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arXiv:2503.18153 · Journal of Optics

Mie resonances in optical trapping: their role in kinematics and back-action

Sharareh Sayyad, Gerd Leuchs, Vsevolod Salakhutdinov

Published May 20, 2026• 0 citations
arXivHTMLPDF

Abstract

Abstract The heating rate plays a crucial role in the decoherence of the harmonic motion of an optically levitated nanoparticle. The values of this rate vary depending on both the scattering photon rate and the kinetic energy acquired through individual photon recoils. While the combined roles of these factors have been extensively studied, the energy transfer per recoil has not been explicitly examined. This energy transfer is often approximated using a linear dipole model with coefficients {1/5, 2/5, 7/5} which applies in the Rayleigh limit. In this work, we analyze the evolution of energy transfer per photon recoil for low-absorption dielectric nanospheres with diameters ranging from 2 nm to 500 nm. Using a far-field approximation, we demonstrate that the Kerker condition, which enhances the alignment between incident and scattered wavevectors, may significantly reduce the energy transferred per recoil. Although this reduction is counterbalanced by the increasing scattering rate, for an individual scattering event, the reduction of recoil suggests an intrinsic suppression of back-action. Our results reveal a potential enhancement in the accuracy of estimations in tabletop experiments involving Mie particles of the considered sizes and provide guidance for the selection of optimal probe sizes and materials. Our interpretation of recoil reduction as a manifestation of back-action suppression indicates a potential pathway toward minimizing measurement-induced disturbances through engineered control of scattering directivity, potentially enabled by metamaterial-based designs.

DOI
10.1088/2040-8986/ae709c

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•Jul 15, 2021•247 citations
Abstract The heating rate plays a crucial role in the decoherence of the harmonic motion of an optically levitated nanoparticle. The values of this rate vary depending on both the scattering photon rate and the kinetic energy acquired through individual photon recoils. While the combined roles of these factors have been extensively studied, the energy transfer per recoil has not been explicitly examined. This energy transfer is often approximated using a linear dipole model with coefficients {1/5, 2/5, 7/5} which applies in the Rayleigh limit. In this work, we analyze the evolution of energy transfer per photon recoil for low-absorption dielectric nanospheres with diameters ranging from 2 nm to 500 nm. Using a far-field approximation, we demonstrate that the Kerker condition, which enhances the alignment between incident and scattered wavevectors, may significantly reduce the energy transferred per recoil. Although this reduction is counterbalanced by the increasing scattering rate, for an individual scattering event, the reduction of recoil suggests an intrinsic suppression of back-action. Our results reveal a potential enhancement in the accuracy of estimations in tabletop experiments involving Mie particles of the considered sizes and provide guidance for the selection of optimal probe sizes and materials. Our interpretation of recoil reduction as a manifestation of back-action suppression indicates a potential pathway toward minimizing measurement-induced disturbances through engineered control of scattering directivity, potentially enabled by metamaterial-based designs.
Recoil heating from photon scattering is a fundamental source of decoherence in optical trapping, severely limiting the preparation of nonclassical motional states. In cavity setups in the coherent scattering configuration, a predictive theory of recoil heating rate is missing, as usual perturbative approaches fail in the presence of sharp optical resonances. Hence, current works assume that the recoil heating rate is approximately equal to its free-space value. Here we show that this is not the case, as the electromagnetic environment can strongly modify recoil heating rate by the Purcell effect. Specifically, we predict that this rate can be significantly suppressed in state-of-the-art microcavities, for both center-of-mass and librational motion. To establish these results, we develop a general theoretical framework based on macroscopic quantum electrodynamics and on the few-mode quantization approach developed in nanophotonics. Our method applies to particles trapped in the presence of arbitrary electromagnetic structures, thus providing a route to engineering motional decoherence in levitated optomechanics by photonic structure design.
We theoretically show that laser recoil heating in free-space levitated optomechanics can be arbitrarily suppressed by shining squeezed light onto an optically trapped nanoparticle. The presence of squeezing modifies the quantum electrodynamical light-matter interaction in a way that enables us to control the amount of information that the scattered light carries about a given mechanical degree of freedom. Moreover, we analyze the trade-off between measurement imprecision and back-action noise and show that optical detection beyond the standard quantum limit can be achieved. We predict that, with state-of-the-art squeezed light sources, laser recoil heating can be reduced by at least 60% by squeezing a single Gaussian mode with an appropriate incidence direction, and by 98% by squeezing a properly mode-matched mode. Our results, which are valid both for motional and librational degrees of freedom, will lead to improved feedback cooling schemes as well as boost the coherence time of optically levitated nanoparticles in the quantum regime.
Abstract Tests of quantum mechanics on a macroscopic scale require extreme control over mechanical motion and its decoherence [1-4]. Quantum control of mechanical motion has been achieved by engineering the radiation pressure coupling between a micromechanical oscillator and the electromagnetic field in a resonator [5-8]. Furthermore, measurement-based feedback control relying on cavity-enhanced detection schemes has been used to cool micromechanical oscillators to their quantum ground states [9]. In contrast to mechanically tethered systems, optically levitated nanoparticles are particularly promising candidates for matter-wave experiments with massive objects [10,11], since their trapping potential is fully controllable. In this work, we optically levitate a femto-gram dielectric particle in cryogenic free space, which suppresses thermal effects sufficiently to make the measurement backaction the dominant decoherence mechanism. With an efficient quantum measurement, we exert quantum control over the dynamics of the particle. We cool its center-of-mass motion by measurement-based feedback to an average occupancy of 0.65 motional quanta, corresponding to a state purity of 43%. The absence of an optical resonator and its bandwidth limitations holds promise to transfer the full quantum control available for electromagnetic fields to a mechanical system. Together with the fact that the optical trapping potential is highly controllable, our experimental platform offers a route to investigating quantum mechanics at macroscopic scales [12,13].
Mitigating recoil events and minimizing optically induced heating are central challenges in the precise control and cooling of macroscopic particles. To overcome this, we propose trapping resonant dielectric particles for applications in ultra-high vacuum (UHV) levitodynamics. Contrary to other approaches, where suppressing the parasitic resonant scattering was achieved in a standing wave geometry, here we propose a single beam geometry in a dark trap regime. As a promising material platform, we focus on a class of transition-metal dichalcogenide (TMD) particles with high polarizability, characterized by refractive indices in the range 3.73.73.7-4.84.84.8 and densities up to 9.3 g cm−39.3~\mathrm{g\,cm^{-3}}9.3 gcm−3. Using full Mie theory, we identify a range of TMD particle radii that support stable axial and radial magnetic quadrupole trapping in a bottle-beam configuration. We predict that for WS2_22​ particles with a mass of 0.5×1012 amu0.5 \times 10^{12}\,\mathrm{amu}0.5×1012amu, one can expect suppression of the scattering rate relative to the mechanical frequency down to Γ/Ω≃0.02Γ/Ω\simeq 0.02Γ/Ω≃0.02. This corresponds to a coherence time extended by approximately three orders of magnitude compared with silica particles of the same mass trapped in conventional bright optical traps at UHV. Combined with significantly reduced internal heating, remaining well below the melting point of the material, dark trapping of resonant TMD macroscopic particles emerges as a promising platform for exploring quantum physics with large masses.
Radiative and nonradiative resonant couplings between defects are ubiquitous phenomena in photonic devices used in classical and quantum information technology applications. In this work, we present a first-principles approach to enable quantitative predictions of the energy transfer between defects in photonic cavities, beyond the dipole-dipole approximation and including the many-body nature of the electronic states. As an example, we discuss the energy transfer from a dipolelike emitter to an F center in MgO in a spherical cavity. We show that the cavity can be used to controllably enhance or suppress specific spin-flip and spin-conserving transitions. Specifically, we predict that an ∼10–100 enhancement in the resonant energy transfer rate can be gained in the case of the F center in MgO at ∼10 nm distances from a dipolar source, using rather moderate cavity with quality factor Q ∼ 400. We also show that a similar suppression in the transfer rate can be achieved by off-tuning the cavity resonance relative to the emitter transition energy. The framework presented here is general and readily applicable to a wide range of devices where localized emitters are embedded in microspheres, core-shell nanoparticles, and dielectric Mie resonators. Hence, our approach paves the way to predict how to control energy transfer in quantum memories and in ultrahigh-density optical memories, and in a variety of quantum information platforms.
Abstract Tests of quantum mechanics on a macroscopic scale require extreme control over mechanical motion and its decoherence1–3. Quantum control of mechanical motion has been achieved by engineering the radiation–pressure coupling between a micromechanical oscillator and the electromagnetic field in a resonator4–7. Furthermore, measurement-based feedback control relying on cavity-enhanced detection schemes has been used to cool micromechanical oscillators to their quantum ground states8. In contrast to mechanically tethered systems, optically levitated nanoparticles are particularly promising candidates for matter-wave experiments with massive objects9, 10, since their trapping potential is fully controllable. Here we optically levitate a femtogram (10−15 grams) dielectric particle in cryogenic free space, which suppresses thermal effects sufficiently to make the measurement backaction the dominant decoherence mechanism. With an efficient quantum measurement, we exert quantum control over the dynamics of the particle. We cool its centre-of-mass motion by measurement-based feedback to an average occupancy of 0.65 motional quanta, corresponding to a state purity of 0.43. The absence of an optical resonator and its bandwidth limitations holds promise to transfer the full quantum control available for electromagnetic fields to a mechanical system. Together with the fact that the optical trapping potential is highly controllable, our experimental platform offers a route to investigating quantum mechanics at macroscopic scales11.