methods show great promise for quantum applications. We experimentally demonstrate application of electro-optic platform for spectral-temporal manipulation of ultrashort pulsed quantum light. Using techniques analogous to serrodyne frequency shifting we show active spectral translation of few-picosecond single photon pulses by up to 0.5 THz. By employing an approach based on an electro-optic time lens we demonstrate up to 6-fold spectral compression of heralded single photon pulses with efficiency that enables us to significantly increase single photon flux through a narrow bandpass filter. We realize the required temporal phase manipulation by driving a lithium niobate waveguided electrooptic modulator with 33 dBm sinusoidal RF field at the frequency of either 10 GHz or 40 GHz. We use a phase lock loop to temporally lock the RF field to the 80 MHz repetition rate of approximately 1 ps long optical pulses. Heralded single photon wavepackets are generated by means of spontaneous parametric down-conversion in potassium dihydrogen phosphate (KDP) crystal, which enables preparation of spectrally pure single photon wavepackets without the need for spectral filtering. Spectral shifting is achieved by locking single-photon pulses to the linear slope of sinusoidal 40 GHz RF phase modulation. We verify the spectral shift by performing spectrally resolved heralded single photon counting, using frequency-to-time conversion by means of a highly dispersive chirped fiber Bragg grating. We verify the non-classicality of spectrally shifted single photons by measuring high-visibility Hong-Ou-Mandel interference using a reference single photon pulse. Spectral compression is based on the time lens principle, which requires locking optical pulses to approximately quadratic region of sinusoidal phase modulation. We utilize both 10 GHz and 40 GHz RF driving frequencies. Bandwidth compression is achieved by chirping the single photon pulse using an appropriate length of single-mode fibre and subsequently subjecting it to the action of the time lens. We verify spectral compression directly using the aforementioned spectrally-resolved heralded single photon counting method. We achieve 3-fold spectral compression of 2 nm bandwidth single photon pulses using 40 GHZ modulation frequency, and 6-fold spectral compression of 0.9 nm bandwidth single photon pulses using 10 GHz modulation frequency. Overall transmission of our set-up exceeding 30% enables practical usability of our spectral compression method which we demonstrate experimentally by showing an increased photon flux through a narrowband filter. Our results present an important contribution towards implementing quantum information processing in the spectral-temporal degree of freedom of a photon. In the context of quantum networks they present an enabling tool towards efficient photonic interfacing of different quantum information processing platforms.
A frequency shifter of the photon is a key component for frequency-multiplexed high-capacity quantum communications and frequency-encoded quantum computation. Existed methods for shifting the frequency of a photon based on electro-optical or acousto-optical effect, however, suffer the limited frequency shift up to a few hundreds of GHz; furthermore, high-quality micro-wave electronics are required. The frequency of a photon can also be shifted with the frequency difference equal to the frequency of pump laser by using an all optical-wave-mixing approach, which is usually about tens of THz. So, there is a big frequency shifting gap between these methods. Here, we propose a new scheme of a quantum frequency shifter based on an all-optical-wave-mixing process, which can theoretically achieve a frequency shift ranging from GHz to a few THz, therefore bridging the gap. As a principle of poof, by using two pump beams in a three-wave mixing cascading process, a heralded single photon is frequency-shifted more than ±400 GHz, and the shift can be tuned continuously over broadband by changing the frequency difference between two pump lasers. In addition, high coincidence to accidence ratio between the shifted photons and the heralded photon indicates the preserve of quantum properties. The present quantum frequency shifter is in analog to an electro-optical based shifter, but with much broader tuning ability. Our all-optical quantum frequency shifter will become a fundamental building block for high-speed quantum communication networks and frequency-domain photonic quantum computation.
Single-photon frequency conversion for quantum interface plays an important role in quantum communications and networks, which is crucial for the realization of quantum memory, faithful entanglement swapping and quantum teleportation. In this talk, I will present our recent experiments about single-photon frequency conversion based on quadratic nonlinear processes. Firstly, we demonstrated spectrum compression of broadband single photons at the telecom wavelength to the near-visible window. A positively chirped single-photon-level laser pulse and a negatively chirped classical one are converted to a narrowband single-photon pulse, with a spectrum compression factor of 58, through sum-frequency generation (SFG), marking a critical step towards coherent photonic interface. Secondly, we demonstrated the nonlinear interaction between two chirped broadband single-photon-level coherent states. A high SFG efficiency of 1.06 × 10−7 is realized, which may be utilized to achieve heralding entanglement at a distance. Finally, we theoretically introduced and experimentally demonstrated single-photon frequency conversion in the telecom band, enabling switching of single photons between dense wavelength-division multiplexing channels. Using cascaded quasi-phase matched sum/difference frequency generation, the signal photon of a photon pair from spontaneous down-conversion is precisely shifted to identically match its counterpart, i.e. idler photon, in frequency to manifest a clear non-classical dip in the Hong-Ou-Mandel interference. Moreover, quantum entanglement between the photon pair is maintained after the frequency conversion. Our researches have realized three significant quantum interfaces via single-photon frequency conversion, which hold great promise for the development of quantum communications and networks.