Abstract Tests of quantum mechanics on a macroscopic scale require extreme control over mechanical motion and its decoherence1–3. Quantum control of mechanical motion has been achieved by engineering the radiation–pressure coupling between a micromechanical oscillator and the electromagnetic field in a resonator4–7. Furthermore, measurement-based feedback control relying on cavity-enhanced detection schemes has been used to cool micromechanical oscillators to their quantum ground states8. In contrast to mechanically tethered systems, optically levitated nanoparticles are particularly promising candidates for matter-wave experiments with massive objects9, 10, since their trapping potential is fully controllable. Here we optically levitate a femtogram (10−15 grams) dielectric particle in cryogenic free space, which suppresses thermal effects sufficiently to make the measurement backaction the dominant decoherence mechanism. With an efficient quantum measurement, we exert quantum control over the dynamics of the particle. We cool its centre-of-mass motion by measurement-based feedback to an average occupancy of 0.65 motional quanta, corresponding to a state purity of 0.43. The absence of an optical resonator and its bandwidth limitations holds promise to transfer the full quantum control available for electromagnetic fields to a mechanical system. Together with the fact that the optical trapping potential is highly controllable, our experimental platform offers a route to investigating quantum mechanics at macroscopic scales11.
Abstract Tests of quantum mechanics on a macroscopic scale require extreme control over mechanical motion and its decoherence1–3. Quantum control of mechanical motion has been achieved by engineering the radiation–pressure coupling between a micromechanical oscillator and the electromagnetic field in a resonator4–7. Furthermore, measurement-based feedback control relying on cavity-enhanced detection schemes has been used to cool micromechanical oscillators to their quantum ground states8. In contrast to mechanically tethered systems, optically levitated nanoparticles are particularly promising candidates for matter-wave experiments with massive objects9, 10, since their trapping potential is fully controllable. Here we optically levitate a femtogram (10−15 grams) dielectric particle in cryogenic free space, which suppresses thermal effects sufficiently to make the measurement backaction the dominant decoherence mechanism. With an efficient quantum measurement, we exert quantum control over the dynamics of the particle. We cool its centre-of-mass motion by measurement-based feedback to an average occupancy of 0.65 motional quanta, corresponding to a state purity of 0.43. The absence of an optical resonator and its bandwidth limitations holds promise to transfer the full quantum control available for electromagnetic fields to a mechanical system. Together with the fact that the optical trapping potential is highly controllable, our experimental platform offers a route to investigating quantum mechanics at macroscopic scales11.
Abstract Tests of quantum mechanics on a macroscopic scale require extreme control over mechanical motion and its decoherence [1-4]. Quantum control of mechanical motion has been achieved by engineering the radiation pressure coupling between a micromechanical oscillator and the electromagnetic field in a resonator [5-8]. Furthermore, measurement-based feedback control relying on cavity-enhanced detection schemes has been used to cool micromechanical oscillators to their quantum ground states [9]. In contrast to mechanically tethered systems, optically levitated nanoparticles are particularly promising candidates for matter-wave experiments with massive objects [10,11], since their trapping potential is fully controllable. In this work, we optically levitate a femto-gram dielectric particle in cryogenic free space, which suppresses thermal effects sufficiently to make the measurement backaction the dominant decoherence mechanism. With an efficient quantum measurement, we exert quantum control over the dynamics of the particle. We cool its center-of-mass motion by measurement-based feedback to an average occupancy of 0.65 motional quanta, corresponding to a state purity of 43%. The absence of an optical resonator and its bandwidth limitations holds promise to transfer the full quantum control available for electromagnetic fields to a mechanical system. Together with the fact that the optical trapping potential is highly controllable, our experimental platform offers a route to investigating quantum mechanics at macroscopic scales [12,13].
Levitated nanoparticles are a forerunner as an experimental platform to test the limits of quantum mechanics at a macroscopic scale. Some important initial steps have been made towards preparing a macroscopic quantum state of a relatively massive (femtogram) particle. Specifically, the community has achieved ground-state cooling of the center-of-mass motion of a nanoparticle levitated in an optical trap. One crucial further step is now to expand the wavefunction of the particle. This step should happen in the presence of a minimum of decoherence, which makes evolution in an optical trap (inevitably exerting measurement backaction) unsuitable.
About a decade ago, optically levitated nanoparticles have been proposed for macroscopic tests of quantum mechanics.For such tests, the thermal motion of the particle's center of mass is required to be close to its ground state of energy.Ever since these proposals, research groups around the world try to achieve ground-state cooling of optically levitated glass particles.In this dissertation, we cool the center-of-mass motion of a nanoparticle in an optical trap.Based on the position measurement of the particle, we apply a damping force in proportion to the particle's speed, which leads to a cooling effect.We find that the cooling performance of our cold damping scheme is limited by the measurement imprecision.We analyze our detection principle theoretically and find an ideal detection scheme whose imprecision is at the fundamental noise level dictated by quantum mechanics.Such a Heisenberglimited detection would, in principle, allow for ground-state feedback cooling.With these insights applied to our experiment, we cool the motion of our particle to an average of four quanta.Moreover, we resolve an asymmetry between the Stokes and anti-Stokes scattered light from the particle.This quantum effect allows us to calibrate the system to the ground state energy.Our work advances the research field of levitated optomechanics toward quantum control and therefore toward macroscopic tests of quantum mechanics.i Zusammenfassung Vor rund zehn Jahren wurde vorgeschlagen, die Gesetze der Quantenmechanik an makroskopischen Objekten mittels in Laserstrahlen schwebenden Nanopartikeln zu testen.Seitdem versuchen Forschungsgruppen weltweit, die thermische Partikelbewegung von solch schwebenden Glaspartikeln bis nah an ihren Quantengrundzustand zu kühlen.In dieser Dissertation kühlen wir die Schwerpunktsbewegung eines Nanopartikels in seiner optischen Falle.Basierend auf einer Positionsmessung legen wir eine dämpfende Kraft in Proportion zur Partikelgeschwindigkeit an, was zu einer Kühlung der Bewegung führt.Wir beobachten, dass diese Kühltechnik durch unsere Messungenauigkeit limitiert ist.Wir untersuchen unsere optische Detektion theoretisch und finden ein ideales Messverfahren, dessen Ungenauigkeit durch die fundamentalen Nullpunktfluktuationen der Quantenphysik gegeben ist.Solch eine Heisenberg-limitierte Messung würde es uns prinzipiell ermöglichen, das Partikel in seinen Grundzustand zu kühlen.Mit dieser Einsicht angewandt auf unser Experiment kühlen wir die Partikelbewegung zu vier Energiequanten.Damit können wir die sogenannte Seitenbandasymmetrie zwischen Stokes und Anti-Stokes Streuung auflösen.Dieser Quanteneffekt ermöglicht es uns, das System gegen die Grundzustandsenergie zu kalibrieren.Unsere Arbeit bringt das Forschungsfeld der schwebenden Optomechanik einen Schritt näher in Richtung makroskopischer Tests der Quantentheorie.
Abstract Every massive particle behaves like a wave, according to quantum physics. Yet, this characteristic wave nature has only been observed in double-slit experiments with microscopic systems, such as atoms and molecules [1, 2]. The key aspect is that the wavefunction describing the motion of these systems extends coherently over a distance comparable to the slit separation, much larger than the size of the system itself [3]. Preparing these states of more massive and complex objects remains an outstanding challenge. While the motion of solid-state oscillators can now be controlled at the level of single quanta, their coherence length remains comparable to the zero-point motion, limited to subatomic distances [4–7]. Here, we prepare a delocalized state of a levitating solid-state nanosphere with coherence length exceeding the zero-point motion. We first cool its motion to the ground state. Then, by modulating the stiffness of the confinement potential, we achieve more than a threefold increment of the initial coherence length with minimal added noise. Optical levitation gives us the necessary control over the confinement that other mechanical platforms lack. Our work is a stepping stone towards the generation of delocalization scales comparable to the object size, a crucial regime for macroscopic quantum experiments [8], and towards quantum-enhanced force sensing with levitated particles [9].
Abstract The ability to accurately control the dynamics of physical systems by measurement and feedback is a pillar of modern engineering1. Today, the increasing demand for applied quantum technologies requires adaptation of this level of control to individual quantum systems2, 3. Achieving this in an optimal way is a challenging task that relies on both quantum-limited measurements and specifically tailored algorithms for state estimation and feedback4. Successful implementations thus far include experiments on the level of optical and atomic systems5–7. Here we demonstrate real-time optimal control of the quantum trajectory8 of an optically trapped nanoparticle. We combine confocal position sensing close to the Heisenberg limit with optimal state estimation via Kalman filtering to track the particle motion in phase space in real time with a position uncertainty of 1.3 times the zero-point fluctuation. Optimal feedback allows us to stabilize the quantum harmonic oscillator to a mean occupation of 0.56 ± 0.02 quanta, realizing quantum ground-state cooling from room temperature. Our work establishes quantum Kalman filtering as a method to achieve quantum control of mechanical motion, with potential implications for sensing on all scales. In combination with levitation, this paves the way to full-scale control over the wavepacket dynamics of solid-state macroscopic quantum objects in linear and nonlinear systems.
Every massive particle behaves like a wave, according to quantum physics. Yet, this characteristic wave nature has only been observed in double-slit experiments with microscopic systems, such as atoms and molecules. The key aspect is that the wavefunction describing the motion of these systems extends coherently over a distance comparable to the slit separation, much larger than the size of the system itself. Preparing these states of more massive and complex objects remains an outstanding challenge. While the motion of solid-state oscillators can now be controlled at the level of single quanta, their coherence length remains comparable to the zero-point motion, limited to subatomic distances. Here, we prepare a delocalized state of a levitating solid-state nanosphere with coherence length exceeding the zero-point motion. We first cool its motion to the ground state. Then, by modulating the stiffness of the confinement potential, we achieve more than a threefold increment of the initial coherence length with minimal added noise. Optical levitation gives us the necessary control over the confinement that other mechanical platforms lack. Our work is a stepping stone towards the generation of delocalization scales comparable to the object size, a crucial regime for macroscopic quantum experiments, and towards quantum-enhanced force sensing with levitated particles.