Quantum coherence between energy eigenstates of harmonic oscillators is essential for quantum physics. Even the most elementary binary superpositions of the ground and the higher eigenstate are highly required for quantum sensing, thermodynamics, and computing. We derive upper bounds for quantum coherences achieved by classical and Gaussian states and operations and, subsequently, obtain a hierarchy of the thresholds for the off-diagonal elements necessary to reach genuine quantum non-Gaussian coherences. The presented analysis demonstrates that certification based solely on estimation of coherences can cover the quantum non-Gaussian states, which are undetectable by the criteria based solely on the estimation of the corresponding state populations. We experimentally demonstrate the unambiguous observation of quantum non-Gaussian coherences in mechanical vibrations of a single calcium ion up to the superposition of zero and six phonons. The analysis of the robustness with respect to pure dephasing in a motional Ramsey experiment demonstrates the feasibility of their storage for up to more than 20 ms for superpositions with a large energy difference of participating number states. The presented observations prove that atomic oscillations go deeply into a diverse area of discrete quantum non-Gaussian coherent phenomena critical for their applications.
Quantum coherence between energy eigenstates of harmonic oscillators is essential for quantum physics. Even the most elementary binary superpositions of the ground and the higher eigenstate are highly required for quantum sensing, thermodynamics, and computing. We derive upper bounds for quantum coherences achieved by classical and Gaussian states and operations and, subsequently, obtain a hierarchy of the thresholds for the off-diagonal elements necessary to reach genuine quantum non-Gaussian coherences. The presented analysis demonstrates that certification based solely on estimation of coherences can cover the quantum non-Gaussian states, which are undetectable by the criteria based solely on the estimation of the corresponding state populations. We experimentally demonstrate the unambiguous observation of quantum non-Gaussian coherences in mechanical vibrations of a single calcium ion up to the superposition of zero and six phonons. The analysis of the robustness with respect to pure dephasing in a motional Ramsey experiment demonstrates the feasibility of their storage for up to more than 20 ms for superpositions with a large energy difference of participating number states. The presented observations prove that atomic oscillations go deeply into a diverse area of discrete quantum non-Gaussian coherent phenomena critical for their applications.
Quantum non-Gaussian states of photons and phonons are conclusive and direct witnesses of higher-than-quadratic nonlinearities in optical and mechanical processes. Moreover, they are proven resources for quantum sensing, communication and error correction with diverse continuous-variable systems. This review introduces theoretical analyses of nonclassical and quantum non-Gaussian states of photons and phonons. It recapitulates approaches used to derive operational criteria for photons tolerant to optical losses, their application in experiments and their nowadays extension to quantum non-Gaussian photon coincidences. It extends to a recent comparison of quantum non-Gaussianity, including robustness to thermal noise, and sensing capability for high-quality phononic Fock states of single trapped cooled ions. The review can stimulate further development in the criteria of quantum non-Gaussian states and experimental effort to prepare and detect such useful features, navigating the community to advanced quantum physics and technology.
Quantum non-Gaussian (QNG) mechanical states from inherently nonlinear quantum processes are already required in quantum sensing, become essential in quantum thermodynamics, and also open directions in quantum computing with continuous variables. The discrete building blocks of such states are the energy eigenstates - Fock states. Despite the progress in their experimental preparation, the remaining energy uncertainty can still invisibly cause loss of the critical quantum non-Gaussian aspects of the phonon distribution relevant for the applications.
Quantum non-Gaussian mechanical states are already required in a range of applications. The discrete building blocks of such states are the energy eigenstates-Fock states. Despite progress in their preparation, the remaining imperfections can still invisibly cause loss of the aspects critical for their applications. We derive and apply the most challenging hierarchy of quantum non-Gaussian criteria on the characterization of single trapped-ion oscillator mechanical Fock states with up to 10 phonons. We analyze the depth of these quantum non-Gaussian features under intrinsic mechanical heating and predict their requirement for reaching quantum advantage in the sensing of a mechanical force.
The generation of high Fock states of light pulses and their superpositions with provable quantum non-Gaussian features is still very challenging, although the power of conditional methods to herald the approximate state from the available Gaussian states is growing. The atom-light interaction in the high- cavity has been considered a viable alternative to the heralded Fock states of the light pulses from nonlinear optics limited to three-photon Fock states for the last decade. Here, by optimizing the realistic protocol combining it with available optical delay elements, we conclusively predict filtering of Fock states up to ten photons with a high success rate of 20 % using a hierarchy of quantum non-Gaussian criteria. Moreover, the filtering protocol enables the preparation of superposition of Fock states, and we analyze this emerging case up to two photons with provable quantum non-Gaussian coherence and high success rate of 50 % . To demonstrate their quality for applications, we evaluate the robustness of such features, the bunching capability in a linear network, and the sensing capability to estimate the magnitude of unknown force, noise, and phase. These assessments outline the essential conditions and application criteria for realistic optical cavity QED interaction on light pulses to outperform photon detection methods.
Non-Gaussianity is a trademark of bosonic quantum states and a critical resource for advancing quantum technologies like fault-tolerant quantum computing, quantum networks, and high-precision metrology [1]. Unlike Gaussian states, non-Gaussian states cannot be efficiently simulated or characterized using classical methods due to the absence of a canonical representation [2]. In recent years, our group has developed robust capabilities in quantum state engineering and networking applications, exemplified by our generation of non-Gaussian states [3]. However, non-Gaussianity alone does not capture the application-specific properties required for many quan-tum tasks, such as error correction and sensing, where quantum coherence plays an important role. To build on these efforts, we propose a hierarchical framework for assessing non-Gaussian coherence, tailored to the specific requirements of various quantum applications [4].
A trapped-ion harmonic oscillator represents a rich and well-controlled platform for tests of quantum physics, with applications to quantum simulations, quantum sensing, and quantum information processing. Owing to its net charge, the ion's motion is affected by changes in the electric potential. Consequently, electric field and potential curvature noise will limit the coherence of the ion's harmonic oscillation. While in some respects, this serves as a limitation in the performance of the trapped ion system (for example, in the fidelity of two-qubit gates or quantum simulations with motional quanta), it also opens an opportunity to use the ion as a precise field sensor and to use engineered quantum states of motion to enhance the sensitivity to these fields beyond the standard quantum limit (SQL). This thesis describes the implementation of such applications on a single beryllium ion confined in a Paul trap. In the thesis, I present the theory of an ideal harmonic oscillator and the implementation of this system using the motion of a single trapped ion, including producing special quantum states of motion; these states include the energy eigenstates of the harmonic oscillator, called number states, up to n=100, superpositions of number states of the form (1/√2)(|0> + |n>), with n up to 18, and coherently displaced number states with an average occupation up to approximately 300. I describe how we use these quantum states of motion for precise sensing of fluctuations of the harmonic oscillator frequency. The sensitivity of the (1/√2)(|0> + |n>) state ideally follows the 1/n Heisenberg scaling for frequency sensitivity. Additionally, I describe investigations of the spectrum of motional frequency noise using a series of coherent displacements of the motion of the ion, with features similar to Ramsey and dynamical decoupling sequences for two-level systems. While these displaced states don't improve sensitivity over the SQL, they can be simply and rapidly implemented with trapped ions. I discuss extensions to all of these experiments, including to multiple ions in a new trap designed to confine 3 or 4 ions in individually tunable potential wells.